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Ultracold quantum gases in three-dimensional optical lattice potentials

Markus Greiner

Published Jan 1, 2003• 67 citations
Publisher

Abstract

In this thesis I report on experiments that enter a new regime in the many body physics of ultracold atomic gases. A Bose-Einstein condensate is loaded into a three-dimensional optical lattice potential formed by a standing wave laser light field. In this novel quantum system we have been able to both realize a quantum phase transition from a superfluid to a Mott insulator, and to observe the collapse and revival of a macroscopic matter wave field. Quantum phase transitions are driven by quantum fluctuations and occur, even at zero temperature, as the relative strength of two competing energy terms in the underlying Hamiltonian is varied across a critical value. In the first part of this work I report on the observation of such a quantum phase transition in a Bose-Einstein condensate with repulsive interactions, held in a three-dimensional optical lattice potential. In the superfluid ground state, each atom is spread-out over the entire lattice, whereas in the Mott insulating state, exact numbers of atoms are localized at individual lattice sites. We observed the reversible transition between those states and detected the gap in the excitation spectrum of the Mott insulator. A Bose-Einstein condensate is usually described by a macroscopic matter wave field. However, a quantized field underlies such a "classical" matter wave field of a Bose-Einstein condensate. The striking behavior of ultracold matter due to the field quantization and the nonlinear interactions between the atoms is the focus of the second part of this work. The matter wave field of a Bose-Einstein condensate is observed to undergo a series of collapses and revivals as time evolves. Furthermore, we show that the collisions between individual pairs of atoms lead to a fully coherent collisional phase shift in the corresponding many-particle state, which is a crucial cornerstone of proposed novel quantum computation schemes with neutral atoms. With these experiments we enter a new field of physics with ultracold quantum gases. In this strongly correlated regime, interactions between atoms dominate the behavior of the many-body system such that it can no longer be described by the usual theories for weakly interacting Bose gases. This novel quantum system offers the unique possibility to experimentally address fundamental questions of modern solid state physics, atomic physics, quantum optics, and quantum information.

