We theoretically study the interaction between two semiconductor quantum dots (SQDs) and a metal nanoparticle (MNP) within the quantum description. The plasmon field produced in the MNP excited by ...
Although the enhanced near fields produced by plasmon resonances in metal nanoparticles can enable strong local light-matter interactions, the strong dissipation of plasmon resonances would seem to be incompatible with quantum-mechanical phenomena such as entanglement. Counter to this intuition, the dissipation can in fact lead to the production of transient entanglement between the occupation states of dots coupled to a common plasmonic system. Building on previous results that showed entanglement between pairs of dots, we scale to larger systems of two, three, and more closely spaced dots. Moreover, we show that tuning the degree of coupling between each dot and the common plasmonic nanostructure enables entanglement to be created in the case where the entire system begins in its ground state and is excited by a single laser pulse. Entanglement is achieved without the need for the dots to be individually addressable, and without the need for controlled quantum gates, postselective measurements, or engineering of the dissipative environment. Through analytical solutions and numerical simulation of a model Hamiltonian based on a cavity-quantum-electrodynamics approach, we determine system configurations that maximize pairwise entanglement among the quantum dots, illustrating in principle the potential for true “quantum plasmonics.
We theoretically study the interaction between two semiconductor quantum dots (SQDs) and a metal nanoparticle\ (MNP) within the quantum description. The plasmon field produced in the MNP excited by the external field can play the platform of F\"{o}rster energy transfer between two SQDs which gives rise to the generation of entangled states. The Fano effect can be shown in the energy absorption spectrum of MNP, which originates from constructive or destructive interference between two competing optical pathways. Since the generated entangled state is in one pathway, the steady-state concurrence of entanglement can be evaluated by the observation of Fano profile. Because the concurrence of two SQDs is determined by both the pump intensity and the energy difference, one can properly choose these two parameters for detecting the non-negligible entanglement. When the pump intensity is very strong, there is no entanglement. The method to observe entanglement with the Fano profile, so, has a limited range of applicability. The optical observation is a novel approach to reveal entanglement. It may be used to optically detect quantum entanglement in many solid-state systems.
We study optical effects in a hybrid system composed of a semiconductor quantum dot (SQD) and a spherical metal nanoparticle (MNP) that interacts with a weak probe and a strong pump electromagnetic field. We use modified nonlinear density matrix equations for the description of the optical properties of the system and calculate, numerically, the first-order susceptibilities of the SQD, the MNP, and the total hybrid nanostructure of the probe field in the presence of the pump field. We investigate the dependence of the probe absorption and dispersion spectra of the SQD, the MNP, and the total nanostructure on the interparticle distance and the detuning of the pump field, and stress the influence of the MNP contribution to the total optical response. The results we find are explained according to the theory of two distinct metastates, which constitute conjugations of the SQD excitonic and the MNP plasmonic excitations. We also show that the optical response strongly depends on the actual values of the SQD material parameters.