We describe a matter-wave amplifier for vibrational ground-state molecules which uses a Feshbach resonance to first form quasibound molecules starting from an atomic Bose-Einstein condensate. The quasibound molecules are then driven into their stable vibrational ground state via a two-photon Raman transition inside an optical cavity. The transition from the quasibound state to the electronically excited state is driven by a classical field. Amplification of ground state molecules is then achieved by using a strongly damped cavity mode for the transition from the electronically excited molecules to the molecular ground state.We describe a matter-wave amplifier for vibrational ground-state molecules which uses a Feshbach resonance to first form quasibound molecules starting from an atomic Bose-Einstein condensate. The quasibound molecules are then driven into their stable vibrational ground state via a two-photon Raman transition inside an optical cavity. The transition from the quasibound state to the electronically excited state is driven by a classical field. Amplification of ground state molecules is then achieved by using a strongly damped cavity mode for the transition from the electronically excited molecules to the molecular ground state.

arXiv:cond-mat/0404006Physical Review LettersSep 29, 200423 citations

Nonlinear optical processes in a system of colliding atoms

A. M. Bonch-Bruevich, Sergey G. Przhibel'skii, V. V. Khromov

Bulletin of the Russian Academy of Sciences PhysicsFeb 1, 19790 citations

Probing the interaction energy of two Rb85 atoms in an optical tweezer via spin-motion coupling

Jun Zhuang, Kunpeng Wang, Pengxiang Wang +8 more

The inherent polarization gradients in tight optical tweezers can be used to couple the atomic spins to the two-body motion under the action of a microwave spin-flip transition, so that such a spin-motion coupling offers an important control knob on the motional states of optically trapped two colliding atoms. Here, after preparing two elastically scattering $^{85}\mathrm{Rb}$ atoms in the three-dimensional ground-state in the optical tweezer, we employed this control in order to probe the colliding energies of elastic and inelastic channels. The combination of microwave spectra and corresponding s-wave pseudopotential model allows us to infer the effect of the state-dependent trapping potentials on the elastic colliding energies, as well as to reveal how the presence of inelastic interactions affects elastic part of the relative potential. Our work shows that the spin-motion coupling in a tight optical tweezer expand the experimental toolbox for fundamental studies of ultracold collisions in the two body systems with reactive collisions, and potentially for that of more complex interactions, such as optically trapped atom-molecule and molecule-molecule interactions.The inherent polarization gradients in tight optical tweezers can be used to couple the atomic spins to the two-body motion under the action of a microwave spin-flip transition, so that such a spin-motion coupling offers an important control knob on the motional states of optically trapped two colliding atoms. Here, after preparing two elastically scattering $^{85}\mathrm{Rb}$ atoms in the three-dimensional ground-state in the optical tweezer, we employed this control in order to probe the colliding energies of elastic and inelastic channels. The combination of microwave spectra and corresponding s-wave pseudopotential model allows us to infer the effect of the state-dependent trapping potentials on the elastic colliding energies, as well as to reveal how the presence of inelastic interactions affects elastic part of the relative potential. Our work shows that the spin-motion coupling in a tight optical tweezer expand the experimental toolbox for fundamental studies of ultracold collisions in the two body systems with reactive collisions, and potentially for that of more complex interactions, such as optically trapped atom-molecule and molecule-molecule interactions.

arXiv:2402.08054Physical Review AApr 23, 20243 citations

^{85}\mathrm{Rb}

atoms in the three-dimensional ground-state in the optical tweezer, we employed this control in order to probe the colliding energies of elastic and inelastic channels. The combination of microwave spectra and corresponding s-wave pseudopotential model allows us to infer the effect of the state-dependent trapping potentials on the elastic colliding energies, as well as to reveal how the presence of inelastic interactions affects elastic part of the relative potential. Our work shows that the spin-motion coupling in a tight optical tweezer expand the experimental toolbox for fundamental studies of ultracold collisions in the two body systems with reactive collisions, and potentially for that of more complex interactions, such as optically trapped atom-molecule and molecule-molecule interactions.