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arXiv:1205.2110 · Physical Review Letters

Exotic Quantum Spin Models in Spin-Orbit-Coupled Mott Insulators

Juraj Radić, Andrea Di Ciolo, Kai Sun, Victor M. Galitski

Published Aug 20, 2012• 156 citations
arXivHTMLPDF

Abstract

We study cold atoms in an optical lattice with synthetic spin-orbit coupling in the Mott-insulator regime. We calculate the parameters of the corresponding tight-binding model using Peierls substitution and "localized Wannier states method" and derive the low-energy spin Hamiltonian for bosons and fermions. The spin Hamiltonian is a combination of Heisenberg model, quantum compass model and Dzyaloshinskii-Moriya interactions and it has a rich classical phase diagram with collinear, spiral and vortex phases. We discuss the state of the art of experiments to realize and detect magnetic orderings in strongly correlated optical lattices.

DOI
10.1103/physrevlett.109.085303

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We study cold atoms in an optical lattice with synthetic spin-orbit coupling in the Mott-insulator regime. We calculate the parameters of the corresponding tight-binding model using Peierls substitution and "localized Wannier states method" and derive the low-energy spin Hamiltonian for bosons and fermions. The spin Hamiltonian is a combination of Heisenberg model, quantum compass model and Dzyaloshinskii-Moriya interactions and it has a rich classical phase diagram with collinear, spiral and vortex phases. We discuss the state of the art of experiments to realize and detect magnetic orderings in strongly correlated optical lattices.
We show that the recent experimental realization of spin-orbit coupling in ultracold atomic gases can be used to study different types of spin spiral order and resulting multiferroic effects. Spin-orbit coupling in optical lattices can give rise to the Dzyaloshinskii-Moriya (DM) spin interaction which is essential for spin spiral order. By taking into account spin-orbit coupling and an external Zeeman field, we derive an effective spin model in the Mott insulator regime at half filling and demonstrate that the DM interaction in optical lattices can be made extremely strong with realistic experimental parameters. The rich finite temperature phase diagrams of the effective spin models for fermions and bosons are obtained via classical Monte Carlo simulations.
Motivated by the experimental realization of synthetic spin-orbit coupling for ultracold atoms, we investigate the phase diagram of the Bose-Hubbard model in a non-Abelian gauge field in two dimensions. Using a strong coupling expansion in the combined presence of spin-orbit coupling and tunable interactions, we find a variety of interesting magnetic Hamiltonians in the Mott insulator (MI), which support magnetic textures such as spin spirals and vortex and Skyrmion crystals. An inhomogeneous mean-field treatment shows that the superfluid (SF) phases inherit these exotic magnetic orders from the MI and display, in addition, unusual modulated current patterns. We present a slave-boson theory which gives insight into such intertwined spin-charge orders in the SF, and discuss signatures of these orders in Bragg scattering, in situ microscopy, and dynamic quench experiments.
Motivated by recent experimental advances, we study two-component spin-orbit coupled ultracold bosonic atoms in two dimensions on a square optical lattice. Using a Bose-Hubbard model with spin-conserving and non-spin-conserving nearest neighbour hoppings and spin-dependent on-site density-density interaction, our goal is to characterize phase separation and spin structure in the weakly interacting and deep Mott regimes. \nFor the weakly coupled regime, we decouple interactions through a real space uniform density mean field theory. At zero temperature, this gives an analytic condition for the phase separation transition driven by inter- relative to intracomponent interaction. Solving the self-consistent equations at finite temperature reveals entropic remixing in the phase separated regime and a more surprising entropy driven phase separation in the mixed regime. This is a consequence of complex interplay between interaction and spin-orbit coupling, and can be explained through the effect of component imbalance on the effective single-particle dispersion relation. We also provide an alternate explanation based on thermal occupation of eigenstates with a characteristic imbalance.\nIn the strongly interacting Mott regime, we derive an effective spin Hamiltonian describing the magnetic phases of the Mott insulator. The competition between anisotropic {Heisenberg} and Dzyaloshinskii-Moriya interactions gives rise to various ferromagnetic, antiferromagnetic, spiral, stripe, vortex, and skyrmion phases. On basis of classical Monte-Carlo simulations in the literature, we reconstruct the phase diagram with a classical variational approach, while magnon excitation spectra and quantum fluctuations are calculated with Holstein-Primakoff transformation and subsequent spin wave expansion. The analysis shows that states with ferromagnetic or antiferromagnetic ordering of boson species are protected against thermal fluctuations by a gap, and well described by classical states. States with equal superposition of boson species at each lattice site are subject to relatively large quantum fluctuations, which may cause breakdown of the states within their classical parameter space regions. The dispersion relations are gapless and linear around the minima to lowest order in the spin wave expansion.
We study the magnetic interactions in Mott-Hubbard systems with partially filled t_{2g} levels and with strong spin-orbit coupling. The latter entangles the spin and orbital spaces, and leads to a rich variety of the low energy Hamiltonians that extrapolate from the Heisenberg to a quantum compass model depending on the lattice geometry. This gives way to "engineer" in such Mott insulators an exactly solvable spin model by Kitaev relevant for quantum computation. We, finally, explain "weak" ferromagnetism, with an anomalously large ferromagnetic moment, in Sr2IrO4.
We study the topological phases in spin-orbit-coupled dipolar bosons in a one-dimensional optical lattice. The magnetic dipolar interactions between atoms give rise to intersite interactions. In the Mott-insulating regime, this system can be described by the quantum XYZ spin model with Dzyaloshinskii-Moriya interactions in a transverse field. We focus on investigating the effect of dipolar interactions on the topological phase. The topological phase can be shown when spin-orbit coupling combines with the repulsive dipolar interaction. We find that the dipolar interaction can broaden the range of parameters of spin-orbit coupling and transverse field for exhibiting the topological phase. The sum of spin correlations between the two nearest-neighboring atoms can be used to indicate the topological phase. This may be useful for detecting topological phases in experiments.
We use a variational order method to explore the ground state phase diagrams of spin–orbit coupled Bose atoms in optical lattices. By properly parameterizing the order with an ansatz function for each possible phase and comparing their energies which are minimized with respect to the variational parameters, we can effectively identify the lowest energy states and depict the phase diagram. While the Mott-insulator-superfluid phase boundary is computed by the usual Gutzwiller method, the spin-ordered phase structures of the deep Mott regime as well as the superfluid regime are studied by the variational order method. For the isotropic spin–orbit coupling, the phase diagram in the deep Mott insulator regime is qualitatively similar to results derived by the classical Monte-Carlo simulations or other numerical methods. The spiral phases with different spatial periods are discussed in detail. We find three new spin-ordered phases in the deep Mott insulator regime with anisotropic spin–orbit coupling. We also identify the uniform superfluid, stripe and checkerboard supersolid phases with exotic spin orders in the superfluid regime.