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Chinese Physics B

Study of optical clocks based on ultracold 171Yb atoms*

Di Ai, Hao Qiao, Shuang Zhang, Limeng Luo, Changyue Sun, Sheng Zhang, Chengquan Peng, Qi-Chao Qi, Taoyun Jin, Min Zhou, Xinye Xu

Published Jun 29, 2020• 16 citations
Publisher

Abstract

The optical atomic clocks have the potential to transform global timekeeping, relying on the state-of-the-art accuracy and stability, and greatly improve the measurement precision for a wide range of scientific and technological applications. Herein we report on the development of the optical clock based on 171Yb atoms confined in an optical lattice. A minimum width of 1.92-Hz Rabi spectra has been obtained with a new 578-nm clock interrogation laser. The in-loop fractional instability of the 171Yb clock reaches 9.1 × 10−18 after an averaging over a time of 2.0 × 104 s. By synchronous comparison between two clocks, we demonstrate that our 171Yb optical lattice clock achieves a fractional instability of 4.60 × 10 − 16 / τ .

DOI
10.1088/1674-1056/aba099

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Abstract Optical clocks are the most precise measurement devices. Here we experimentally characterize one such clock based on the 1S0-3P0 transition of neutral 171Yb atoms confined in an optical lattice. Given that the systematic evaluation using an interleaved stabilization scheme is unable to avoid noise from the clock laser, synchronous comparisons against a second 171Yb lattice system were implemented to accelerate the evaluation. The fractional instability of one clock falls below 4 × 10−17 after an averaging over a time of 5,000 seconds. The systematic frequency shifts were corrected with a total uncertainty of 1.7 × 10−16. The lattice polarizability shift currently contributes the largest source. This work paves the way to measuring the absolute clock transition frequency relative to the primary Cs standard or against the International System of Units (SI) second.

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Atoms confined in the optical lattice can be interrogated with Doppler- and recoil-free operation. However, if not properly controlled, the optical lattice may limit clock accuracy. To improve the lattice-light-shift uncertainty, the cooling and trapping lasers' frequency stability is optimized, and the atom's signal stability is enhanced. A ring-cavity Ti:sapphire laser is locked to the optical frequency comb, which is referenced to a 578 nm ultra-stable laser, and the beat note's stability is on the order of 10−16. Using a 10 cm Fabry–Pérot cavity referenced to the Ti:sapphire laser, the optical frequency stability is transferred to the 399 nm cooling laser, creating favorable conditions for evaluating the lattice-light-shift accurately. We reevaluate lattice-light-shift in our 171Yb optical lattice clock with an uncertainty of 8.1 × 10−18, which is an order lower than our previous result, and the magic frequency is determined to be 394 798 266.6(1.3) MHz.

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Realization of advanced 171Yb optical lattice frequency standard

Gianmaria Milani

Atomic clocks constitute a fundamental tool for time and frequency metrology and their application is widespread in many technological fields. In particular, the International System of units (SI) defines the second on a microwave transition of Caesium atoms. The realization is made by clocks reaching uncertainties of few parts in 10^−16, making the second to be the quantity realized with the smallest uncertainty in the SI. However, a new generation of atomic clocks, called optical clocks, have already demonstrated to surpass Caesium standards both in accuracy and stability. The research performed during my PhD activity has been focused on the development and characterization of Ytterbium (Yb) optical lattice clocks. These systems operate with a large number of ultra-cold neutral atoms having a clock transition in the visible region of the electromagnetic spectrum. The atomic sample is trapped in an periodical optical potential called optical lattice that gives the advantage to interrogate many quantum absorbers for an extended time, with small perturbations, allowing to achieve an unprecedented stability and accuracy. The main experimental work has been carried out in the laboratories of the Istituto Nazionale di Ricerca Metrologica (INRIM) in Turin, where several atomic clocks are present including the Italian primary frequency standard, the Caesium fountain ITCsF2, and where an Yb optical lattice clock is currently being developed. This thesis describes the functioning of the system along with the full characterization of systematic effects, the complete uncertainty budget and its first absolute frequency measurement against the primary frequency standard. The clock exhibited an accuracy of 1.6 × 10^−16 and the comparison with the Cs fountain resulted in a frequency of f171Yb = 518 295 836 590 863.59(31) Hz, limited by the fountain uncertainty. This measurement is in agreement with the ytterbium frequency recommended as a secondary representation of the second in the SI and constitutes the first measurement of a Yb clock in Europe and the second one in the world against a primary frequency standard. Several upgrades have been applied after the absolute measurement. In particular, the design and realization a system capable to frequency stabilize several lasers on a single optical cavity is illustrated. This cavity has been implemented to lock the lasers used to cool and trap the atomic sample at 399, 556 and 759nm using the offset sideband locking technique, a modified version of the Pound–Drever–Hall method that gives an extended frequency tunability. The system proved to be an easy-to-use and reliable tool for the experimental activity showing a linewidth below 300 Hz at 556nm, which is the wavelength that requires the most stringent performance, and a long term drift below 20 kHz per day at 759nm. That is suitable for operating the lattice laser with a light shift uncertainty below 1 × 10−18. During my PhD I have been guest researcher at the National Institute of Standards and Technology (NIST) of Boulder, Colorado, for nine months in 2016. In these laboratories two Yb optical lattice clocks are operative. I worked on the instability measurement of a composite system exploiting the two clocks to suppress the Dick effect, called zero-dead-time (ZDT) clock, which demonstrated a fractional instability of 3 × 10−17 at 1s. The two clocks can also be operated to extend the interrogation time obtaining a spectroscopic feature after 4 s of 120(20)mHz corresponding to a quality factor Q > 4 × 10^15. I also worked on the characterization of several systematic shifts that allowed to complete the uncertainty budget of the clocks at 1.6 × 10^−18. In particular, I contributed to the characterization of lattice light shifts considering the effect of atomic sample temperature and the identification of a metrological regime called operational magic frequency where frequency shifts are insensitive to changes in trap depth.

