This thesis discusses a series of studies that investigate the effects of interaction – essentially the s-wave scattering – in the various properties of Bose-Einstein condensates (BEC). The phonon wavefunction in a BEC was measured using Bragg spectroscopy and compared with the well-known Bogoliubov theory. Phonons were first excited in a BEC of 3× 10 condensed Na atoms via small-angle two-photon Bragg scattering. Large angle Bragg scattering was then used to probe the momentum distribution. We found reasonable agreement with the theory. With the same technique of Bragg diffraction, we studied the four-wave mixing process for matter waves. The BEC was split into two strong source waves and a weak seed wave. The s-wave scattering coherently mixed pairs of atoms from the sources into the seed and its conjugate wave, creating a pair-correlated atomic beams with “squeezed” number difference. A Feshbach resonance was used to produce ultracold Na2 molecules with initial phase-space density in excess of 20. Starting from an atomic BEC, a magnetic field ramp shifted a bound state from above the threshold of the unbound continuum to below, creating a molecular population with almost zero center-of-mass motion. A reverse field ramp dissociated the cold molecules into free atom pairs carrying kinetic energy dependent on the ramp speed. This dependence provided a measure of the coupling strength between the bound state and the continuum. Condensates were loaded into optical lattices formed with retro-reflected single frequency lasers. Quantum phase transition from the superfluid state to Mott-insulator state was observed in a three dimensional lattice. The increased interaction and flattened dispersion relation led to strongly enhanced quantum depletion in the superfluid state. Thesis Supervisor: Wolfgang Ketterle Title: John D. MacAurthur Professor of Physics
This thesis discusses a series of studies that investigate the effects of interaction – essentially the s-wave scattering – in the various properties of Bose-Einstein condensates (BEC). The phonon wavefunction in a BEC was measured using Bragg spectroscopy and compared with the well-known Bogoliubov theory. Phonons were first excited in a BEC of 3× 10 condensed Na atoms via small-angle two-photon Bragg scattering. Large angle Bragg scattering was then used to probe the momentum distribution. We found reasonable agreement with the theory. With the same technique of Bragg diffraction, we studied the four-wave mixing process for matter waves. The BEC was split into two strong source waves and a weak seed wave. The s-wave scattering coherently mixed pairs of atoms from the sources into the seed and its conjugate wave, creating a pair-correlated atomic beams with “squeezed” number difference. A Feshbach resonance was used to produce ultracold Na2 molecules with initial phase-space density in excess of 20. Starting from an atomic BEC, a magnetic field ramp shifted a bound state from above the threshold of the unbound continuum to below, creating a molecular population with almost zero center-of-mass motion. A reverse field ramp dissociated the cold molecules into free atom pairs carrying kinetic energy dependent on the ramp speed. This dependence provided a measure of the coupling strength between the bound state and the continuum. Condensates were loaded into optical lattices formed with retro-reflected single frequency lasers. Quantum phase transition from the superfluid state to Mott-insulator state was observed in a three dimensional lattice. The increased interaction and flattened dispersion relation led to strongly enhanced quantum depletion in the superfluid state. Thesis Supervisor: Wolfgang Ketterle Title: John D. MacAurthur Professor of Physics
Bose-Einstein condensate (BEC) is a new state of matter, experimentally realized in a dilute alkali gas of weakly interacting bosons. The gas is cooled to very low temperatures, of the order of nano-Kelvin, at which point a large fraction of the atoms occupy the lowest quantum state. Under such conditions, the quantum effects become apparent on a macroscopic scale. Many fundamental ideas
of quantum mechanics have been realized and proven to be true in experiments,
by studying the Bose-Einstein condensates. Amongst them, the observation of
macroscopic matter wave interference, the creation of vortices, dark and bright
solitons etc, find special mention. The dynamics of this system in presence of an
optical lattice reveals a superfluid to Mott insulator quantum phase transition.
