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Journal of the Optical Society of America A

Theory of forbidden atomic transitions due to cesium and thallium (A)

Bhanu Pratap Das, Supriya Ray, Taesul Lee, J. Riessen, Mina Vajed-Samii, T. P. Das

Published Jun 1, 1980• 0 citations
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We report measurements of the following spontaneous-emission rates in atomic thallium: $A(6{D}_{\frac{3}{2}}\ensuremath{-}7{P}_{\frac{1}{2}})=(5.97\ifmmode\pm\else\textpm\fi{}0.78)\ifmmode\times\else\texttimes\fi{}{10}^{5}{\mathrm{s}}^{\ensuremath{-}1}$, $A(7{P}_{\frac{1}{2}}\ensuremath{-}7{S}_{\frac{1}{2}})=(1.71\ifmmode\pm\else\textpm\fi{}0.07)\ifmmode\times\else\texttimes\fi{}{10}^{7}{\mathrm{s}}^{\ensuremath{-}1}$, $A(7{P}_{\frac{3}{2}}\ensuremath{-}7{S}_{\frac{1}{2}})=(2.37\ifmmode\pm\else\textpm\fi{}0.09)\ifmmode\times\else\texttimes\fi{}{10}^{7}{\mathrm{s}}^{\ensuremath{-}1}$, and $A(8{P}_{\frac{3}{2}}\ensuremath{\rightarrow}\mathrm{all})=(9.2\ifmmode\pm\else\textpm\fi{}1.0)\ifmmode\times\else\texttimes\fi{}{10}^{6}{\mathrm{s}}^{\ensuremath{-}1}$. These results are compared to predictions of theoretical models and lend support to calculations of the recently measured parity-nonconserving circular dichroism of the $6{P}_{\frac{1}{2}}\ensuremath{-}7{P}_{\frac{1}{2}}$ forbidden $M1$ transition in thallium.

Physical Review A•Feb 1, 1982•14 citations
Frequency conversion of cw CO 2 laser radiation to the 276.8 nm ultraviolet range was achieved in a mixture of thallium and cesium vapor by parametric mixing with radiation from a rhodamine 6G dye laser. Two-photon resonance of the pump radiation with the 6 P 1/2 –7 P 3/2 forbidden transition and the proximity of the converted radiation frequency to the frequency of the 6 D 3/2 –7 P 3/2 transition in the thallium atom were utilized. Cesium vapor was used to match the refractive indices of the interacting waves.
We report measurements of the following spontaneous-emission rates in atomic thallium: $A(6{D}_{\frac{3}{2}}\ensuremath{-}7{P}_{\frac{1}{2}})=(5.97\ifmmode\pm\else\textpm\fi{}0.78)\ifmmode\times\else\texttimes\fi{}{10}^{5}{\mathrm{s}}^{\ensuremath{-}1}$, $A(7{P}_{\frac{1}{2}}\ensuremath{-}7{S}_{\frac{1}{2}})=(1.71\ifmmode\pm\else\textpm\fi{}0.07)\ifmmode\times\else\texttimes\fi{}{10}^{7}{\mathrm{s}}^{\ensuremath{-}1}$, $A(7{P}_{\frac{3}{2}}\ensuremath{-}7{S}_{\frac{1}{2}})=(2.37\ifmmode\pm\else\textpm\fi{}0.09)\ifmmode\times\else\texttimes\fi{}{10}^{7}{\mathrm{s}}^{\ensuremath{-}1}$, and $A(8{P}_{\frac{3}{2}}\ensuremath{\rightarrow}\mathrm{all})=(9.2\ifmmode\pm\else\textpm\fi{}1.0)\ifmmode\times\else\texttimes\fi{}{10}^{6}{\mathrm{s}}^{\ensuremath{-}1}$. These results are compared to predictions of theoretical models and lend support to calculations of the recently measured parity-nonconserving circular dichroism of the $6{P}_{\frac{1}{2}}\ensuremath{-}7{P}_{\frac{1}{2}}$ forbidden M1M1M1 transition in thallium.