For most kinds of already known Bose-Einstein condensates experimental evidence for the existence of a macroscopic coherent quantum state has been provided, e.g., from the observation of interference phenomena, the formation vortices, the detection of Josephson effects, or even by the manifestation of superfluid behaviour. However, none of these hallmarks for a true, macroscopic phase-coherent state has ever been reported for any insulating spin system in a solid in which magnetic bosonic quasiparticles are thought to condense close to a quantum critical point. We describe an attempt to detect superfluid behaviour in TlCuCl3, and discuss in more detail a proposal for an experiment in which the a.c. Josephson effect can be probed by using a device composed of two weakly coupled magnetic insulators with different critical fields. We conclude that the detection of the a.c. Josephson effect is feasible for a proper choice of compounds with realistic material parameters.
For most kinds of already known Bose-Einstein condensates experimental evidence for the existence of a macroscopic coherent quantum state has been provided, e.g., from the observation of interference phenomena, the formation vortices, the detection of Josephson effects, or even by the manifestation of superfluid behaviour. However, none of these hallmarks for a true, macroscopic phase-coherent state has ever been reported for any insulating spin system in a solid in which magnetic bosonic quasiparticles are thought to condense close to a quantum critical point. We describe an attempt to detect superfluid behaviour in TlCuCl3, and discuss in more detail a proposal for an experiment in which the a.c. Josephson effect can be probed by using a device composed of two weakly coupled magnetic insulators with different critical fields. We conclude that the detection of the a.c. Josephson effect is feasible for a proper choice of compounds with realistic material parameters.
For most kinds of already known Bose-Einstein condensates experimental evidence for the existence of a macroscopic coherent quantum state has been provided, e.g., from the observation of interference phenomena, the formation vortices, the detection of Josephson effects, or even by the manifestation of superfluid behaviour. However, none of these hallmarks for a true, macroscopic phase-coherent state has ever been reported for any insulating spin system in a solid in which magnetic bosonic quasiparticles are thought to condense close to a quantum critical point. We describe an attempt to detect superfluid behaviour in TlCuCl 3 , and discuss in more detail a proposal for an experiment in which the a.c. Josephson effect can be probed by using a device composed of two weakly coupled magnetic insulators with different critical fields. We conclude that the detection of the a.c. Josephson effect is feasible for a proper choice of compounds with realistic material parameters.
The alternating current (ac) Josephson effect in a time-independent spatially inhomogeneous setting is manifested by the occurrence of Josephson oscillations---periodic macroscopic phase-induced collective motions of the quantum condensate. So far, this phenomenon was observed at cryogenic temperatures in superconductors, in superfluid helium, and in Bose-Einstein condensates (BECs) of trapped atoms. Here, we report on the discovery of the ac Josephson effect in a magnon BEC carried by a room-temperature ferrimagnetic film. The BEC is formed in a parametrically populated magnon gas in the spatial vicinity of a magnetic trench created by a dc electric current. The appearance of the Josephson effect is manifested by oscillations of the magnon BEC density in the trench, caused by a coherent phase shift between this BEC and the BEC in the nearby regions. Our findings advance the physics of room-temperature macroscopic quantum phenomena and will allow for their application for data processing in magnon spintronics devices.
The recent experimental advances in the field of quantum spin materials have led to well-controlled systems which can be used in order to simulate complex quantum models in a clean fashion. Here we discuss how fascinating effects normally known from bosonic systems such as the Bose-Einstein condensation can be investigated with the help of such materials. We discuss as an example how a crossover between an effectively one-dimensional geometry described by a Luttinger liquid to a three-dimensional Bose-Einstein condensation can be induced. Additionally, we point out how more complex phases as the Bose-glass phase could be realized in these quantum magnets. Introduction Although it can seem paradoxical, the quantum magnetic states found in insulators offer an interesting route to study Bose-Einstein condensation (BEC) and more generally phenomena related to itinerant, interacting bosonic systems. In many materials, the repulsion between the electrons causes the ground state to be a Mott insulator with one electron localized per site. In such a case, the charge degrees of freedom are completely locked by large charge gaps (usually of the order of tens of electron volts). However, one can study the fascinating physics of the spin degrees of freedom. As was shown a long time ago, the localized spins are coupled by a so-called superexchange which may be ferro- or antiferromagnetic. The properties of the exchange coupling between the spins depend mainly on the underlying atomic structure of the material. The resulting physics is extremely rich and such materials can have a host of phases ranging from ordered magnetic phases to so-called spin-liquid phases in which spin–spin correlations decay extremely fast with distance. The field of research concerning these materials, dubbed quantum magnetism, is thus an extremely active field in its own right [1]. Additionally, one can exploit the formal mapping that exists between spin operators and bosonic ones, as will be described in the next section, to connect the magnetic materials to itinerant bosonic systems with interactions between the bosons. This opens the way to use such quantum spin systems as quantum simulators. A quantum simulator means that the experimental system can be employed in order to “solve” in a controlled way a problem/Hamiltonian known from a different less controlled physical realization, e.g., inspired by fundamental many-body physics, quantum information or computational applications.