This has opened a new avenue for research on BEC and its applications. From
a theoretical standpoint, the dynamics of BEC can be described by means of an
effective mean-field theory. This formalism is much simpler than the many-body
Schr¨odinger equation and based on a classical nonlinear evolution equation, known
as Gross-Pitaevskii equation. The nonlinear nature of the GPE leads to several interesting phenomena like soliton propagation, vortices, four wave mixing etc.,
which are closely related to nonlinear fiber optics.
The present thesis deals with nonlinear excitations and different phases of BEC
and is organized as follows: after a brief introduction, in chapter two, we start
with BEC in a one-dimensional shallow optical lattice, experiencing both cubic
and quintic nonlinearity. A superfluid density wave, of twice the periodicity of
lattice potential, is identified. This indicates matter redistribution, where atoms
from neighbouring sites have been depleted leading to a density wave behaviour.
Interestingly, it ceases to exist when only one of these interactions is operative.
We predict the loss of superfluidity through a classical dynamical phase transition,
where modulational instability leads to the loss of phase coherence. In presence
of pure two-body interaction, the superfluid density shows a periodicity commensurate
with the lattice potential. Apart from the superfluid state, a density wave
insulating phase is also found to exist, possessing two frequency modulations commensurate
with the lattice potential. A dynamical phase transition connects the
superfluid phase with an insulating phase, which in turn, is connected with the
density wave insulating phase. The solutions are found to be marginally stable, as
per the Vakhitov-Kolokolov (VK) criterion.
Chapter three describes the dynamics of the atomic-molecular Bose-Einstein
condensate (AMBEC) by mean-field Gross-Pitaevskii equation (GPE), taking into
account the atom-molecular interaction, as well as atom-molecule inter-conversion.
The two-body atom-atom, atom-molecule and molecule-molecule interactions are
analogous to the cubic nonlinearity of the standard GPE, whereas, the quadratic
nonlinear term arising from the inter-conversion between atoms and molecules is
identical to the scenario in strongly coupled BEC in one dimension. The presence
of both weak and strong interactions adds further richness to this system. We
find the molecular BEC possesses a complex dark (grey) soliton, while the atomic condensate is a bright one. The energy and momentum of this system is computed
in order to see the effect of the both weak and strong interactions on Lieb mode
profile and compare it with the pure atomic condensate profile. Another class
of solutions exist in this system, where both atomic and molecular condensates
possess bright solitons.
In chapter four, we investigate the effect of a harmonic trap on the dynamics
of grey solitons in Bose-Einstein condensates. It is observed that, these nonlinear
excitations of the cigar-shaped Bose-Einstein condensate have strong coupling
with the trap at low momenta and hence can be effectively isolated from the
Bogoliubov sound modes, which respond weakly to harmonic confinement. This
strong coupling with the trap also makes the grey soliton amenable for control and
manipulation through trap modulation and temporal variation of the two-body interaction.
We have shown that in presence of an expulsive oscillator trap, the grey
soliton gets amplified, while having a compression in its width. Exact solutions are
also obtained in case of the two component Bose-Einstein condensates (TBECs),
where one component is a grey soliton and the other a bright one. The presence
of the trap and inter-species interaction significantly affects the grey soliton dynamics.
Similar to the single component, in the present case, we have shown that
both grey and bright soliton can be compressed simultaneously. A detailed study
of the energy and momentum of the soliton is reported, in order to find the effect
of the trap on the Lieb mode.
In chapter five, we study a BEC-defect complex in a quasi-one dimensional
scenario, where the defect atom moves in the condensate with constant velocity.
Explicit solutions of the coupled mean-field equations, describing defect-grey soliton
dynamics are obtained, demonstrating the coexistence of grey soliton and a
localized defect. Unlike the case of dark soliton, where the defect trapping center
has vanishing superfluid density, the moving grey soliton necessarily possesses a finite superfluid component at the defect location. The presence of the defect can
lower the grey soliton’s maximum velocity, as compared to the defect free case,
where the maximum velocity is the sound velocity. We have also carried out the
stability analysis of the obtained solutions using renormalized momentum formalism
and Vakhitov-Kolokolov criteria and find that the obtained solutions are stable
through both the methods. The grey soliton’s energy gets substantially modified
through its interaction with the defect, opening up the possibility of its control
through defect dynamics.