DOI
10.5282/edoc.968

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In this thesis I report on experiments that enter a new regime in the many body physics of ultracold atomic gases. A Bose-Einstein condensate is loaded into a three-dimensional optical lattice potential formed by a standing wave laser light field. In this novel quantum system we have been able to both realize a quantum phase transition from a superfluid to a Mott insulator, and to observe the collapse and revival of a macroscopic matter wave field. Quantum phase transitions are driven by quantum fluctuations and occur, even at zero temperature, as the relative strength of two competing energy terms in the underlying Hamiltonian is varied across a critical value. In the first part of this work I report on the observation of such a quantum phase transition in a Bose-Einstein condensate with repulsive interactions, held in a three-dimensional optical lattice potential. In the superfluid ground state, each atom is spread-out over the entire lattice, whereas in the Mott insulating state, exact numbers of atoms are localized at individual lattice sites. We observed the reversible transition between those states and detected the gap in the excitation spectrum of the Mott insulator. A Bose-Einstein condensate is usually described by a macroscopic matter wave field. However, a quantized field underlies such a "classical" matter wave field of a Bose-Einstein condensate. The striking behavior of ultracold matter due to the field quantization and the nonlinear interactions between the atoms is the focus of the second part of this work. The matter wave field of a Bose-Einstein condensate is observed to undergo a series of collapses and revivals as time evolves. Furthermore, we show that the collisions between individual pairs of atoms lead to a fully coherent collisional phase shift in the corresponding many-particle state, which is a crucial cornerstone of proposed novel quantum computation schemes with neutral atoms. With these experiments we enter a new field of physics with ultracold quantum gases. In this strongly correlated regime, interactions between atoms dominate the behavior of the many-body system such that it can no longer be described by the usual theories for weakly interacting Bose gases. This novel quantum system offers the unique possibility to experimentally address fundamental questions of modern solid state physics, atomic physics, quantum optics, and quantum information.
By loading Bose-Einstein condensates into a three dimensional optical lattice potential we are able to demonstrate several new intriguing regimes in the physics of ultracold atoms. For example by changing the lattice potential depth we have been able to induce a quantum phase transition from a superfluid to a Mott insulating ground state of the system. Furthermore, by rapidly isolating the different potential wells from each other the collapse and revival of the matter wave field of a Bose-Einstein condensate has been observed. 1
In the present thesis we study several schemes where the detection of the emitted light from an atomic ensemble gives information about the state of the atoms. In chapter 1 we review the basic theory for the light matter interaction in second quantized form. In chapter 2 we show how conservative potentials for the atoms, such as dispersive optical lattices, can be realized experimentally due to the dispersive interaction with a far detuned laser We then review some basic properties of the physics of a particle in a periodic potential. We show that the ground state and the lowest lying excitations of a Bose-Einstein condensate in a dispersive optical lattice can be described by the Bose-Hubbard Hamiltonian. In chapter 3 we study the photonic bandstructure of a chain of fixed pointlike atoms in a biperiodic configuration. We calculate the photonic spectra and the probe transmission if the atoms are in free space and inside a standing wave optical resonator. In chapter 4 we consider light scattering from ultracold atoms in an optical lattice where we calculate the photonic scattering cross section as a function of energy and direction of emission along the Mott-insulator-superfluid phase transition. We take into account the finite tunneling rate for the atoms, when evaluating the scattering cross section of the photons and the effect of photon recoil onto the atoms. In chapter 5 we consider a gas of ultracold atoms trapped at two spatially separated regions in space. Using a two Raman lasers to couple atoms out of the systems we show that it is possible to measure the mean value of the atomic field operator of the two systems by measuring the scattered light intensity of one of the Raman lasers. We show how this setup might be used to measure the temperature of a Bose-Einstein condensate and to monitor the superfluid to Mott-insulator phase transition for a gas of ultracold atoms in an optical lattice.
An optical lattice is a periodic potential for atoms, created using a standing wave pattern of light. Due to the interaction between the light and the atoms, the atoms are attracted to either the nodes or the anti-nodes of the standing wave, depending on the exact wave lenght of the light. This means that if such a lattice is loaded with a sufficiently high number of ultracold atoms, a periodic array of atoms is obtained, we an interatomic distance of a few tenths of a micrometer. In order to obtain such a high number of cold atoms, one first has to create a so-called Bose-Einstein condensate. When an optical lattice is loaded from a Bose-Einstein condensate, it is possible to create a system in which every atom is in the lowest band of the lattice and there is on average one atom in each lattice site. Because the lattice potential is created with laser light, the depth of the lattice can easily be tuned by changing the intensity of the laser. When the intensity of the laser light is low, the atoms can tunnel from one site to the next. Due to this tunneling, the gas of atoms in the lattice will remain superfluid. However, if the intensity of the laser light is increased to above a certain critical value, a quantum phase transition occurs to a so-called Mott insulator. In this state, the atoms can no longer tunnel due to the fact that the on-site interaction between atoms becomes more important then the tunneling probability. In this PhD thesis, a description is given of the experimental setup that is being constructed in our group to create these systems in our lab. Also, a theoretical description is given of these systems and several important quantities our derived, such as the gap of the Mott-insulating state. Furthermore, an experiment is proposed that can be used to accurately measure this gap.
