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Journal of Experimental and Theoretical Physics

Chaotic Walking of Cold Atoms in a 2D Optical Lattice

Sergey V. Prants

Published Sep 1, 2020• 4 citations
Publisher

Abstract

Abstract Coherent dynamics of cold atoms in a 2D optical lattice with interfering laser beams is studied with account for internal and external degrees of freedom of an atom. A system of differential equations for coupled degrees of freedom obtained in the semiclassical approximation has regular and chaotic solutions depending on the atomic-field detuning from resonance. The Hamilton chaos is manifested in the form of chaotic Rabi oscillations and random walks of cold atoms in the lattice for relatively small resonance detunings. It is shown that the deterministic chaos appears as a result of jumps in the value of the electric dipole moment of an atom approaching the nodes of a 2D standing wave. This in turn causes a pseudorandom behavior of momenta of atoms and, as a consequence, their random walks in the absolutely rigid 2D optical lattice without any external modulation of its parameters. It is shown in numerical experiments with 106 atoms that their distributions over the lattice for different resonance detunings differ significantly. This fact can be used for detecting the effect of random walks of cold atoms in a real experiment by the absorption image method.

DOI
10.1134/s106377612008004x

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Abstract Coherent dynamics of cold atoms in a 2D optical lattice with interfering laser beams is studied with account for internal and external degrees of freedom of an atom. A system of differential equations for coupled degrees of freedom obtained in the semiclassical approximation has regular and chaotic solutions depending on the atomic-field detuning from resonance. The Hamilton chaos is manifested in the form of chaotic Rabi oscillations and random walks of cold atoms in the lattice for relatively small resonance detunings. It is shown that the deterministic chaos appears as a result of jumps in the value of the electric dipole moment of an atom approaching the nodes of a 2D standing wave. This in turn causes a pseudorandom behavior of momenta of atoms and, as a consequence, their random walks in the absolutely rigid 2D optical lattice without any external modulation of its parameters. It is shown in numerical experiments with 106 atoms that their distributions over the lattice for different resonance detunings differ significantly. This fact can be used for detecting the effect of random walks of cold atoms in a real experiment by the absorption image method.
The possibility of experimental observation of chaotic motion of cold atoms in a one-dimensional rigid optical lattice without any modulation of its parameters and additional impact is demonstrated theoretically and numerically. This effect of deterministic chaos arises near the optical resonance due to the nonlinear coupling of electronic and mechanical degrees of freedom in the atom. In a certain range of resonance detunings, at each crossing of the lattice-forming standing wave node by the atom, the atomic dipole moment changes pseudorandomly in a step-like manner, accompanied by an appropriate change in the atom momentum. This leads to the effect of chaotic wandering of atoms, possessing the properties of the classical deterministic chaos, namely, to the exponential sensitivity of atomic trajectories to small variations of the initial conditions and/or the control parameters. With time, part of atoms from the initial cloud changes the direction of their motion to the opposite one, which can be detected in a real experiment. Numerical experiments with lithium atoms with the spontaneous emission taken into account show that by varying the laser radiation intensity (normalised detuning of resonance) in the rigid optical lattice, one can implement the transition from the regular regime of the atomic motion to the chaotic wandering in a real experiment.
Abstract This paper is a review article on some aspects of quantum–classical correspondence in chaotic dynamics of cold atoms interacting with a standing-wave laser field forming an optical lattice. The problem is treated from both (semi)classical and quantum points of view. In both approaches, the interaction of an atomic electic dipole with the laser field is treated quantum mechanically. Translational motion is described, at first, classically (atoms are considered to be point-like objects) and then quantum mechanically as a propagation of matter waves. Semiclassical equations of motion are shown to be chaotic in the sense of classical dynamical chaos. Point-like atoms in an absolutely deterministic and rigid optical lattice can move in a random-like manner demonstrating a chaotic walking with typical features of classical chaos. This behavior is explained by random-like ‘jumps’ of one of the atomic internal variable when atoms cross nodes of the standing wave and occurs in a specific range of the atom-field detuning. When treating atoms as matter waves, we show that they can make nonadiabatic transitions when crossing the standing-wave nodes. The point is that atomic wave packets split at each node in the same range of the atom-field detuning where the classical chaos occurs. The key point is that the squared amplitude of those semiclassical ‘jumps’ equal to the quantum Landau–Zener parameter which defines the probability of nonadiabatic transitions at the nodes. Nonadiabatic atomic wave packets are much more complicated compared to adiabatic ones and may be called chaotic in this sense. A few possible experiments to observe some manifestations of classical and quantum chaos with cold atoms in horizontal and vertical optical lattices are proposed and discussed.