Chapter six describes a parametrically forced Bose-Einstein condensate in the
presence of a general moving optical lattice. The interaction between the atoms in
the condensate and the time dependent lattice potential leads to a novel propagating
superfluid matter wave, which can be controlled through chirp management.
This system, when placed in a trap, accelerates and undergoes rapid nonlinear
compression, controlled by the chirp. The density achieves its maximum, when
the matter wave changes direction. It is also shown that this system exhibits dynamical
superfluid insulator transition, where superfluidity breaks down and the
condensate transits to an insulating phase. The stability has been investigated
using Vakhitov-Kolokolov criterion and found that it depends on the chirp, as well
as on the nature of the atom-atom interaction. The exact expression for energy
is obtained and analyzed in detail to gain physical understanding of the chirp
management of the sinusoidal excitations and also the dynamical phase transition.
The first successful experimental realization of a Bose-Einstein condensate (BEC) in 1995 sparked a still growing research activity that in the meantime has led to beautiful and surprising results, such as the interference of matter waves [4], the Mott-superfluid phase transition [49] or the direct observation of Anderson localization of matter waves [10]. The strong interest in BECs arises, among others, from the possibility to investigate known but hard to study quantum systems on a rather macroscopic scale: for example one can load ultra-cold bosons into an optical lattice created by a standing light wave, and thereby simulate a solid state device. When it comes to a measurement on the BEC, however, essentially all measurement techniques result in the destruction of the condensate: for example in the so called “time of flight method” the optical lattice is switched off to observe the expansion of the trapped atoms and thereby directly visualize their momentum distribution, which highlights the condensed component [11]. In this thesis we elaborate on a means to probe a Bose-Einstein condensate from outside, with a scattering particle. The interaction between the probe particle and the bosons allows energy exchange between them, i.e., this setup includes inelastic scattering. After the scattering process, the condensate is still confined in the optical lattice and can therefore be used for further investigations. Of course, this method of probing a BEC is only then a serious alternative if the properties of the BEC can be inferred from the scattering signal. Besides outlining the scattering formalism, the central aim of this work is to show how the properties of the BEC can be deduced from those quantities accessible in a scattering experiment, like for example the transmission or the inelastic cross section. The other, equally strong motivation of this work concerns the signature of the interaction between the bosons in the scattering quantities. The dynamics of an analog classical system depends strongly on the interaction strength, which can induce a complex structure of the underlying phase space like, e.g., the appearance of a separatrix or even the emergence of chaotic dynamics in a globally mixed regular-chaotic phase space. We are interested to which extent such phase-space metamorphosis is reflected in the properties of the scattering particle. Currently light scattering (Bragg spectroscopy) on an optical lattice [78, 77] or rather on an optical lattice embedded into a cavity [62,68,19] is under intense investigation. These efforts predominantly aim at a characterization of the Mott-superfluid transition by specific scattering properties. In the present thesis we focus on condensates loaded in two and three lattice sites, with a large number of bosons. These systems exhibit a diversity of important physical effects (as we will see below) and thus are of paradigmatic relevance for a detailed understanding of multiparticle quantum dynamics in periodic potentials.
This thesis focuses on the analysis of Bardeen-Cooper-Schrieffer (BCS) \nto Bose-Einstein condensation (BEC) evolution in ultracold superfluid \nFermi gases when the interaction between atoms is varied. The tuning of \nattractive interactions permits the ground state of the system to evolve from a weak \nfermion attraction BCS limit of loosely bound and largely overlapping Cooper pairs \nto a strong fermion attraction limit of tightly bound small bosonic molecules \nwhich undergo BEC. \nThis evolution is accompanied by anomalous behavior of many superfluid \nproperties, and reveals several quantum phase transitions. \nThis thesis has two parts: \nIn the first part, I analyze zero and nonzero orbital angular momentum \npairing effects, and show that a quantum phase transition occurs for \nnonzero angular momentum pairing, unlike the s-wave case where the BCS \nto BEC evolution is just a crossover. \nIn the second part, I analyze two-species fermion mixtures with mass and \npopulation imbalance in continuum, trap and lattice models. In contrast with \nthe crossover physics found in the mass and population balanced mixtures, \nI demonstrate the existence of phase transitions between normal and \nsuperfluid phases, as well as phase separation between superfluid (paired) \nand normal (excess) fermions in imbalanced mixtures as a function of scattering \nparameter and mass and population imbalance.
