Relaxation of quantum systems is a central problem in nonequilibrium physics. In contrast to classical systems, the underlying quantum dynamics results not only from atomic interactions but also from long-range coherence of the quantum system's wave function. Quantum dynamics of superfluids out of equilibrium was studied in various nonequilibrium realizations of superfluid helium, but also in turbulent relaxation of nonequilibrium, ultracold quantum gases. Such nonequilibrium states are usually created using moving objects or laser potentials, directly perturbing the system's density. However, the role of long-range phase coherence for the breakdown of quantum dynamics or the importance of coherence for the relaxation of quantum systems is still unexplored. Here, we unravel the contributions of density relaxation and coherent dynamics by studying a molecular Bose-Einstein condensate of Li atoms upon quenches of an optical speckle potential. We find that coherent dynamics breaks down one order of magnitude faster than the density of the quantum gas responds. Moreover, the system needs two orders of magnitude longer to reestablish long-range coherence and hence quantum dynamics, compared to the density response. Our results shed light on the importance of long-range coherence and the possibility of topologically robust phase excitations for the relaxation of nonequilibrium quantum systems. It thus suggests a possible route towards controlling quantum dynamics via nonequilibrium phase control.
Relaxation of quantum systems is a central problem in nonequilibrium physics. In contrast to classical systems, the underlying quantum dynamics results not only from atomic interactions but also from long-range coherence of the quantum system's wave function. Quantum dynamics of superfluids out of equilibrium was studied in various nonequilibrium realizations of superfluid helium, but also in turbulent relaxation of nonequilibrium, ultracold quantum gases. Such nonequilibrium states are usually created using moving objects or laser potentials, directly perturbing the system's density. However, the role of long-range phase coherence for the breakdown of quantum dynamics or the importance of coherence for the relaxation of quantum systems is still unexplored. Here, we unravel the contributions of density relaxation and coherent dynamics by studying a molecular Bose-Einstein condensate of Li atoms upon quenches of an optical speckle potential. We find that coherent dynamics breaks down one order of magnitude faster than the density of the quantum gas responds. Moreover, the system needs two orders of magnitude longer to reestablish long-range coherence and hence quantum dynamics, compared to the density response. Our results shed light on the importance of long-range coherence and the possibility of topologically robust phase excitations for the relaxation of nonequilibrium quantum systems. It thus suggests a possible route towards controlling quantum dynamics via nonequilibrium phase control.
Significance Understanding the combined effects of disorder and interactions in quantum many-body systems is a key topic of condensed matter physics. While most studies have considered a static disorder, here we investigate the relaxation dynamics of a three-dimensional Bose–Einstein condensate after switching on or off an optical disorder potential. We study, experimentally and numerically, the transient and steady-state atomic density distribution and the ability of the gas to hydrodynamically expand, directly reflecting long-range phase coherence. We find that, when the gas is exposed to disorder, long-range phase coherence breaks down one order of magnitude faster than the density distribution responds. In the opposite case, surprisingly, long-range coherence takes two orders of magnitude longer times to revive than the density relaxation.
Macroscopic coherence is an important feature of quantum many-body systems exhibiting collective behaviors, with examples ranging from atomic Bose-Einstein condensates, and quantum liquids to superconductors. Probing many-body coherence in a dynamically unstable regime, however, presents an intriguing and outstanding challenge in out-of-equilibrium quantum many-body physics. Here, we experimentally study the first- and second-order coherence of degenerate quasi-one-dimensional (1D) Bose gases quenched from repulsive to modulationally unstable attractive interaction regimes. The resulting dynamics, monitored by in situ density and matter-wave interference imaging, reveals phase-coherent density wave evolutions, clearly distinguished from iconic soliton trains previously observed in attractive gases. This arises from the interplay between noise-amplified density modulations and dispersive shock waves of broad interest in nonlinear physics, plasmas, granular systems, and beyond. At longer times, the gases become phase-scrambled, exhibiting a finite correlation length. Interestingly, following an interaction quench back to the repulsive regime, we observe that quasi-long-range coherence can be spontaneously re-established. This captivating rephasing dynamics can be attributed to the nucleation and annihilation of density defects in the quasi-1D geometry. These results shed light on out-of-equilibrium phase coherence in quantum many-body systems in a regime where beyond mean-field effects may arise and theoretical approaches have not been well-established. Attractive Bose gases are modulationally unstable yet exhibit rich nonlinear many-body behaviors, owing to the interplay between their coherence and unstable collective excitations. Here, the authors probe out-of-equilibrium dynamics in quasi-1D Bose-Einstein condensates subject to quench dynamics between repulsive and attractive interactions.
The kinetics of the formation of coherent correlation properties associated with Bose condensation is studied in detail. The evolution of a nonequilibrium state with no “condensate-seed” is related to a hierarchy of relaxation times. At the first stage, a particle flux in energy space toward low energies sets in. The evolution in this case is described by a nonlinear Boltzmann equation, with a characteristic time given by interparticle collisions. When the particles which will later form the condensate have a kinetic energy which is less than the potential energy, a quasicondensate starts to form. In this stage, fluctuations of the density (but not of the phase) are suppressed and short-range coherent correlation properties are governed by the equation of motion for a quasiclassical complex field. The next stage is connected with the formation of the long-range order. The time for forming topological order and therefore genuine superfluidity proves to be dependent on the system size. The off-diagonal long-range order, arising after the attenuation of long-wave phase fluctuations, has a size-dependent relaxation time as well. Introduction The problem of Bose–Einstein Condensation (BEC) kinetics, being interesting in itself, has acquired a special significance in connection with experimental efforts to observe this condensation in a number of systems with particles with a finite lifetime. Such systems include spin-polarized atomic hydrogen [1], excitons [2] and biexcitons [3] in semiconductors and, more recently, laser-cooled atomic systems [4].
