Decoherence and parameter fluctuations are two of the mayor obstacles for solid-state quantum computing. In this work, decoherence in superconducting qubits of the transmon type is investigated. For this purpose, a time-multiplexed measurement protocol was developed and applied in long-term measurements. The resulting simultaneous measurement of the qubit's relaxation and dephasing rate, as well as its resonance frequency enables analysis of correlations between these parameters. A spectral noise analysis complements these measurements. Together, the results agree well with the interacting defect model of two-level-systems and yield information about the microscopic origin of the intrinsic decoherence mechanisms in Josephson qubits. Our measurements show inherent correlations between dephasing and fluctuations in qubit frequency on the timescale of seconds to days, which is attributed to the influence of individual defects, located close to conductor edges. Cross-correlation and spectral noise analysis confirm this interpretation and ascribe the source of fluctuation to interactions between thermal fluctuators and surface defects. Single defects reducing the coherence of qubits by up to one order of magnitude are a major challenge for future quantum computers. Non-tunable qubits are intrinsically insensitive to some decoherence channels and thus ideal for this fundamental analysis. However, to widen the focus and contrast the results of different material systems, we pursue the fabrication of voltage controlled gatemon qubits. In the course of this work, the theoretical foundation and technical implementation of transmon qubits based on regular Josephson weak links, and semiconducting nanowires is given. The experimental design and measurement setup are explained in detail. Our findings make continuous re-calibration a necessity in today's solid-state qubits, although new materials or processing techniques might mitigate the problem. However, the results of this work imply that fundamental improvements of qubit parameter stability are necessary in order to realize scalable and coherent qubit circuits.
Superconducting quantum circuits are promising platforms for scalable quantum computing, where qubit coherence is critically determined by microscopic defects in the oxide tunneling barrier of Josephson junctions. Amorphous Al
2O
3 is widely used as a barrier material, but under irradiation, oxygen vacancy (V
O) defects are readily generated, introducing noise sources that accelerate qubit decoherence. We systematically investigate the structural characteristics and electronic impact of V
O defects in amorphous Al
2O
3 using first-principles calculations and \textit{ab initio} molecular dynamics. Our results show that both the coordination environment and concentration of V
Os strongly influence electrical conductivity. In particular, two- and three-coordinated V
Os, unique to the amorphous structure, enhance conductivity more than conventional four-coordinated vacancies. Increasing V
O concentration amplifies conductivity fluctuations, which we link to critical current noise in Josephson junctions. Using a noise model, we estimate that higher V
O densities lead to shorter qubit coherence times. These findings provide insights for radiation-hard design of superconducting quantum devices.
Superconducting integrated circuits incorporating Josephson junctions are an attractive candidate for scalable quantum information processing in the solid state. The strong nonlinearity of the Josephson effect enables one to tailor an anharmonic potential and thus to realize an artificial quantum two-level system (“qubit”) from a macroscopic superconducting circuit. Josephson qubits can be made to interact strongly and controllably, and it should be straightforward to fabricate circuits incorporating hundreds or even thousands of Josephson qubits using standard thin-film processing techniques. Work over the last several years has shown that qubit performance is limited by spurious coupling of the qubit to microscopic defect states in the materials that are used to implement the circuit. Here we discuss the materials origins of dissipation and dephasing in superconducting qubits. A deeper understanding of the underlying materials physics that governs decoherence in superconducting quantum circuits will guide the search for improved, low-noise materials and fuel continued progress in the field of superconducting quantum computing.