The year 2015 marks the 20th anniversary of the achievement of Bose–Einstein condensation (BEC) in atomic vapors. Atomic BEC, realized by Eric Cornell, Carl Wieman and Wolfgang Ketterle in 1995, commenced an exciting wave to explore quantum few- and many-body physics. Different from solid state matter and helium superfluids, atomic condensates in the gas phase come with drastically lower densities and temperatures, which place the systems in a unique regime where the atomic interactions are simple and precisely known. Furthermore, the condensates are typically weakly interacting: the interaction length scale of few nanometers is much shorter than the interatomic separation of hundreds of nanometers. Thus many early experimental observations can be well understood based on mean-field theory. One celebrated model is the Gross-Pitaevskii equation which provides a precise and quantitative description of weakly interacting Bose condensates [1]. Opportunities to extend cold atom research beyond the weak interaction regime emerged in the early 2000s. Several experimental schemes were developed to prepare atoms in the strong correlation and interaction regimes. One approach is loading atoms into an optical lattice, the interference pattern of laser beams. The lattice potential enhances the interactions of localized atoms and quenches their kinetic energy. A variety of lattice configurations are realized that promise novel quantum phases of ultracold atoms. Another route to strong interaction is based on Feshbach resonance, typically induced by magnetically shifting a molecular state near the scattering continuum of atoms. The resonant coupling between scattering atoms and the molecular state leads to a divergence of the atomic interaction length scale. Exactly on Feshbach resonance, the collision cross section reaches the quantum mechanical limit, and the system becomes strongly hydrodynamic with mean-free path as short as interparticle separation. Fascinating observations in the strong coupling regime soon followed: prominent examples include the superfluid-Mott insulator transition in optical lattices [2], resonantly interacting Fermi gases in the BEC–BCS (Bardeen–Cooper–Schieffer superfluid) crossover [3] and Efimov three-body states [4], and they lead to tremendous research interest into novel quantum states and quantum dynamics. One of the key motivations in these explorations is to uncover new, universal principles that underpin the physics of strongly correlated quantum systems. A well-studied universal behavior in many-body physics manifests in the critical phenomena near a continuous phase transition. Near the critical point, the system develops a diverging correlation length, which suppresses the dependence on other microscopic length scales. The systems are thus scale invariant and can be universally characterized by a few critical exponents. In cold atoms, divergence of correlation lengthes has been observed near the superfluid phase transition [5,6], as well as the superfluid-Mott insulator quantum phase transition in optical lattices. In the lattice experiments, scale invariance can be tested based on the equation of state measurements [7]. These works complement the transport measurements in condensed matter experiments. Has a new class of universal physics been discovered in atomic quantum gases? Yes, it turns out that a special class of strongly interacting quantum gas with ‘intrinsic’ scaling symmetry emerges near a Feshbach resonance [8]. Near the resonance, the scattering length scale diverges a → ∞ [9], unimaginable in classical systems, and the interaction length reaches the maximum value allowed by quantum mechanics as 1/k, called the ‘unitarity limit’ and k is the momentum of the scattering state. A famous example is the strongly interacting Fermi gas in the BEC–BCS crossover regime, where the resonant interactions lead to strong pairing and and universal hydrodynamic behavior. An exciting development in the study of the BEC–BCS crossover focuses on the Fermi gas exactly on Feshbach resonance. Here the system, also called a ‘unitary Fermi gas’, is the most complex and strongly correlated. The resonant interaction, however, implies a special scaling symmetry of the system. To understand the symmetry, we consider a scale transformation: x → Λx that stretches the coordinates of all atoms by a factor of Λ, and thus reduces the atomic density n by a factor of Λ3 in a 3D gas and the kinetic energy Ek ∝ −∇2 by Λ2. One can see that both kinetic energy Ek and interaction energy in the unitarity limit na → n/k are reduced by the same factor Λ2. The system is thus hypothesized to be invariant under the scale transformation [8]. Remarkably, similar scaling symmetry also holds for 2D quantum gas with a constant coupling g = const. [10]. Here stretching the size of the 2D gas by a factor of Λ also reduces both the