Bose-Einstein condensation (BEC) is a quantum phenomenon of formation of the collective quantum state, in which the macroscopic number of particles occupies the lowest energy state and thus is governed by a single wave function. Here we highlight the BEC in a magnetic subsystem -- the BEC of magnons, elementary magnetic excitations. Magnon BEC is manifested as the spontaneously emerging state of the precessing spins, in which all spins precess with the same frequency and phase even in the inhomogeneous magnetic field. We consider this phenomenon on example of spin precession in superfluid phases of 3He. The magnon BEC in these phases has all the properties of spin superfluidity. The states of the phase-coherent precession belong to the class of the coherent quantum states, which manifest themselves by superfluidity, superconductivity, quantum Hall effect, Josephson effect and many other macroscopic quantum phenomena.
A quantised spin wave – magnon – in magnetic films can undergo Bose-Einstein condensation (BEC) into two energetically degenerate lowest-energy quantum states with nonzero wave vectors ±k BEC . This corresponds to two interfering condensates forming spontaneously in momentum space. Brillouin Light Scattering studies for a microwavepumped film with submicrometer spatial resolution experimentally confirm the existence of the two wavefunctions and show that their interference results in a nonuniform ground state of the condensate with the density oscillating in space. Moreover, fork dislocations in the density fringes provide direct experimental evidence for the formation of pinned half-quantum vortices in the magnon condensate. The measured amplitude of the density oscillation implies the formation of a nonsymmetric state that corresponds to nonequal occupation of two energy minima. We discuss the experimental findings and consider the theory of magnon condensates, which includes, to leading order, the contribution from the noncondensed magnons. The effect of the noncondensed magnon cloud is to increase the contrast of the asymmetric state and to bring about the experimental measurements. Introduction Magnons are quasiparticles corresponding to quantised spin waves that describe the collective motion of spins [1]. In recent years, it has become possible to realise a BEC of magnons in two remarkably different systems: in superfluid phases of an isotope of helium – Helium-3 at ultralow temperatures [2, 3] and in ferrimagnetic insulators [4, 5, 6, 7]. In the normal, noncondensed state, these magnetic materials exhibit a magnetically ordered state with a gas of magnons whose phases are not correlated. However, once condensation occurs, spins develop phase coherence resulting in a common global frequency and phase of precession. At room temperature, ferrimagnetic insulators, such as yttrium-iron garnet (YIG) films, together with a combination of an in-plane magnetic field and microwave radiation, are required for the magnon condensation [4, 5, 6, 7]. Therefore, in analogy with exciton– polariton condensates, this provides yet another example of a BEC of quasiparticle excitations in a solid-state system. Experimental Realisation of a Bose-Einstein Condensate of Magnons in an Epitaxial YIG-film A room-temperature Bose-Einstein condensate of magnons was created in an epitaxial YIG-film using an experimental setup shown in Fig. 25.1a, which, in general, is similar to that used in our previous studies [4, 5]. Given that magnons are quasiparticle excitations, their number is not conserved and, therefore, the chemical potential is zero.
Abstract The spontaneous emergence of coherence is a defining feature of multibody quantum systems, underlying phenomena from superconductivity to quantum information processing. Although Bose–Einstein condensates provide a unique setting for studying this process, direct observation of how a condensate acquires a coherent global phase has remained challenging. Here we provide evidence of spontaneous phase formation in a magnon Bose–Einstein condensate. Using a phase-referenced detection technique, we track the phase of the condensate coherent state relative to an external reference, revealing how an initially incoherent magnon gas thermalizes and undergoes a spontaneous transition into a coherent quantum state with a well-defined macroscopic phase. This observation provides evidence of spontaneous symmetry breaking in a quasiparticle condensate, confirming a central prediction of Bose–Einstein condensation theory that extends across diverse quantum systems.