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Optics and Spectroscopy

Conversion of optical pumping into the IR region under conditions of two-photon resonance

V. M. Arutyunyan, A. Zh. Muradyan, L Kh Muradyan, M. K. Oganesyan, T. A. Papazyan, Ruben Khachatryan

Published Sep 1, 1984• 0 citations
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Soviet Journal of Quantum Electronics•Oct 31, 1981•4 citations
Six-photon parametric up-conversion under conditions of two-, three-, and four-photon resonance of a constant nonmonochromatic pump field is analyzed allowing for population migration, transient response of the medium, Stark shift of the levels, and width of the frequency spectrum of the the pump field. It is found that in the steady-state conversion regime, the maximum average conversion efficiency in the four-photon resonance case differs only negligibly from the maximum conversion efficiency in a monochromatic field, whereas in the two-photon and three-photon resonance cases it is higher than the maximum efficiency in a monochromatic pump field. An analysis is made of the influence of optically induced relaxation on the average conversion efficiency under conditions of pulsed excitation of two-, three-, and four-photon resonances.
Four-photon parametric up-conversion of a weak infrared signal under conditions of two-photon resonance of a constant nonmonochromatic pump field is analyzed allowing for population migration, transient response of the medium, Stark shift of the levels, and width of the pump frequency spectrum. It is found that under steady-state conversion conditions in a nonmonochromatic pump field, it is possible to achieve an average conversion efficiency differing only negligibly from the maximum conversion efficiency in a monochromatic pump field. An analysis is made of the influence of optically induced relaxation on the average conversion efficiency in the transient regime. Numerical estimates are made of the transition parameters for an alkali metal vapor in a frequency-degenerate pump field exciting a two-photon transition.