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Time-Resolved Two-Photon Quantum Interference

T. Legero, Tatjana Wilk, A. Kuhn, G. Rempe

Published Jan 1, 2003• 113 citations
OpenAlex

Abstract

Abstract The interference of two independent single-photon pulses impinging on a beam splitter is analysed in a generalised time-resolved manner. Different aspects of the phenomenon are elaborated using different representations of the single-photon wave packets, like the decomposition into single-frequency field modes or spatio-temporal modes matching the photonic wave packets. Both representations lead to equivalent results, and a photon-by-photon analysis reveals that the quantum-mechanical two-photon interference can be interpreted as a classical one-photon interference once a first photon is detected. A novel time-dependent quantum-beat effect is predicted if the interfering photons have different frequencies. The calculation also reveals that full two-photon fringe visibility can be achieved under almost any circumstances by applying a temporal filter to the signal. PACS 42.50.Dv, 42.50.Ct 1

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Abstract The interference of two independent single-photon pulses impinging on a beam splitter is analysed in a generalised time-resolved manner. Different aspects of the phenomenon are elaborated using different representations of the single-photon wave packets, like the decomposition into single-frequency field modes or spatio-temporal modes matching the photonic wave packets. Both representations lead to equivalent results, and a photon-by-photon analysis reveals that the quantum-mechanical two-photon interference can be interpreted as a classical one-photon interference once a first photon is detected. A novel time-dependent quantum-beat effect is predicted if the interfering photons have different frequencies. The calculation also reveals that full two-photon fringe visibility can be achieved under almost any circumstances by applying a temporal filter to the signal. PACS 42.50.Dv, 42.50.Ct 1
The interference of two single photons impinging on a beam splitter is measured in a time-resolved manner. Using long photons of different frequencies emitted from an atom-cavity system, a quantum beat with a visibility close to 100% is observed in the correlation between the photodetections at the output ports of the beam splitter. The time dependence of the beat amplitude reflects the coherence properties of the photons. Most remarkably, simultaneous photodetections are never observed, so that a temporal filter allows one to obtain perfect two-photon coalescence even for nonperfect photons.
Summary form only given. Consider an experiment where a single photon is split into two wave-packets by a beam splitter and where the two wave packets are made to overlap in a specific region in space. If the two wave-packets arrive at the same time, an interference pattern can be recorded by a classical detector such as a photographic plate. If however, the difference in arrival time between the two wave-packets is made to be larger than the coherence time of the wave packets, the interference pattern, as recorded by the detector, will disappear. It has been argued that if the classical detector is replaced by a material that can remember the phase of the electromagnetic field, i.e. a material with a long homogeneous dephasing time, it would be possible to record the interference between the two wave-packets even if the time difference between them is much larger than the coherence time. We denote this single-photon self-interference. The interference pattern would take the form of a frequency dependent population grating in the material and could be detected by diffracting a light pulse on this grating. The delayed single-photon self-interference experiment has several unique features. It is a four-wave mixing experiment where the two first pulses share a total of only one photon. Thus interaction between these two pulses and the material, normally considered as a nonlinear multiphoton process, is here carried out by a single photon. We have performed experiments with multiphoton excitation pulses and extrapolated the data to the single photon level. These experiments support the conclusion from the theoretical calculations that delayed single-photon self-interference could be observed.
The distinguishing of the multiphoton quantum interference effect from the classical one forms one of the most important issues in modern quantum mechanics and experimental quantum optics. For a long time, the two-photon interference (TPI) of correlated photons has been recognized as a pure quantum effect that cannot be simulated with classical lights. In the meantime, experiments have been carried out to investigate the classical analogues of the TPI. In this study, we conduct TPI experiments with uncorrelated photons with different center frequencies from a luminescent light source, and we compare our results with the previous ones of correlated photons. The observed TPI fringe can be expressed in the form of three phase terms related to the individual single-photon and two-photon states, and the fringe pattern is strongly affected by the two single-photon-interference fringes and also by their visibilities. With the exception of essential differences such as valid and accidental coincidence events within a given resolving time and the two-photon spectral bandwidth, the interference phenomenon itself exhibits the same features for both correlated and uncorrelated photons in the single-photon counting regime.
We present time-resolved diffraction and two-slit interference experiments using a streak camera as a detector for femtosecond pulses of photons. These experiments show how the diffraction pattern is built by adding frames of a few photons to each frame. It is estimated that after 300 photons the diffraction pattern emerges. With time resolution we can check the speed of light and put an upper limit of 2 ps at our resolution to the time for wave function collapse in the quantum measurement process. We then produce interference experiments with photons of different energies impinging on the slits, i.e. we know which photon impinges on each slit. We show that for poor time resolution, no interference is observed, but for high time resolution, we have interference that is revealed as beats of 100 GHz frequency. The condition for interference is that the two pulses should overlap spatially at the detector, even if the pulses have different energies but are generated from the same pulse of the laser. The interference seems to be in agreement with classical theory at first sight. However, closer study and analysis of the data show deviations in the visibility of the interference fringes and of their phase. These experiments are discussed in connection with quantum mechanics and it may be concluded that the time resolution provides new data for understanding the longstanding and continuing arguments on wave-particle duality initiated by Newton, Young, Fresnel, Planck and others. A thought experiment is presented in the appendix to try to distinguish the photons at the detector by making it sensitive to colour.
Two-photon interference (TPI) is a fundamental phenomenon in quantum optics and plays a crucial role in optical quantum technologies. TPI is commonly considered as quantum interference with an upper bound of 100% for both the TPI and the beat visibility in contrast to its classical counterpart with a maximum visibility of 50%. However, this is not always the case. Here, we report a simultaneous observation of quantum and classical TPI of single photons with ultralong coherence time, which is five orders of magnitude longer than the photon correlation time. We observe a TPI visibility of 94.3% ± 0.2% well above the 50% classical limit indicating the quantum feature, and a beat visibility of 50% reflecting the classical feature. In addition an anti-bunching central dip due to single-photon anti-correlation, we also observe two bunching side peaks in cross correlation curves for indistinguishable photons. Using the general wave superposition theory and the quantum field approach, we derive the same cross correlation functions, which fully reproduce and explain the experiments. Our results reveal that the quantum and classical features of TPI result from the same interference, as the fourth-order temporal interference arises from the second-order temporal interference between two photons on the timescale of the photon coherence time.
We report two-photon interference with continuous-wave multi-mode coherent light. We show that the two-photon interference, in terms of the detection time difference, reveals two-photon beating fringes with the visibility V = 0.5. While scanning the optical delay of the interferometer, Hong-Ou-Mandel dips or peaks are measured depending on the chosen detection time difference. The HOM dips/peaks are repeated when the optical delay and the first-order coherence revival period of the multi-mode coherent light are the same. These results help to understand the nature of two-photon interference and also can be useful for quantum information science.