The first successful experimental realization of a Bose-Einstein condensate (BEC) in 1995 sparked a still growing research activity that in the meantime has led to beautiful and surprising results, such as the interference of matter waves [4], the Mott-superfluid phase transition [49] or the direct observation of Anderson localization of matter waves [10]. The strong interest in BECs arises, among others, from the possibility to investigate known but hard to study quantum systems on a rather macroscopic scale: for example one can load ultra-cold bosons into an optical lattice created by a standing light wave, and thereby simulate a solid state device. When it comes to a measurement on the BEC, however, essentially all measurement techniques result in the destruction of the condensate: for example in the so called “time of flight method” the optical lattice is switched off to observe the expansion of the trapped atoms and thereby directly visualize their momentum distribution, which highlights the condensed component [11]. In this thesis we elaborate on a means to probe a Bose-Einstein condensate from outside, with a scattering particle. The interaction between the probe particle and the bosons allows energy exchange between them, i.e., this setup includes inelastic scattering. After the scattering process, the condensate is still confined in the optical lattice and can therefore be used for further investigations. Of course, this method of probing a BEC is only then a serious alternative if the properties of the BEC can be inferred from the scattering signal. Besides outlining the scattering formalism, the central aim of this work is to show how the properties of the BEC can be deduced from those quantities accessible in a scattering experiment, like for example the transmission or the inelastic cross section. The other, equally strong motivation of this work concerns the signature of the interaction between the bosons in the scattering quantities. The dynamics of an analog classical system depends strongly on the interaction strength, which can induce a complex structure of the underlying phase space like, e.g., the appearance of a separatrix or even the emergence of chaotic dynamics in a globally mixed regular-chaotic phase space. We are interested to which extent such phase-space metamorphosis is reflected in the properties of the scattering particle. Currently light scattering (Bragg spectroscopy) on an optical lattice [78, 77] or rather on an optical lattice embedded into a cavity [62,68,19] is under intense investigation. These efforts predominantly aim at a characterization of the Mott-superfluid transition by specific scattering properties. In the present thesis we focus on condensates loaded in two and three lattice sites, with a large number of bosons. These systems exhibit a diversity of important physical effects (as we will see below) and thus are of paradigmatic relevance for a detailed understanding of multiparticle quantum dynamics in periodic potentials.
The first successful experimental realization of a Bose-Einstein condensate (BEC) in 1995 sparked a still growing research activity that in the meantime has led to beautiful and surprising results, such as the interference of matter waves [4], the Mott-superfluid phase transition [49] or the direct observation of Anderson localization of matter waves [10]. The strong interest in BECs arises, among others, from the possibility to investigate known but hard to study quantum systems on a rather macroscopic scale: for example one can load ultra-cold bosons into an optical lattice created by a standing light wave, and thereby simulate a solid state device. When it comes to a measurement on the BEC, however, essentially all measurement techniques result in the destruction of the condensate: for example in the so called “time of flight method” the optical lattice is switched off to observe the expansion of the trapped atoms and thereby directly visualize their momentum distribution, which highlights the condensed component [11]. In this thesis we elaborate on a means to probe a Bose-Einstein condensate from outside, with a scattering particle. The interaction between the probe particle and the bosons allows energy exchange between them, i.e., this setup includes inelastic scattering. After the scattering process, the condensate is still confined in the optical lattice and can therefore be used for further investigations. Of course, this method of probing a BEC is only then a serious alternative if the properties of the BEC can be inferred from the scattering signal. Besides outlining the scattering formalism, the central aim of this work is to show how the properties of the BEC can be deduced from those quantities accessible in a scattering experiment, like for example the transmission or the inelastic cross section. The other, equally strong motivation of this work concerns the signature of the interaction between the bosons in the scattering quantities. The dynamics of an analog classical system depends strongly on the interaction strength, which can induce a complex structure of the underlying phase space like, e.g., the appearance of a separatrix or even the emergence of chaotic dynamics in a globally mixed regular-chaotic phase space. We are interested to which extent such phase-space metamorphosis is reflected in the properties of the scattering particle. Currently light scattering (Bragg spectroscopy) on an optical lattice [78, 77] or rather on an optical lattice embedded into a cavity [62,68,19] is under intense investigation. These efforts predominantly aim at a characterization of the Mott-superfluid transition by specific scattering properties. In the present thesis we focus on condensates loaded in two and three lattice sites, with a large number of bosons. These systems exhibit a diversity of important physical effects (as we will see below) and thus are of paradigmatic relevance for a detailed understanding of multiparticle quantum dynamics in periodic potentials.
