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Physica Scripta

Quantum–classical correspondence in chaotic dynamics of laser-driven atoms

Sergei V Prants

Published Mar 6, 2017• 9 citations

Abstract

Abstract This paper is a review article on some aspects of quantum–classical correspondence in chaotic dynamics of cold atoms interacting with a standing-wave laser field forming an optical lattice. The problem is treated from both (semi)classical and quantum points of view. In both approaches, the interaction of an atomic electic dipole with the laser field is treated quantum mechanically. Translational motion is described, at first, classically (atoms are considered to be point-like objects) and then quantum mechanically as a propagation of matter waves. Semiclassical equations of motion are shown to be chaotic in the sense of classical dynamical chaos. Point-like atoms in an absolutely deterministic and rigid optical lattice can move in a random-like manner demonstrating a chaotic walking with typical features of classical chaos. This behavior is explained by random-like ‘jumps’ of one of the atomic internal variable when atoms cross nodes of the standing wave and occurs in a specific range of the atom-field detuning. When treating atoms as matter waves, we show that they can make nonadiabatic transitions when crossing the standing-wave nodes. The point is that atomic wave packets split at each node in the same range of the atom-field detuning where the classical chaos occurs. The key point is that the squared amplitude of those semiclassical ‘jumps’ equal to the quantum Landau–Zener parameter which defines the probability of nonadiabatic transitions at the nodes. Nonadiabatic atomic wave packets are much more complicated compared to adiabatic ones and may be called chaotic in this sense. A few possible experiments to observe some manifestations of classical and quantum chaos with cold atoms in horizontal and vertical optical lattices are proposed and discussed.

DOI: 10.1088/1402-4896/aa5f8f

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Abstract This paper is a review article on some aspects of quantum–classical correspondence in chaotic dynamics of cold atoms interacting with a standing-wave laser field forming an optical lattice. The problem is treated from both (semi)classical and quantum points of view. In both approaches, the interaction of an atomic electic dipole with the laser field is treated quantum mechanically. Translational motion is described, at first, classically (atoms are considered to be point-like objects) and then quantum mechanically as a propagation of matter waves. Semiclassical equations of motion are shown to be chaotic in the sense of classical dynamical chaos. Point-like atoms in an absolutely deterministic and rigid optical lattice can move in a random-like manner demonstrating a chaotic walking with typical features of classical chaos. This behavior is explained by random-like ‘jumps’ of one of the atomic internal variable when atoms cross nodes of the standing wave and occurs in a specific range of the atom-field detuning. When treating atoms as matter waves, we show that they can make nonadiabatic transitions when crossing the standing-wave nodes. The point is that atomic wave packets split at each node in the same range of the atom-field detuning where the classical chaos occurs. The key point is that the squared amplitude of those semiclassical ‘jumps’ equal to the quantum Landau–Zener parameter which defines the probability of nonadiabatic transitions at the nodes. Nonadiabatic atomic wave packets are much more complicated compared to adiabatic ones and may be called chaotic in this sense. A few possible experiments to observe some manifestations of classical and quantum chaos with cold atoms in horizontal and vertical optical lattices are proposed and discussed.

Abstract Coherent dynamics of cold atoms in a 2D optical lattice with interfering laser beams is studied with account for internal and external degrees of freedom of an atom. A system of differential equations for coupled degrees of freedom obtained in the semiclassical approximation has regular and chaotic solutions depending on the atomic-field detuning from resonance. The Hamilton chaos is manifested in the form of chaotic Rabi oscillations and random walks of cold atoms in the lattice for relatively small resonance detunings. It is shown that the deterministic chaos appears as a result of jumps in the value of the electric dipole moment of an atom approaching the nodes of a 2D standing wave. This in turn causes a pseudorandom behavior of momenta of atoms and, as a consequence, their random walks in the absolutely rigid 2D optical lattice without any external modulation of its parameters. It is shown in numerical experiments with 106 atoms that their distributions over the lattice for different resonance detunings differ significantly. This fact can be used for detecting the effect of random walks of cold atoms in a real experiment by the absorption image method.

