As a subset of quantum optics, single photons are one of the competing physical resources for quantum information processing. When used as carriers of quantum information, they have no equal. For the processing of quantum information, single photons have proven difficult to scale beyond the order of ~10 photons. The lack of single-photon-level interaction has led to creative approaches which rely on post-selection to filter the possible measured outcomes to those which appear as though interaction occurred. This approach of post-selection leans heavily on the ability to not only generate but also detect scores of single photons simultaneously and with near perfect efficiency. Our work relaxes the emphasis which has been placed on single photons for quantum information processing to that of states with, in principle, an arbitrary number of photons. Central moment expectations on two-mode squeezed states are shown to exhibit post-selection behavior which reflects the single-photon counterpart. These measures are proven to be robust to loss and return entangled state statistics on average. With naive estimation of the central moment, states with ~20 modes are within reach with current technology, closing the gap between quantum states which can and cannot be classically simulated.
As a subset of quantum optics, single photons are one of the competing physical resources for quantum information processing. When used as carriers of quantum information, they have no equal. For the processing of quantum information, single photons have proven difficult to scale beyond the order of ~10 photons. The lack of single-photon-level interaction has led to creative approaches which rely on post-selection to filter the possible measured outcomes to those which appear as though interaction occurred. This approach of post-selection leans heavily on the ability to not only generate but also detect scores of single photons simultaneously and with near perfect efficiency. Our work relaxes the emphasis which has been placed on single photons for quantum information processing to that of states with, in principle, an arbitrary number of photons. Central moment expectations on two-mode squeezed states are shown to exhibit post-selection behavior which reflects the single-photon counterpart. These measures are proven to be robust to loss and return entangled state statistics on average. With naive estimation of the central moment, states with ~20 modes are within reach with current technology, closing the gap between quantum states which can and cannot be classically simulated.
Single photons are the smallest excitation states of the elctromagnetic field. They can be experimentally created but there is no apparatus that performs this task with 100% efficiency. Many techniques and theorems of optical quantum information theory use single photons. In order to utilize them for information processing, it is reasonable to know if they had been successfully produced. In other words: One needs heralded single photons. How to achieve this, is the main result of this diploma thesis. The task has been to improve the efficiency of already existing single photon sources. An apparatus had to be found which postprocesses the output of such sources in order to either herald the photons or at least to improve the efficiency. This apparatus is explicitly allowed to use other optical sources, for example coherent states (laser). The situation has been formally represented by the assumption that single photon sources produce a mixture of vacuum and the single photon state. It is known that experimental set-ups also create higher photon contributions. These contributions are considered to be small in corresponding publications. For some cases they even seem to vanish at all. One can distinguish two regimes concerning the techniques which have been used in this work: linear and nonlinear optics. Linear optical tools, for example the beam splitter, do not absorb photons in the ideal case, but it is not easy to implement useful transformations by their means. Absorption and weak coupling are drawbacks which arise mainly in nonlinear optical media. This work shows that the interactions two-photon absorption and cross phase modulation can be used in schemes, which enable the heralding of single photons. Already there are some linear optical quantum gates which manipulate optical states by means of single photons. Photons do not interact with each other directly, in contrast to electrons for example. Therefore quantum gates which act on more than one mode are interesting. The effective interaction of these gates is not quitecomparable to unitary dynamics. Moreover, these gates do not function in each case. Measurements required in auxiliary modes yield different results for each single case and in order to obtain the desired effect the cases have to be selected according to the measurement results. It has been investigated, how such gates perform if they have statistical mixtures as a resource instead of perfect single-photon states. Yet, no improvement of the single-photon contribution has been accomplished by means of these apparatuses. Hereby it has not been disproved that it is possible to achieve this goal using other apparatuses and techniques of linear optics. Yet, it has been shown that an enhancement is possible but then a non-vanishing two-photon contribution is appended. One of the most basic quantum gates is the conditional sign flip. The optical 8 interaction cross phase modulation acts in quite the same way considering only single photons. This effect enables the heralding of single photons in the ideal case. Within this work it has been shown that a Mach-Zehnder interferometer, a cross phase modulating medium and a photo-detector can be employed for this purpose. One could use any source of light as input to the interferometer but a strong coherent state (laser) may be preferred for the purpose of enhancing the interaction. The absorption of two-photon states is another non-linear effect. Astonishingly this effect serves to generate a heralded single-photon state given two imperfect single-photon sources. First the photon adding tool is employed which consists of a beam splitter and a photo-detector. By means of that and the statistical mixtures of two single-photon sources one creates a mixture which contains vacuum, the single-photon state and additionally the two-photon Fock state. This mixture propagates through a Mach-Zehnder interferometer. The interferometer is adjusted such that it is transparent for incoming light. In addition to the interferometer alone a two-photon absorbing medium is placed in one of its arms. For this reason there is a chance that the two-photon contribution entering the interferometer is absorbed within this medium. We cannot exclude this unfortunate case. A detector is placed in one of the two output modes. The interferometer is adjusted such that the single photon state does not leave in the mode in which the detector is placed, but always in the other mode. The detector can only click if the two-photon state propagates through the interferometer and if it is not destroyed in the absorbing medium. If the detector then receives one photon it is obvious that another one must leave in the other mode. The whole phenomenon is very similar to the concept of null measurement. Although not a main result, it has been shown here that the so-called Hong-Ou-Mandel effect can be generalized. It has been proven that the beam splitter transforms Fock states with equal Fock number into superpositions of Fock numbers which are even in each mode. Another effect on special odd Fock states is conjectured.