kinetic Ek and interaction energy gσ by Λ2, where σ is the 2D density. Since the scaling symmetry in these systems comes directly from the form of the interactions, intrinsic scale invariance is robust at all temperatures T and chemical potentials μ and does not rely on the proximity to a phase transition. The scaling symmetry suggests that the only independent variables are the ratios of the length scales or the equivalent energy scales. In a grand canonical ensemble, the independent ratio can be chosen as μ/kBT. This realization greatly simplifies theoretical description as well as the experimental characterization of the system. Theoretically, a new set of universal thermodynamic relations are expected to be insensitive to the microscopic details; experimentally, measurements are expected to collapse into universal functions that only depend on μ/kBT. Measurements on unitary Fermi gas and the 2D Bose gas are consistent with the scaling hypothesis, shown in Fig. 1(a) and (b). Remarkable quantitative agreement between measurements and calculations has greatly advanced our understanding of the ‘unitary Fermi gas’ and 2D atomic gas. Ultracold atomic gases which are intrinsically scale invariant: (a) unitary Fermi gas, (b) 2D Bose gas and (c) unitary Bose gas. The scaling symmetry suggests that thermodynamic observables only depend on the ratio of chemical potential and thermal energy |μ~=μ/kBT|. In (a), thermodynamic pressure of a unitary Fermi gas is compared with calculations and other measurements. Figure courtesy of M. Zwierlein [11]. In (b), the collapse of the density measurement at various temperatures (inset) confirms the scaling symmetry. Figure adopted from [12]. Panel (c) shows the three-body loss spectrum in a 6Li133Cs mixture. The geometric progression of the Efimov resonance positions at B = B1, B2 and B3 toward the Feshbach resonance at B0 results from the discrete scaling symmetry of Efimov physics. Figure adopted from [13]. We may expect the same scaling symmetry for a resonantly interacting Bose gas. Here, however, the scaling symmetry is more subtle because of the presence of three-body physics. Predicted by Vitaly Efimov in the context of nuclear physics [14], an infinite number of three-body bound states exist for resonantly interacting bosons and their energies follow a discrete scaling law, breaking the otherwise continuous scaling symmetry. Identical fermions do not form such three-body states due to Pauli's exclusion principle. Theoretically the three-body bound states are supported by the ‘Efimov potential’ V(R)∝ − 1/R2, where R is the characteristic length scale of the three interacting atoms. While the Efimov potential does not break the continuous scaling symmetry, the presence of discrete three-body states does break the symmetry. An alternative picture based on renormalization group limited cycles [15] also explains the discrete scaling symmetry of the system, a scenario that rarely happens in electronic systems. Experimentally, Efimov states have been observed in cold gases of alkali atoms, as well as in helium-4. The geometric scaling symmetry of Efimov states is reported in a recent experiment, shown in Fig. 1(c). The same discrete scaling symmetry is expected for unitary quantum gas of bosons, which, if confirmed, will establish a unique and fascinating class of strongly interacting quantum systems. While in this article, we focus on atoms in optical lattices and unitary atomic gases as primary examples of universal physics that have been actively investigated, efforts in many new research frontiers have shown promising prospects to uncover new universal physics in the strongly correlated and interacting systems. Non-equilibrium dynamics is one of the hottest directions. Ultracold atoms are particularly suited for the study of quantum dynamics due to their slow evolution time scales of miniseconds to seconds. Dynamics near a quantum phase transition and the thermalization of isolated quantum systems are two research topics with many unanswered questions. Cold atom experiments may provide new universal insights that go beyond current theoretical framework. Another exciting direction is quantum many-body systems with long range or very strong interactions. Examples include trapped ions, and condensates of exotic atoms with huge magnetic dipole moments, polar molecules, as well as those with Rydberg excitations. These systems possess various long range interactions. Novel universal dynamics, for example, propagation of information and entanglement, are predicted to depend solely on the asymptotic form of the interaction and the dimension of the systems. The author thanks Yijun Wang for discussion and careful reading of the article. This work was supported by National Science Foundation (PHY-0747907) and Army Research Office-Multiple University Research Initiative (W911NF-14-1-0003).