The possibility of experimental observation of chaotic motion of cold atoms in a one-dimensional rigid optical lattice without any modulation of its parameters and additional impact is demonstrated theoretically and numerically. This effect of deterministic chaos arises near the optical resonance due to the nonlinear coupling of electronic and mechanical degrees of freedom in the atom. In a certain range of resonance detunings, at each crossing of the lattice-forming standing wave node by the atom, the atomic dipole moment changes pseudorandomly in a step-like manner, accompanied by an appropriate change in the atom momentum. This leads to the effect of chaotic wandering of atoms, possessing the properties of the classical deterministic chaos, namely, to the exponential sensitivity of atomic trajectories to small variations of the initial conditions and/or the control parameters. With time, part of atoms from the initial cloud changes the direction of their motion to the opposite one, which can be detected in a real experiment. Numerical experiments with lithium atoms with the spontaneous emission taken into account show that by varying the laser radiation intensity (normalised detuning of resonance) in the rigid optical lattice, one can implement the transition from the regular regime of the atomic motion to the chaotic wandering in a real experiment.

We study the motion of a cold atom in a frequency-modulated standing laser wave. If the detuning between the atomic electronic transition and the field is large, the atom moves in a modulated optical potential demonstrating known classical nonlinear effects such as chaos and nonlinear resonances. If the atom-field detuning is small, then two optical potentials emerge in the system, and the atom performs Landau-Zener (LZ) tunnelings between them. It is a radically non-classical behavior. However, we show that classical nonlinear structures in system's phase space (KAM-tori and chaotic layers) survive. Quantum effect of LZ tunnelings only induces small random jumps of trajectories between these structures (dynamical tunneling).

We study dissipative transport of spontaneously emitting atoms in a one-dimensional (1D) standing-wave laser field in the regimes where the underlying deterministic Hamiltonian dynamics is regular and chaotic. A Monte Carlo stochastic wave-function method is applied to simulate semiclassically the atomic dynamics with coupled internal and translational degrees of freedom. It is shown in numerical experiments and confirmed analytically that chaotic atomic transport can take the form either of ballistic motion or a random walking with specific statistical properties. The character of spatial and momentum diffusion in the ballistic atomic transport is shown to change abruptly in the atom-laser detuning regime where the Hamiltonian dynamics is irregular in the sense of dynamical chaos. We find a clear correlation between the behavior of the momentum diffusion coefficient and Hamiltonian chaos probability which is a manifestation of chaoticity of the fundamental atom-light interaction in the diffusivelike dissipative atomic transport. We propose to measure a linear extent of atomic clouds in a 1D optical lattice and predict that, beginning with those values of the mean cloud's momentum for which the probability of Hamiltonian chaos is close to 1, the linear extent of the corresponding clouds should increase sharply. A sensitive dependence of statistical characteristics of dissipative transport on the values of the detuning allows us to manipulate the atomic transport by changing the laser frequency.

A group-theoretical approach is applied to study the behavior of lossless two-level atoms in a standing-wave laser field. Due to the recoil effect, the internal and external atomic degrees of freedom become coupled. The internal dynamics is described quantum mechanically in terms of the SU (2) group parameters. The evolution operator is found in an explicit way after solving a single ODE for one of the group parameters. The translational motion in a standing wave is governed by the classical Hamilton equations which are coupled to the SU (2) group equations. It is shown that the full set of equations may be chaotic in some ranges of the control parameters and initial conditions. It means physically that there are regimes of motion with chaotic center-of-mass motion and irregular internal dynamics. It is established that the chaotic regime is specified by the character of oscillations of the group parameter characterizing the mean interaction energy between the atom and the laser field. It is shown that the effect of chaotic walking can be observed in a real experiment with cold atoms crossing a standing-wave laser field.

A semiclassical theory of chaotic atomic transport in a one-dimensional nondissipative optical lattice, when the standing-wave field and center-of-mass motion are treated classically, is developed. Using the basic equations of motion for the Bloch and translational atomic variables, we derive a stochastic map for the synchronized component of the atomic dipole moment that determines the center-of-mass motion. We find the analytical relations between the atomic and lattice parameters under which atoms typically alternate between flying through the lattice and being trapped in the wells of the optical potential. We use the stochastic map to derive formulas for the probability density functions (PDFs) for the flight and trapping events. Statistical properties of chaotic atomic transport strongly depend on the relations between the atomic and lattice parameters. We show that there is a good quantitative agreement between the analytical PDFs and those computed with the stochastic map and the basic equations of motion for different ranges of the parameters. Typical flight and trapping PDFs are shown to be broad distributions with power law segments with the slope $\ensuremath{-}1.5$ and exponential ``tails.'' The lengths of the power law and exponential segments of the PDFs depend on the values of the parameters. We find analytical conditions under which deterministic atomic transport has fractal properties and explain a hierarchical structure of the dynamical fractals.