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APS

Exotic phases in Mott insulating Iridates with strong spin-orbit coupling: Phase diagram of the Kitaev-Heisenberg model in a magnetic field

Hong‐Chen Jiang, Zheng‐Cheng Gu, Xiao-Liang Qi, Simon Trebst

Published Mar 1, 2011• 0 citations
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Possible proximity of the Iridates (Na,Li)2_22​IrO3_33​ to a topologically ordered Mott insulator: Phase diagram of the Heisenberg-Kitaev model
Motivated by the recent experimental observation of a Mott insulating state for the layered iridate Na2{}_{2}2​IrO3{}_{3}3​, we discuss possible ordering states of the effective iridium moments in the presence of strong spin-orbit coupling and a magnetic field. For a field pointing in the $\ensuremath{\langle}111\ensuremath{\rangle}$ direction---perpendicular to the hexagonal lattice formed by the iridium moments---we find that a combination of Heisenberg and Kitaev exchange interactions gives rise to a rich phase diagram with both symmetry breaking magnetically ordered phases as well as a topologically ordered phase that is stable over a small range of coupling parameters. Our numerical simulations further indicate two exotic critical points at the boundaries between these ordered phases.
The exact solution of Kitaev's spin-1/21/21/2 honeycomb spin-liquid model has sparked an intense search for Mott insulators hosting bond-dependent Kitaev interactions, of which Na2IrO3{\mathrm{Na}}_{2}{\mathrm{IrO}}_{3}Na2​IrO3​ and $\ensuremath{\alpha}\text{\ensuremath{-}}\mathrm{Ru}{\mathrm{Cl}}_{3}$ are prime examples. Subsequently, it has been proposed that also spin-1 and spin-3/23/23/2 analogs of Kitaev interactions may occur in materials with strong spin-orbit coupling. As a minimal model to describe these Kitaev materials, we study the Heisenberg-Kitaev Hamiltonian in a consistent 1/S1/S1/S expansion, with SSS being the spin size. We present a comprehensive study of this model in the presence of an external magnetic field applied along two different directions, [001] and [111], for which an intricate classical phase diagram has been reported. In both settings, we employ spin-wave theory in a number of ordered phases to compute phase boundaries at the next-to-leading order in 1/S1/S1/S and show that quantum corrections substantially modify the classical phase diagram. More broadly, our work presents a consistent route to investigate the leading quantum corrections in spin models that break spin-rotational symmetry.
We study cold atoms in an optical lattice with synthetic spin-orbit coupling in the Mott-insulator regime. We calculate the parameters of the corresponding tight-binding model using Peierls substitution and "localized Wannier states method" and derive the low-energy spin Hamiltonian for bosons and fermions. The spin Hamiltonian is a combination of Heisenberg model, quantum compass model and Dzyaloshinskii-Moriya interactions and it has a rich classical phase diagram with collinear, spiral and vortex phases. We discuss the state of the art of experiments to realize and detect magnetic orderings in strongly correlated optical lattices.