This thesis intends to familiarize the reader with the concepts of photon statistics and correlations in quantum optics. Developing light sources that emit quantum states is central for the realization of quantum technologies. One important step in characterizing these sources is the measurement of field fluctuations and correlations, by coincidence measurements. The expectation value of a coincidence measurement, a simultaneous measurement of two intensities (or, more general, four fields), is represented by the fourth-order correlation function. The value of the correlation function, at zero delay between the detection of two photons, reveals important properties of the state to which they belonged, for example the fluctuations of the photon number. Since predictability is important for many applications, light sources emitting single photons are also characterized by the indistinguishability of consecutively emitted photons, or of two photons from separate emitters. In paper I we investigate blinking behaviour in quantum emitters, and its effect on the interference pattern and photon statistics with photons from two separate emitters. Blinking refers to an emitters transition into a non-emitting state, and subsequent transition back to an emitting state. We show that blinking can not be treated as linear loss, when measuring the fourth-order correlation function for two emitters in a Hong-Ou-Mandel setup. In general, a measurement of the fourth-order correlation function is robust to loss, which makes it a very practical tool. However, the relation between recorded coincidence counts and the correlation function is only direct in the limit of zero detection efficiency, and depends on the detection system. In paper II, we show that by adding a variable attenuation in the beam path, we can trace back to the ''true'' value of the correlation function at zero quantum efficiency. This method improves accuracy in correlation measurements by decreasing a systematic error at the expense of an increased statistical error, which is easier to handle, extending the use of coincidence methods to classical and non-classical multi-photon states.
Two-photon interference effects and correlated-photon statistics have traditionally been observed in the coincidence detection rate between two detectors. Here, we report observations of correlated-photon statistics, which are due to two-photon entanglement and interference, in the single-photon detection rate. The observed effects are explained by considering all possible photon number states that reach the detector, rather than considering just the state post-selected by the coincidence circuit.
Photons are natural carriers of quantum information due to their ease of distribution and long lifetime. This thesis concerns various related aspects of quantum information processing with single photons. Firstly, we demonstrate N-photon entanglement generation through a generalised N X N symmetric beam splitter known as the Bell multiport. A wide variety of 4-photon entangled states as well as the N-photon W-state can be generated with an unexpected non-monotonic decreasing probability of success with N. We also show how the same setup can be used to generate multiatom entanglement. A further study of multiports also leads us to a multiparticle generalisation of the Hong-Ou-Mandel dip which holds for all Bell multiports of even number of input ports. Next, we demonstrate a generalised linear optics based photon filter that has a constant success probability regardless of the number of photons involved. This filter has the highest reported success probability and is interferometrically robust. Finally, we demonstrate how repeat-until-success quantum computing can be performed with two distant nodes with unit success probability using only linear optics resource. We further show that using non-identical photon sources, robustness can still be achieved, an illustration of the nature and advantages of measurement-based quantum computation. A direct application to the same setup leads naturally to arbitrary multiphoton state generation on demand. Finally, we demonstrate how polarisation entanglement of photons can be detected from the emission of two atoms in a Young's double-slit type experiment without linear optics, resulting in both atoms being also maximally entangled.
We report an experimental observation of correlated-photon statistics using a single detector. The usual coincidence dip in a two-photon polarization interferometer is accompanied by a dip in single-photon detection rates. Surprisingly, a dip in the singles rate is also observed when the interferometer is aligned for a coincidence peak, or anti-dip. This effect is explained by taking into account all possible photon number states that reach the detector, rather than considering just the state post-selected by the coincidence measurement.
Quantum metrology enables estimation of optical phase shifts with precision beyond the shot-noise limit. One way to exceed this limit is to use squeezed states, where the quantum noise of one observable is reduced at the expense of increased quantum noise for its complementary partner. Because shot-noise limits the phase sensitivity of all classical states, reduced noise in the average value for the observable being measured allows for improved phase sensitivity. However, additional phase sensitivity can be achieved using phase estimation strategies that account for the full distribution of measurement outcomes. Here we experimentally investigate a model of optical spin-squeezing, which uses post-selection and photon subtraction from the state generated using a parametric downconversion photon source, and we investigate the phase sensitivity of this model. The Fisher information for all photon-number outcomes shows it is possible to obtain a quantum advantage of 1.58 compared to the shot-noise value for five-photon events, even though due to experimental imperfection, the average noise for the relevant spin-observable does not achieve sub-shot-noise precision. Our demonstration implies improved performance of spin squeezing for applications to quantum metrology.