In the present thesis we study several schemes where the detection of the emitted light from an atomic ensemble gives information about the state of the atoms. In chapter 1 we review the basic theory for the light matter interaction in second quantized form. In chapter 2 we show how conservative potentials for the atoms, such as dispersive optical lattices, can be realized experimentally due to the dispersive interaction with a far detuned laser We then review some basic properties of the physics of a particle in a periodic potential. We show that the ground state and the lowest lying excitations of a Bose-Einstein condensate in a dispersive optical lattice can be described by the Bose-Hubbard Hamiltonian. In chapter 3 we study the photonic bandstructure of a chain of fixed pointlike atoms in a biperiodic configuration. We calculate the photonic spectra and the probe transmission if the atoms are in free space and inside a standing wave optical resonator. In chapter 4 we consider light scattering from ultracold atoms in an optical lattice where we calculate the photonic scattering cross section as a function of energy and direction of emission along the Mott-insulator-superfluid phase transition. We take into account the finite tunneling rate for the atoms, when evaluating the scattering cross section of the photons and the effect of photon recoil onto the atoms. In chapter 5 we consider a gas of ultracold atoms trapped at two spatially separated regions in space. Using a two Raman lasers to couple atoms out of the systems we show that it is possible to measure the mean value of the atomic field operator of the two systems by measuring the scattered light intensity of one of the Raman lasers. We show how this setup might be used to measure the temperature of a Bose-Einstein condensate and to monitor the superfluid to Mott-insulator phase transition for a gas of ultracold atoms in an optical lattice.
Cold atoms trapped in optical lattices (crystals of light) provide a pristine platform for exploring quantum many body physics. Motivated by several recent experiments, this thesis examines the equilibrium and non-equilibrium dynamics of a Bose-Einstein condensate (BEC) loaded in a low dimensional optical lattice in order to realize novel quantum phases. There are two main research directions in this thesis. The first one involves the possibility that exotic order spontaneously forms when two-component bosons are trapped in a honeycomb lattice. My studies on this theme is motivated by the observation of a “twisted superfluid” state in Prof. Klaus Sengstock’s group at Hamburg (Soltan-Panahi et al., Nat. Phys. 8, 71 (2012)). A twisted superfluid involves Bose-Einstein condensation into a state whose order parameter has a spatially varying phase. In chapter 3, I study the stability of a Bose-Einstein condensate towards forming a twisted superfluid within the framework of mean field theory. Despite a exhaustive numerical search I do not find a parameter regime with a twisted superfluid. This search involved all experimentally relevant parameter regimes and therefore mean field theory predicted that the experimentalists should not observe a twisted superfluid. I conclude that the experimental observations were either a manifestation of counter superfluidity or due to interactions during time-of-flight. Subsequent experiments showed that the observations were an artifact of the measurement process. The second research direction in this thesis is an exploration of the stability of periodically driven quantum systems (also known as Floquet systems). Floquet systems can be used to realize exotic non-equilibrium quantum phases which do not have a counterpart in static systems. However, the driving can cause these systems to heat up which presents a major obstacle to creating exotic states. To explore this issue in a concrete example, I model an experiment (Parker, Ha, and Chin, Nat. Phys. 9, 769 (2013)) where a Bose-Einstein condensate loaded in an optical lattice is subjected to periodic shaking. I investigate the stability of this Floquet BEC to interactions. This research direction consists of 3 studies. In chapter 4, I first do this analysis for a purely one-dimensional system and identify a large parameter regime where the BEC is stable. In the next two chapters, I go beyond 1D and consider the role of transverse degrees of freedom. This is because the shaken lattice experiments that I model involves a 1D array of pancakes. I find that this geometry leads to much more dissipation than a purely 1D system. This extra dissipation arises because interactions can transfer energy between different directions. In chapter 5, I consider the extreme case where there is no transverse confinement. I find that in the absence of transverse confinement, a one-dimensional Floquet BEC is generically unstable. Finally, in chapter 6, I consider harmonic transverse confinement modeling the crossover between chapters 4 and 5. I find that as the transverse confinement is made stronger, the atom loss rate initially increases, but beyond a critical transverse confinement, the atom loss disappears due to unavailability of phase space for scattering. I also predict that if the transverse confinement is tuned to the vicinity of certain magic values, the heating rate exhibits a sharp drop. I perform similar analyses for a shaken square lattice and find that generically a low-dimensional Floquet BEC can be stabilized by suitably designing the transverse confinement.
Since Feynman's realization of using quantum systems to investigate quantum dynamics, interest in creating controllable quantum systems to simulate condensed matter phenomenon has been high. With the realization of BECs in 1995, the realization of a relatively clean testbed for simulating some of these phenomenon became a reality. \n My PhD research has been an exploration of the production and use of Bose-Einstein Condensates for the study of superfluidity. The first 3 years have been spent in the actual building of a Na BEC apparatus. During this time, we’ve implemented a distinct technique to trap ultra cold Na atoms, i.e. the Optically Plugged Trap. In the process, we have shown how atoms in a linear trap can show spin metastability and thus maintain a nonequilibrium state for long periods of time.\n In studying the interaction of ultra-cold atoms with light, we have developed a technique to measure the velocity distribution of atoms using a standing optical wave (Bragg Spectroscopy). Alongside this, we have also created optical traps for atoms in which we can change to shape of the trap itself to probe different condensed matter systems. The eventual goal being the investigation of condensed matter physics, specifically superfluidity, using ultra-cold atoms.