•May 2, 2018•1 citation
The optical atomic clocks have the potential to transform global timekeeping, relying on the state-of-the-art accuracy and stability, and greatly improve the measurement precision for a wide range of scientific and technological applications. Herein we report on the development of the optical clock based on 171Yb atoms confined in an optical lattice. A minimum width of 1.92-Hz Rabi spectra has been obtained with a new 578-nm clock interrogation laser. The in-loop fractional instability of the 171Yb clock reaches 9.1 × 10−18 after an averaging over a time of 2.0 × 104 s. By synchronous comparison between two clocks, we demonstrate that our 171Yb optical lattice clock achieves a fractional instability of 4.60 × 10 − 16 / τ .
Abstract Optical clocks are the most precise measurement devices. Here we experimentally characterize one such clock based on the 1S0-3P0 transition of neutral 171Yb atoms confined in an optical lattice. Given that the systematic evaluation using an interleaved stabilization scheme is unable to avoid noise from the clock laser, synchronous comparisons against a second 171Yb lattice system were implemented to accelerate the evaluation. The fractional instability of one clock falls below 4 × 10−17 after an averaging over a time of 5,000 seconds. The systematic frequency shifts were corrected with a total uncertainty of 1.7 × 10−16. The lattice polarizability shift currently contributes the largest source. This work paves the way to measuring the absolute clock transition frequency relative to the primary Cs standard or against the International System of Units (SI) second.
We report the realization of closed-loop operation of an optical lattice clock based on 171 Yb atoms. We interrogate the 1 S 0 → 3 P 0 clock transition using single Rabi pulses of 578 nm laser light. The two π-transitions from m F = ± 1 / 2 ground states are alternatively interrogated, and the clock laser frequency is locked to the center of the two resonances. The in-loop error signal stability of the clock reaches 3 × 10 − 17 for an average time of 3500 s. We also perform interleaved operations of the clock with two independent servo loops, and the fractional frequency difference averages down to 2 × 10 − 16 in 7200 s.
Atomic clocks have been instrumental in science and technology, leading to innovations such as global positioning, advanced communications, and tests of fundamental constant variation. Timekeeping precision at 1 part in 10(18) enables new timing applications in relativistic geodesy, enhanced Earth- and space-based navigation and telescopy, and new tests of physics beyond the standard model. Here, we describe the development and operation of two optical lattice clocks, both using spin-polarized, ultracold atomic ytterbium. A measurement comparing these systems demonstrates an unprecedented atomic clock instability of 1.6 × 10(-18) after only 7 hours of averaging.
Rapid progress in the precision and accuracy of optical atomic clocks over the last decade has advanced the frontiers of timekeeping, metrology, and quantum science. However, the stabilities of most optical clocks remain limited by the local oscillator rather than the atoms themselves, leaving room for further progress. Here we implement a "multiplexed" one-dimensional optical lattice clock, in which spatially-resolved, movable ensembles of ultra-cold strontium atoms are trapped in the same optical lattice, interrogated simultaneously by a shared clock laser, and read-out in parallel. By performing synchronized Ramsey interrogations of ensemble pairs we observe atom-atom coherence times up to 26 seconds, a 270-fold improvement over the atom-laser coherence time, demonstrate a relative stability of 9.7(4)×10−18/τ9.7(4)\times10^{-18}/\sqrtτ9.7(4)×10−18/τ​ (where τττ is the averaging time in seconds), and reach a fractional uncertainty of 8.9(3)×10−208.9(3)\times 10^{-20}8.9(3)×10−20 after 3.3 hours of averaging. These results demonstrate that applications requiring ultra-high-precision comparisons between optical atomic clocks need not be limited by the stability of the local oscillator. With multiple ensemble pairs, we realize a miniaturized clock network consisting of 6 atom ensembles, resulting in 15 unique pairwise clock comparisons with relative stabilities below 3×10−17/τ3\times10^{-17}/\sqrtτ3×10−17/τ​. Finally, we demonstrate the capability to simultaneously load spatially-resolved, heterogeneous ensemble pairs of all four stable isotopes of strontium in a lattice. The unique capabilities offered by this platform pave the way for future studies of precision isotope shift measurements, spatially resolved characterization of limiting clock systematics, development of clock-based gravitational wave and dark matter detectors, and novel tests of relativity including measurements of the gravitational redshift at sub-centimeter scales.
