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Optics and Spectroscopy

Resonance broadening and lifetime of the 3 1 P 0 1 level of Mg I

Жувикин Георгий Викторович, N. P. Penkin, L. N. Shabanova

Published Nov 1, 1976• 3 citations
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MAGNETIC RESONANCE MEASUREMENT OF THE "COHERENCE TIME" OF Hg$sup 199$ AND Hg$sup 201$ ISOTOPES

F. Hartmann-Boutron, J.-P. Barratt, J. Brossel

A study of the 6/sup 3/P/sub 1/ level of isotope pairs of Mg by magnetic resonance methods leads to the determination of a coherence time'' which is much longer than the duration of the life of the level. At very low vapor densities, the coherence time'' approaches the level lifetime. Experimental resilts verified that the coherence time'' is dependent only on the number of diffusing atoms and on the obseved hypefiine level and that it approaches the level lifetime. (J.S.R.)

Compt. rend.•Dec 16, 1957•0 citations
We have measured the lifetime of the 3P1^{3}P_{1}3P1​ metastable state of Mg and obtained a value of 2.2 \ifmmode\pm\else\textpm\fi{} 0.2 msec. The level was excited with a dye laser tuned to the intercombination line ($3s3p^{3}P_{1}\ensuremath{\leftrightarrow}3{s}^{2}^{1}S_{0}$). In addition to the 3P1^{3}P_{1}3P1​ state, the 3P2^{3}P_{2}3P2​ and 3P0^{3}P_{0}3P0​ levels were populated by mixing collisions owing to the presence of an inert buffer gas. The populations of all three metastable levels were monitored as a function of time by observing the absorption of Mg resonance radiation ($^{3}P_{0,1,2}\ensuremath{\rightarrow}^{3}S_{1}$) out of each level. The mixing time was short compared to the 3P1^{3}P_{1}3P1​ lifetime, so that the populations of the three metastable levels were in thermal equilibrium with each other. This produced an apparent lengthening of the 3P1^{3}P_{1}3P1​ lifetime, which would introduce a large systematic error if the degree of mixing were not known. Cenventionally, one observes the fluorescence from the excited levels to obtain their lifetimes. Because the lifetimes of the 3P2^{3}P_{2}3P2​ and 3P0^{3}P_{0}3P0​ states are too long, fluorescence from these states cannot be observed, and the observation of fluorescence from the 3P1^{3}P_{1}3P1​ state alone provides insufficient information to determine its lifetime.
The lifetime of the metastable 3P1^{3}P_{1}3P1​ state of Mg has been remeasured by a dye-laser excitation technique. The metastable state was populated by an intense pulse of 4571-\AA{} radiation from a flashlamp-pumped dye laser, and the decay of the population was monitored by observing the absorption of 5173-\AA{} resonance radiation from a Mg discharge lamp. The measured value for the 3P1^{3}P_{1}3P1​ lifetime is 4.5 \ifmmode\pm\else\textpm\fi{} 0.5 msec.
MAGNETIC RESONANCE MEASUREMENT OF THE "COHERENCE TIME" OF Hgsup199sup 199sup199 AND Hgsup201sup 201sup201 ISOTOPES
A study of the 6/sup 3/P/sub 1/ level of isotope pairs of Mg by magnetic resonance methods leads to the determination of a coherence time'' which is much longer than the duration of the life of the level. At very low vapor densities, the coherence time'' approaches the level lifetime. Experimental resilts verified that the coherence time'' is dependent only on the number of diffusing atoms and on the obseved hypefiine level and that it approaches the level lifetime. (J.S.R.)