Bose-Einstein condensate (BEC) is a new state of matter, experimentally realized in a dilute alkali gas of weakly interacting bosons. The gas is cooled to very low temperatures, of the order of nano-Kelvin, at which point a large fraction of the atoms occupy the lowest quantum state. Under such conditions, the quantum effects become apparent on a macroscopic scale. Many fundamental ideas
of quantum mechanics have been realized and proven to be true in experiments,
by studying the Bose-Einstein condensates. Amongst them, the observation of
macroscopic matter wave interference, the creation of vortices, dark and bright
solitons etc, find special mention. The dynamics of this system in presence of an
optical lattice reveals a superfluid to Mott insulator quantum phase transition.
This has opened a new avenue for research on BEC and its applications. From
a theoretical standpoint, the dynamics of BEC can be described by means of an
effective mean-field theory. This formalism is much simpler than the many-body
Schr¨odinger equation and based on a classical nonlinear evolution equation, known
as Gross-Pitaevskii equation. The nonlinear nature of the GPE leads to several interesting phenomena like soliton propagation, vortices, four wave mixing etc.,
which are closely related to nonlinear fiber optics.
The present thesis deals with nonlinear excitations and different phases of BEC
and is organized as follows: after a brief introduction, in chapter two, we start
with BEC in a one-dimensional shallow optical lattice, experiencing both cubic
and quintic nonlinearity. A superfluid density wave, of twice the periodicity of
lattice potential, is identified. This indicates matter redistribution, where atoms
from neighbouring sites have been depleted leading to a density wave behaviour.
Interestingly, it ceases to exist when only one of these interactions is operative.
We predict the loss of superfluidity through a classical dynamical phase transition,
where modulational instability leads to the loss of phase coherence. In presence
of pure two-body interaction, the superfluid density shows a periodicity commensurate
with the lattice potential. Apart from the superfluid state, a density wave
insulating phase is also found to exist, possessing two frequency modulations commensurate
with the lattice potential. A dynamical phase transition connects the
superfluid phase with an insulating phase, which in turn, is connected with the
density wave insulating phase. The solutions are found to be marginally stable, as
per the Vakhitov-Kolokolov (VK) criterion.
Chapter three describes the dynamics of the atomic-molecular Bose-Einstein
condensate (AMBEC) by mean-field Gross-Pitaevskii equation (GPE), taking into
account the atom-molecular interaction, as well as atom-molecule inter-conversion.
The two-body atom-atom, atom-molecule and molecule-molecule interactions are
analogous to the cubic nonlinearity of the standard GPE, whereas, the quadratic
nonlinear term arising from the inter-conversion between atoms and molecules is
identical to the scenario in strongly coupled BEC in one dimension. The presence
of both weak and strong interactions adds further richness to this system. We
find the molecular BEC possesses a complex dark (grey) soliton, while the atomic condensate is a bright one. The energy and momentum of this system is computed
in order to see the effect of the both weak and strong interactions on Lieb mode
profile and compare it with the pure atomic condensate profile. Another class
of solutions exist in this system, where both atomic and molecular condensates
possess bright solitons.
In chapter four, we investigate the effect of a harmonic trap on the dynamics
of grey solitons in Bose-Einstein condensates. It is observed that, these nonlinear
excitations of the cigar-shaped Bose-Einstein condensate have strong coupling
with the trap at low momenta and hence can be effectively isolated from the
Bogoliubov sound modes, which respond weakly to harmonic confinement. This
strong coupling with the trap also makes the grey soliton amenable for control and
manipulation through trap modulation and temporal variation of the two-body interaction.
We have shown that in presence of an expulsive oscillator trap, the grey
soliton gets amplified, while having a compression in its width. Exact solutions are
also obtained in case of the two component Bose-Einstein condensates (TBECs),
where one component is a grey soliton and the other a bright one. The presence
of the trap and inter-species interaction significantly affects the grey soliton dynamics.
Similar to the single component, in the present case, we have shown that
both grey and bright soliton can be compressed simultaneously. A detailed study
of the energy and momentum of the soliton is reported, in order to find the effect
of the trap on the Lieb mode.
In chapter five, we study a BEC-defect complex in a quasi-one dimensional
scenario, where the defect atom moves in the condensate with constant velocity.