This thesis reports on the first observation of optical tuning of interactions in an ultracold atomic gas. To control the elastic interactions, we use optically induced scattering resonances. They are realized by coupling pairs of atoms to a bound molecular state with the help of laser light. In comparison to the well-known magnetic Feshbach resonances, these optical Feshbach resonances allow a very fast switching of interactions in a spatially resolved way. This is because laser light can be switched on and off much faster than magnetic fields and because the light intensity can be spatially structured. Our experiments are performed with a Bose-Einstein condensate (BEC) of Rb atoms, which we produce in our new BEC setup. This apparatus has been constructed in the framework of this thesis and offers excellent optical access to the ultracold atom cloud. To investigate the tunability of atomic interactions with single-frequency laser light, we optically couple pairs of free atoms to an electronically excited molecular state. The coupling is achieved with a laser that is tuned close to the respective free-bound photoassociation transition. By changing the laser detuning we are able to adjust the atomic scattering length to any value between 10 a0 and 190 a0, where a0 denotes the Bohr radius. The atomic scattering length is a single quantity that fully describes ultracold elastic interactions. Since laser induced atom losses restrict the duration of our experiments, Bragg spectroscopy is employed as a fast method to measure the scattering length. We also demonstrate that optical Feshbach resonances can be realized with a two-color Raman coupling scheme. To implement this scheme, a second laser is added that couples the excited molecular state to a weakly bound molecular level in a ground state potential. Tuning the second laser results in a modification of the atomic scattering length similar to the one observed with a single laser. In addition, this scheme allows to control the width of the resonance via the detuning of the first laser. For the one-color and two-color coupling schemes, we investigate how the elastic scattering properties depend on the different available parameters, i.e. the laser detunings and intensities. Our experimental findings can successfully be described with an available theoretical model, which treats ultracold collisions in the presence of laser light. Optical Feshbach resonances have the possibility of becoming a valuable tool for fast switching of interactions. This is of special interest in quantum computation schemes with neutral atoms, where interactions between different atomic qubits need to be controlled.
A Bose-Einstein condensate (BEC) is a macroscopic ensemble of atoms that collectively behaves as a single quantum-mechanical object. In this thesis I describe an apparatus built to create and study a BEC, as well as initial experiments carried out using a one-dimensional optical standing wave (optical lattice) to manipulate the BEC. In the first experiment, a weak optical lattice Bragg-reflects a BEC moving in a nearly harmonic trap. The Bragg reflection combined with the harmonic trapping potential cause the BEC to oscillate, much as light oscillates in an optical cavity. In the second experiment, a deep optical lattice applied to an atom cloud for a short duration is used to split and recombine the atomic wavefunction. By doing this we can create two different types of atom interferometer: a small-separation atom interferometer which works with either a BEC or a thermal gas, and a large-separation atom interferometer which works only with a BEC and whose interferometric arms are, in principle, separately addressable. In the third experiment, an optical lattice potential is slowly turned on. Under the influence of this lattice potential, the BEC loses its superfluid properties, but fully regains them when the lattice is turned back off. This behavior is consistent both with a reversible transition to a 1-D Mott insulator state and with mean-field effects in a deep lattice; both interpretations are discussed. In the latter part of this thesis I describe an apparatus designed to accommodate experiments involving both a BEC and an ion. The interactions between an ion and a BEC have never before been experimentally investigated. Our apparatus includes both the means to localize an ion by actively shielding against stray electric fields and to spatially image ions. This should allow future experiments in which a single ion is embedded in a BEC. In addition to imaging ions, the apparatus provides the capability to create high-resolution images of distributions of neutral atoms by photoionizing them and then quickly imaging them. I conclude the thesis with a discussion of future experiments exploring ion-BEC interactions.