In this thesis I report on experiments that enter a new regime in the many body physics of ultracold atomic gases. A Bose-Einstein condensate is loaded into a three-dimensional optical lattice potential formed by a standing wave laser light field. In this novel quantum system we have been able to both realize a quantum phase transition from a superfluid to a Mott insulator, and to observe the collapse and revival of a macroscopic matter wave field. Quantum phase transitions are driven by quantum fluctuations and occur, even at zero temperature, as the relative strength of two competing energy terms in the underlying Hamiltonian is varied across a critical value. In the first part of this work I report on the observation of such a quantum phase transition in a Bose-Einstein condensate with repulsive interactions, held in a three-dimensional optical lattice potential. In the superfluid ground state, each atom is spread-out over the entire lattice, whereas in the Mott insulating state, exact numbers of atoms are localized at individual lattice sites. We observed the reversible transition between those states and detected the gap in the excitation spectrum of the Mott insulator. A Bose-Einstein condensate is usually described by a macroscopic matter wave field. However, a quantized field underlies such a "classical" matter wave field of a Bose-Einstein condensate. The striking behavior of ultracold matter due to the field quantization and the nonlinear interactions between the atoms is the focus of the second part of this work. The matter wave field of a Bose-Einstein condensate is observed to undergo a series of collapses and revivals as time evolves. Furthermore, we show that the collisions between individual pairs of atoms lead to a fully coherent collisional phase shift in the corresponding many-particle state, which is a crucial cornerstone of proposed novel quantum computation schemes with neutral atoms. With these experiments we enter a new field of physics with ultracold quantum gases. In this strongly correlated regime, interactions between atoms dominate the behavior of the many-body system such that it can no longer be described by the usual theories for weakly interacting Bose gases. This novel quantum system offers the unique possibility to experimentally address fundamental questions of modern solid state physics, atomic physics, quantum optics, and quantum information.
Spontaneous pattern formation out of homogeneous media is one of the well-understood examples of hydrodynamic instabilities in classical systems, which naturally leads to the question of its manifestation in quantum fluids. Bose-Einstein condensates (BECs) of atomic gases have been an ideal platform for studying many-body quantum phenomena, such as superfluidity, and simultaneously providing an opportunity to broaden our understanding of classical hydrodynamics into quantum systems. In this review, we introduce a range of experimental studies on the pattern formation in quantum fluids of atomic gases under external driving, including Faraday waves in one and two dimensions, surface patterns, and counterflow instabilities in a mixture of superfluids. The pattern formation in the quantum system can be understood through the parametric amplification process, where an unstable dynamical mode can be exponentially amplified, similar to classical systems. Remarkably, the governing equations for surface excitations of trapped BECs can be mathematically equivalent to those of shallow water, indicating a universal description of the hydrodynamic instability across classical and quantum domains. However, the condensates, as superfluids, also possess fundamental quantum characteristics, such as quantized vorticity and a distinct dissipation channel. These unique features showcase many-body fragmentation under strong modulation and the generation of vortices in the nonlinear regime, which could offer a pathway to the study of quantum turbulence. Furthermore, the coexistence of long-range phase coherence and density modulation in driven condensates could provide unexplored features, such as those seen in supersolid-like sound modes, within nonequilibrium settings.
This thesis features fundamental experiments on the coherence properties of Bose-Einstein condensates (BEC) and atom lasers, made possible by a newly developed apparatus combining a Bose-Einstein condensate with an ultrahigh nesse optical cavity.Using the cavity as a single atom detector, atoms extracted from a trapped cloud are detected with unprecedented sensitivity, and the rst time-resolved counting of single atoms from a quantum degenerate source was demonstrated.O-diagonal long-range order is a dening property of a BEC and equivalent to longrange phase coherence.Its formation is a complex process accompanied by spontaneous symmetry breaking.We witnessed this formation in an ultracold cloud of 87 Rb atoms crossing the phase transition of BEC.Two overlapping atomic beams originating from dierent positions inside the condensate propagated downwards into the cavity.They showed a matter wave interference pattern with a visibility determined by the coherence of the probed regions.The modulation of the ux of atoms, recorded with single-atom resolution, yields the visibility, whereas its mean value gives information about the density of the sample.By shock cooling, a cloud of atoms was prepared in a highly nonequilibrium state slightly above the phase transition.While the ensemble subsequently relaxed, it crossed the phase transition into an equilibrium with a small condensate fraction.Employing our minimally invasive measurement method, the growth of both the rst-order coherence and the density of the sample was tracked in real time while the system crossed the phase transition.The growth of the coherence was found to start later, proceed faster and nish earlier than the increase in density.The coherent region increased at one fth of the speed of sound.Employing time-resolved single atom counting with the cavity detector, the full counting statistics of an atom laser beam was recorded.In a Hanbury Brown and Twiss type experiment, the second-order correlation function was found to be constant g (2) (τ ) = 1.00±0.01,proving the atom laser's second-order coherence and the absence of excess intensity uctuations that were observed in a pseudothermal beam.An analysis of the time interval distributions of atoms in the beam conrmed these ndings.The iii