Explicit solutions of the coupled mean-field equations, describing defect-grey soliton
dynamics are obtained, demonstrating the coexistence of grey soliton and a
localized defect. Unlike the case of dark soliton, where the defect trapping center
has vanishing superfluid density, the moving grey soliton necessarily possesses a finite superfluid component at the defect location. The presence of the defect can
lower the grey soliton’s maximum velocity, as compared to the defect free case,
where the maximum velocity is the sound velocity. We have also carried out the
stability analysis of the obtained solutions using renormalized momentum formalism
and Vakhitov-Kolokolov criteria and find that the obtained solutions are stable
through both the methods. The grey soliton’s energy gets substantially modified
through its interaction with the defect, opening up the possibility of its control
through defect dynamics.
Chapter six describes a parametrically forced Bose-Einstein condensate in the
presence of a general moving optical lattice. The interaction between the atoms in
the condensate and the time dependent lattice potential leads to a novel propagating
superfluid matter wave, which can be controlled through chirp management.
This system, when placed in a trap, accelerates and undergoes rapid nonlinear
compression, controlled by the chirp. The density achieves its maximum, when
the matter wave changes direction. It is also shown that this system exhibits dynamical
superfluid insulator transition, where superfluidity breaks down and the
condensate transits to an insulating phase. The stability has been investigated
using Vakhitov-Kolokolov criterion and found that it depends on the chirp, as well
as on the nature of the atom-atom interaction. The exact expression for energy
is obtained and analyzed in detail to gain physical understanding of the chirp
management of the sinusoidal excitations and also the dynamical phase transition.
This thesis discusses a series of studies that investigate the effects of interaction – essentially the s-wave scattering – in the various properties of Bose-Einstein condensates (BEC). The phonon wavefunction in a BEC was measured using Bragg spectroscopy and compared with the well-known Bogoliubov theory. Phonons were first excited in a BEC of 3× 10 condensed Na atoms via small-angle two-photon Bragg scattering. Large angle Bragg scattering was then used to probe the momentum distribution. We found reasonable agreement with the theory. With the same technique of Bragg diffraction, we studied the four-wave mixing process for matter waves. The BEC was split into two strong source waves and a weak seed wave. The s-wave scattering coherently mixed pairs of atoms from the sources into the seed and its conjugate wave, creating a pair-correlated atomic beams with “squeezed” number difference. A Feshbach resonance was used to produce ultracold Na2 molecules with initial phase-space density in excess of 20. Starting from an atomic BEC, a magnetic field ramp shifted a bound state from above the threshold of the unbound continuum to below, creating a molecular population with almost zero center-of-mass motion. A reverse field ramp dissociated the cold molecules into free atom pairs carrying kinetic energy dependent on the ramp speed. This dependence provided a measure of the coupling strength between the bound state and the continuum. Condensates were loaded into optical lattices formed with retro-reflected single frequency lasers. Quantum phase transition from the superfluid state to Mott-insulator state was observed in a three dimensional lattice. The increased interaction and flattened dispersion relation led to strongly enhanced quantum depletion in the superfluid state. Thesis Supervisor: Wolfgang Ketterle Title: John D. MacAurthur Professor of Physics
A Bose-Einstein condensate (BEC) is a macroscopic ensemble of atoms that collectively behaves as a single quantum-mechanical object. In this thesis I describe an apparatus built to create and study a BEC, as well as initial experiments carried out using a one-dimensional optical standing wave (optical lattice) to manipulate the BEC. In the first experiment, a weak optical lattice Bragg-reflects a BEC moving in a nearly harmonic trap. The Bragg reflection combined with the harmonic trapping potential cause the BEC to oscillate, much as light oscillates in an optical cavity. In the second experiment, a deep optical lattice applied to an atom cloud for a short duration is used to split and recombine the atomic wavefunction. By doing this we can create two different types of atom interferometer: a small-separation atom interferometer which works with either a BEC or a thermal gas, and a large-separation atom interferometer which works only with a BEC and whose interferometric arms are, in principle, separately addressable. In the third experiment, an optical lattice potential is slowly turned on. Under the influence of this lattice potential, the BEC loses its superfluid properties, but fully regains them when the lattice is turned back off. This behavior is consistent both with a reversible transition to a 1-D Mott insulator state and with mean-field effects in a deep lattice; both interpretations are discussed. In the latter part of this thesis I describe an apparatus designed to accommodate experiments involving both a BEC and an ion. The interactions between an ion and a BEC have never before been experimentally investigated. Our apparatus includes both the means to localize an ion by actively shielding against stray electric fields and to spatially image ions. This should allow future experiments in which a single ion is embedded in a BEC. In addition to imaging ions, the apparatus provides the capability to create high-resolution images of distributions of neutral atoms by photoionizing them and then quickly imaging them. I conclude the thesis with a discussion of future experiments exploring ion-BEC interactions.