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Hyperfine quenching of 3s3p 3P0, 3P2 level of Mg-like ions

Huihui Kang, Jiguang Li, Chenzhong Dong, Per Jönsson, Gediminas Gaigalas A

Published Jan 1, 2009• 0 citations
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We experimentally determine the absolute frequencies and hyperfine splittings of the 6s6p 3P0,2 − 6s7s 3S1 transitions of ultracold 171Yb atoms in an optical lattice. A frequency comb referenced to an ultrastable optical cavity is used to measure the electric-dipole transition frequencies. With the normalized shelving detection technique, about 12 MHz and 10 MHz linewidth of atomic spectra are obtained, respectively, which is some greater than the natural linewidth of 1.5 MHz and 5.9 MHz and is limited by the broadening from the probe and lattice light. By reference to our 171Yb 6 s2 1S0 − 6s6p 3P0 clock, the absolute frequencies are found to be 461861338.03 (0.21) MHz and 461871596.07 (0.31) MHz for the 6s6p 3P0 − 6s7s 3S1 (F = 1/2 and F = 3/2) transitions, which are more accurate than the previous measurement by one order of magnitude. For the 6s6p 3P2 (F = 3/2 and F = 5/2) − 6s7s 3S1 (F = 1/2 and F = 3/2) transitions, the measured frequencies are 389257019.71 (0.65) MHz, 389267277.10 (0.37) MHz and 389260569.95 (0.89) MHz, respectively, which are the first measurements to our knowledge. Furthermore, the hyperfine constants for the 6s6p 3P2 and 6s7s 3S1 states are determined to be 2682.86(0.38) MHz and 6838.69(0.25) MHz, both of which agree well with other recent experimental results.

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An anomalous resonant dip of two-photon ionisation with 3s3p 1 P as an intermediate state and a stimulated emission by the 3s4s 3 S-3s3p 3 P transition, at 518.37 nm following the pulsed laser excitation near the 3s 2 1 S-3s3p 1 P resonance at 285.21 nm in magnesium vapour are observed and studied. The mechanism of the ionisation dip is attributed to formation and predissociation of the A 1 Sigma + u Mg 2 dimer, which transfer the population from the laser-pumped 3s3p 1 P level to 3s3p 3 P levels. Re-excitation of the produced 3s3p 3 P atoms and the subsequent radiative processes are presumed to explain the generation of stimulated emission. A theoretical model is employed to interpret the experimental phenomena.

Journal of Physics B Atomic Molecular and Optical Physics•Feb 28, 1988•3 citations
Hyperfine quenching rates of nsnp 3P0−ns2 1S0nsnp\,^3P_0-ns^2\,^1S_0nsnp3P0​−ns21S0​ transition in 25^{25}25Mg, 87^{87}87Sr and 113^{113}113Cd
We experimentally determine the absolute frequencies and hyperfine splittings of the 6s6p 3P0,2 − 6s7s 3S1 transitions of ultracold 171Yb atoms in an optical lattice. A frequency comb referenced to an ultrastable optical cavity is used to measure the electric-dipole transition frequencies. With the normalized shelving detection technique, about 12 MHz and 10 MHz linewidth of atomic spectra are obtained, respectively, which is some greater than the natural linewidth of 1.5 MHz and 5.9 MHz and is limited by the broadening from the probe and lattice light. By reference to our 171Yb 6 s2 1S0 − 6s6p 3P0 clock, the absolute frequencies are found to be 461861338.03 (0.21) MHz and 461871596.07 (0.31) MHz for the 6s6p 3P0 − 6s7s 3S1 (F = 1/2 and F = 3/2) transitions, which are more accurate than the previous measurement by one order of magnitude. For the 6s6p 3P2 (F = 3/2 and F = 5/2) − 6s7s 3S1 (F = 1/2 and F = 3/2) transitions, the measured frequencies are 389257019.71 (0.65) MHz, 389267277.10 (0.37) MHz and 389260569.95 (0.89) MHz, respectively, which are the first measurements to our knowledge. Furthermore, the hyperfine constants for the 6s6p 3P2 and 6s7s 3S1 states are determined to be 2682.86(0.38) MHz and 6838.69(0.25) MHz, both of which agree well with other recent experimental results.
An anomalous resonant dip of two-photon ionisation with 3s3p 1 P as an intermediate state and a stimulated emission by the 3s4s 3 S-3s3p 3 P transition, at 518.37 nm following the pulsed laser excitation near the 3s 2 1 S-3s3p 1 P resonance at 285.21 nm in magnesium vapour are observed and studied. The mechanism of the ionisation dip is attributed to formation and predissociation of the A 1 Sigma + u Mg 2 dimer, which transfer the population from the laser-pumped 3s3p 1 P level to 3s3p 3 P levels. Re-excitation of the produced 3s3p 3 P atoms and the subsequent radiative processes are presumed to explain the generation of stimulated emission. A theoretical model is employed to interpret the experimental phenomena.