We treat semiclassical nonlinear dynamics of a two-level atom in the strong standing-wave field created in a high-quality cavity and in a free space with the help of two counterpropagating laser beams. First of all, we consider the dynamics of the strongly coupled atom-field system in an ideal cavity without any losses and discuss briefly nonlinear dynamical effects of random walking of an atom in a fully deterministic standing wave and Hamiltonian dynamical fractals. Then we study how these effects change in a free space when we take into account relaxation and external pumping of the standing wave. We discuss briefly new dissipative effects of synchronization between electronic and mechanical degrees of freedom of atoms, limit cycles of different periods and their bifurcations, and strange atomic attractors. Finally, we treat spontaneous relaxation as a random events in the equations of motion and study what happens with atomic fractality and limit cycles. It is shown that a self-similar structure of the scattering function (at least, on a few first levels) is conserved in the presence of spontaneous jumps. As to limit cycles, we could not resolve limit cycles of different period, but the fact of synchronization of internal and external atomic degrees of freedom is strictly established in the system with spontaneous jumps.
We study dissipative transport of spontaneously emitting atoms in a one-dimensional (1D) standing-wave laser field in the regimes where the underlying deterministic Hamiltonian dynamics is regular and chaotic. A Monte Carlo stochastic wave-function method is applied to simulate semiclassically the atomic dynamics with coupled internal and translational degrees of freedom. It is shown in numerical experiments and confirmed analytically that chaotic atomic transport can take the form either of ballistic motion or a random walking with specific statistical properties. The character of spatial and momentum diffusion in the ballistic atomic transport is shown to change abruptly in the atom-laser detuning regime where the Hamiltonian dynamics is irregular in the sense of dynamical chaos. We find a clear correlation between the behavior of the momentum diffusion coefficient and Hamiltonian chaos probability which is a manifestation of chaoticity of the fundamental atom-light interaction in the diffusivelike dissipative atomic transport. We propose to measure a linear extent of atomic clouds in a 1D optical lattice and predict that, beginning with those values of the mean cloud's momentum for which the probability of Hamiltonian chaos is close to 1, the linear extent of the corresponding clouds should increase sharply. A sensitive dependence of statistical characteristics of dissipative transport on the values of the detuning allows us to manipulate the atomic transport by changing the laser frequency.
We study the coupled translational and internal dynamics of a two-level atom in a spatially periodic optical potential created by a single-mode field in a high-finesse Fabry-Perot cavity. The strongly-coupled atom-cavity system with atomic center-of-mass motion included in modeled by semiclassical nonlinear Heisenberg equations of motion with two degrees of freedom. At exact resonance between the internal atomic transition and the cavity eigen frequency, the internal and translational degrees of freedom are separated from each other resulting in periodically modulated Rabi oscillations and regular translational motion. Near the atom-field resonance, the coupled dynamics is found to be irregular and even chaotic in the sense of external sensitivity to initial conditions. It is manifested as a chaotic motion of an atom in an absolutely regular spatially periodic potential in the absence of any random fluctuations. This effect may be explained as a result of the interaction of nonlinear resonances in the atom-field nonlinear pendulum whose low- frequency translational motion is modulated by the high- frequency Rabi oscillations. The irregular motion is studied in detail in numerical experiments using the arsenal of methods of the dynamical systems theory. The results obtained are compared with recent experiments with ultra cold single atoms interacting with single photons in the strong-coupling regime. We estimate the ranges of the system's control parameters, the detuning, the recoil frequency, and the mean number of intracavity photons, in which the interaction of nonlinear resonances may lead, under realistic conditions, to local instability of the center-of-mass motion and some manifestations of dynamical chaos, the effect which is of interest in studying the quantum-classical correspondence and quantum chaos in atomic optics.
Atoms, propagating across a detuned standing laser wave, can be scattered in a chaotic way even in the absence of spontaneous emission and any modulation of the laser field. Spontaneous emission masks the effect in some degree, but the Monte Carlo simulation shows that it can be observed in real experiments by the absorption imaging method or depositing atoms on a substrate. The effect of chaotic scattering is explained by a specific behavior of the dipole moments of atoms crossing the field nodes and is shown to depend strongly on the value of the atom-laser detuning.