Atoms confined in the optical lattice can be interrogated with Doppler- and recoil-free operation. However, if not properly controlled, the optical lattice may limit clock accuracy. To improve the lattice-light-shift uncertainty, the cooling and trapping lasers' frequency stability is optimized, and the atom's signal stability is enhanced. A ring-cavity Ti:sapphire laser is locked to the optical frequency comb, which is referenced to a 578 nm ultra-stable laser, and the beat note's stability is on the order of 10−16. Using a 10 cm Fabry–Pérot cavity referenced to the Ti:sapphire laser, the optical frequency stability is transferred to the 399 nm cooling laser, creating favorable conditions for evaluating the lattice-light-shift accurately. We reevaluate lattice-light-shift in our 171Yb optical lattice clock with an uncertainty of 8.1 × 10−18, which is an order lower than our previous result, and the magic frequency is determined to be 394 798 266.6(1.3) MHz.
Atomic clocks constitute a fundamental tool for time and frequency metrology and their application is widespread in many technological fields. In particular, the International System of units (SI) defines the second on a microwave transition of Caesium atoms. The realization is made by clocks reaching uncertainties of few parts in 10^−16, making the second to be the quantity realized with the smallest uncertainty in the SI. However, a new generation of atomic clocks, called optical clocks, have already demonstrated to surpass Caesium standards both in accuracy and stability. The research performed during my PhD activity has been focused on the development and characterization of Ytterbium (Yb) optical lattice clocks. These systems operate with a large number of ultra-cold neutral atoms having a clock transition in the visible region of the electromagnetic spectrum. The atomic sample is trapped in an periodical optical potential called optical lattice that gives the advantage to interrogate many quantum absorbers for an extended time, with small perturbations, allowing to achieve an unprecedented stability and accuracy. The main experimental work has been carried out in the laboratories of the Istituto Nazionale di Ricerca Metrologica (INRIM) in Turin, where several atomic clocks are present including the Italian primary frequency standard, the Caesium fountain ITCsF2, and where an Yb optical lattice clock is currently being developed. This thesis describes the functioning of the system along with the full characterization of systematic effects, the complete uncertainty budget and its first absolute frequency measurement against the primary frequency standard. The clock exhibited an accuracy of 1.6 × 10^−16 and the comparison with the Cs fountain resulted in a frequency of f171Yb = 518 295 836 590 863.59(31) Hz, limited by the fountain uncertainty. This measurement is in agreement with the ytterbium frequency recommended as a secondary representation of the second in the SI and constitutes the first measurement of a Yb clock in Europe and the second one in the world against a primary frequency standard. Several upgrades have been applied after the absolute measurement. In particular, the design and realization a system capable to frequency stabilize several lasers on a single optical cavity is illustrated. This cavity has been implemented to lock the lasers used to cool and trap the atomic sample at 399, 556 and 759nm using the offset sideband locking technique, a modified version of the Pound–Drever–Hall method that gives an extended frequency tunability. The system proved to be an easy-to-use and reliable tool for the experimental activity showing a linewidth below 300 Hz at 556nm, which is the wavelength that requires the most stringent performance, and a long term drift below 20 kHz per day at 759nm. That is suitable for operating the lattice laser with a light shift uncertainty below 1 × 10−18. During my PhD I have been guest researcher at the National Institute of Standards and Technology (NIST) of Boulder, Colorado, for nine months in 2016. In these laboratories two Yb optical lattice clocks are operative. I worked on the instability measurement of a composite system exploiting the two clocks to suppress the Dick effect, called zero-dead-time (ZDT) clock, which demonstrated a fractional instability of 3 × 10−17 at 1s. The two clocks can also be operated to extend the interrogation time obtaining a spectroscopic feature after 4 s of 120(20)mHz corresponding to a quality factor Q > 4 × 10^15. I also worked on the characterization of several systematic shifts that allowed to complete the uncertainty budget of the clocks at 1.6 × 10^−18. In particular, I contributed to the characterization of lattice light shifts considering the effect of atomic sample temperature and the identification of a metrological regime called operational magic frequency where frequency shifts are insensitive to changes in trap depth.