An important new development in the field of ultracold atomic gases is the study of the properties of these gases in a so-called optical lattice. An optical lattice is a periodic trapping potential for the atoms that is formed by the interference pattern of a few laser beams. A reason for the interest in these systems is that the effects of the interatomic interactions can be strongly enhanced. More specifically, it has been shown in a beautiful experiment by Greiner et al. in 2002 that by loading a Bose-Einstein condensate into an optical lattice it is possible for the system to undergo a quantum phase transition to a new quantum phase of matter, the so-called Mott insulator phase. Within this Mott insulator phase each lattice site is occupied by exactly one atom. This makes the Mott insulator phase especially well suited for applications in the field of quantum computation and quantum information processing. We have theoretically investigated the above mentioned quantum phase transition and our formalism allows for a description of the Mott insulator phase at nonzero temperatures. Another important experimental development in the field of ultracold atomic gases is the use of Feshbach resonances to control the interatomic interactions. Such a resonance occurs whenever two colliding atoms form a long-lived molecule for some time. The crucial point of a Feshbach resonance is that the above mentioned molecule has a magnetic moment that is not equal to twice the magnetic moment of the atom. As a consequence the energy difference between the two atoms and the molecule and hence the interactions between the atoms can be controlled by using an external magnetic field. By combining these two techniques, i.e, by trapping ultracold atomic gases in an optical lattice and by tuning a magnetic field near a Feshbach resonance there can be a new quantum phase transition between two superfluid phases. We gave derived the the theory for the description of these Feshbach resonances in optical lattices and applied it to various systems. To be a bit more precise, if we tune the external magnetic field such that the energy difference between a molecule and two atoms is sufficiently negative, then the gas consists of a Bose-Einstein condensate of molecules. In contrast, if the energy difference is large enough and positive we have a gas that consists primarily of a Bose-Einstein condensate of atoms. It turns out that these two limits are separated by an Ising-like quantum phase transition. By using atomic Bose gases near a Feshbach resonance detailed experimental studies which test the theoretical predictions of the statistical and dynamical properties of these quantum phase transitions can be made.
In this thesis I report on experiments on the quantum dynamics of matter waves in a onedimensional lattice potential. A 87Rb Bose-Einstein condensates is prepared in a one-dimensional waveguide in the lowest band of a superimposed optical lattice potential. The action of a weak lattice potential allows to modify the linear wave dispersion. We realized dispersion management by switching from normal to anomalous dispersion during the evolution. In this way the initial expansion of a wave packet is reversed to a compression and thus the effective spreading can be suppressed. By preparing a BEC at the Brillouin zone edge, we observed bright atomic gap solitons – non-spreading wave packets. They form, if the atom number and the lattice potential depth is tuned such that the effect of the repulsive atomic interaction and the anomalous dispersion cancel. For deep lattice potentials our system is described by a discrete nonlinear Schrödinger equation, whose dynamics is determined by the tunneling between adjacent lattice sites and the nonlinear phase evolution. In the main part of this thesis I report on the first experimental observation of nonlinear self-trapping for matter waves. The transition from the diffusive regime, characterized by an continuous expansion of the condensate, to the self-trapping regime is accomplished by increasing the atomic density. Due to the corresponding increase of the repulsive atomic interaction the initial expansion stops and the width of the wave packet remains finite. The comparison with a numerical analysis reveals that the effect is due to an inhibition of the site-to-site tunneling induced by the nonlinear phase evolution.
This thesis covers most of my work in the field of ultracold atoms loaded in optical lattices. It makes a route through the physics of cold atoms in periodic potentials starting from the simple noninteracting system and going into the many-body physics that describes the strongly correlated Mott insulator regime. Even though this thesis is a theoretical work all the chapters are linked either with experiments already done or with ongoing experimental efforts. This thesis can be divided into four different parts. The first part comprises chapters 1 to 3. In these chapters, after a brief introduction to the field of optical lattices I review the fundamental aspects pertaining to the physics of systems in periodic potentials. The second part deals with the superfluid weakly interacting regime where standard mean field techniques can be applied. This is covered in chapters 4 and 5. Specifically, chapter 4 introduces the discrete nonlinear Schroedinger equation (DNLSE) and uses it to model some experiments. In chapter 5 I go one step further and include the small quantum fluctuations neglected in the DNLSE by studying quadratic approximations of the Bose-Hubbard Hamiltonian. Chapters 6 to 8 can be grouped as the third part of the thesis. In them I adopt an effective action formalism, the so called two particle irreducible effective action (2PI) together with the closed time path (CTP) formalism to study far-from-equilibrium dynamics. The many-body techniques discussed in these chapters systematically include higher order quantum corrections, not included in the quadratic approximations of the Hamiltonian, which we show are crucial for a correct description of the quantum dynamics outside the very weakly interacting regime. Finally, chapter 9 to 11 are devoted to study the Mott insulator phase. In these chapters using perturbation theory I study the Mott insulator ground state and its excitation spectrum, the response of the system to Bragg spectroscopy, and propose a mechanism to correct for the residual quantum coherences inherent to the Mott insulator ground state. Even though small these are not ideal for the use of neutral atoms in optical lattice as a tool for quantum computation.