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A new platform for atom-light interactions on the nano-scale

William Hamlyn

Published Jan 1, 2020• 1 citation
OpenAlex

Abstract

We present the design, fabrication, and operation of a new genera-tion of thermal alkali vapour nano-cells. The nano-cells include in-ternal structures with length scales 200−2000 nm created by laserlithography and reactive ion etching. The assembly process adoptsoptical contact bonding and glassblowing, avoiding the requirementfor any bonding agents or adhesives. We demonstrate a novel methodfor characterising the size of the internal vapour nano-channels. Thedesign allows for greater optical access and compatibility with highnumerical aperture (NA=0.7) optics; we demonstrate this with totalinternal reflection fluorescence spectroscopy and high resolution ima-ging of the nano-channels. Additionally, we report for the first time onthe photon statistics of light from a thin atomic ensemble. Finally, wediscuss the diffusion of atoms inside confined geometries with a num-ber of detection methods, and investigate options for controlling andmanipulating the atomic density and its diffusion. In total, we presentour new nano-cell design as a significant advancement of the field andpropose its use in scalable atomic and quantum optics applications andtechnologies.

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We present the design, fabrication, and operation of a new genera-tion of thermal alkali vapour nano-cells. The nano-cells include in-ternal structures with length scales 200−2000 nm created by laserlithography and reactive ion etching. The assembly process adoptsoptical contact bonding and glassblowing, avoiding the requirementfor any bonding agents or adhesives. We demonstrate a novel methodfor characterising the size of the internal vapour nano-channels. Thedesign allows for greater optical access and compatibility with highnumerical aperture (NA=0.7) optics; we demonstrate this with totalinternal reflection fluorescence spectroscopy and high resolution ima-ging of the nano-channels. Additionally, we report for the first time onthe photon statistics of light from a thin atomic ensemble. Finally, wediscuss the diffusion of atoms inside confined geometries with a num-ber of detection methods, and investigate options for controlling andmanipulating the atomic density and its diffusion. In total, we presentour new nano-cell design as a significant advancement of the field andpropose its use in scalable atomic and quantum optics applications andtechnologies.
Atom-light interactions in nano-scale systems hold great promise for novel technologies based on integrated emitters and optical modes. We present the design architecture, construction method, and characterization of an all-glass alkali-metal vapor cell with nanometer-scale internal structure. Our cell has a glue-free design which allows versatile optical access, in particular with high numerical aperture optics. By performing spectroscopy in different illumination and detection schemes, we investigate atomic densities and velocity distributions in various nanoscopic landscapes. We apply a two-photon excitation scheme to atoms confined in one dimension within our cells, achieving a resonance line-width of 32 MHz in a counter-propagating geometry, and 57.5 MHz in a co-propagating geometry. Both of these are considerably narrower than the Doppler width (GHz), and are limited by transit time broadening and velocity selection. We also demonstrate sub-Doppler line-widths for atoms confined in two dimensions to micron-sized channels. Furthermore, we illustrate control over vapor density within our cells through nano-scale confinement alone, which could offer a scalable route towards room-temperature devices with single atoms within an interaction volume. Our design offers a robust platform for miniaturized devices that could easily be combined with integrated photonic circuits.
The confinement of atoms at the nanoscale is of interest for a diverse range of applications, from spatially selective sensing on the submicrometer scale to emerging quantum technologies. This study describes a bespoke method for manufacturing robust vapor cells with arbitrary nanoscale-confinement geometries. The device is designed with versatile, high-NA optical access. Spectroscopy of Rb atoms in purpose-built cells yields important insight into the diffusion and spatial distribution of a thermal vapor confined to a nanochannel. This work offers routes toward engineering solutions for localized control of atom numbers for scalable quantum optical experiments.
Alkali vapors confined in nano-scale cells are promising tools for future integrated atom-based sensor. In this thesis, we investigate the interaction between light and an ensemble of atoms confined in a nano-geometry. We focus on the different processes that can modify the optical response of the atomic ensemble and possibly affect the sensitivity of a sensor based on that technology. First, we study the non-local response of atoms to a light excitation due the atomic motion in thermal vapors. When the distance over which the atoms relaxes is larger than the size of the cell, the optical response depends on the size of the system. We have observed that for transmission spectroscopy, this leads to a periodic modification of the optical response with a period equal to the wavelength of the optical transition. Subsequently we showed that when the density of atom increases, the atomic response becomes local again. In this dense regime, the resonant dipole-dipole interaction in a sub-wavelength geometry leads to collective frequency shifts of the spectral lines. We demonstrate that these shifts were induced by the cavity formed by the cell walls, hence clarifying a long-standing issue. We developed a model to extract the density shifts deconvolved from the cavity effects. Close to a surface, the optical response is also affected by the van der Waals atom-surface interaction. We introduced a new method to extract precisely the strength of this interaction. We also developed a new generation of super-polished glass nano-cells and we presented promising spectroscopic signals. Finally, using these cells, we have compared transmission and off-axis spectroscopic techniques.
This thesis presents the study of thermal alkali-metal vapours confined in a layer with a sub-micron thickness. This confinement enables the study of high density media without the loss of signal present in usually thermal vapours, but also has additional effects on spectra acquired from the system. Such effects include the suppression of the Doppler broadening and the interaction of the atoms with nearby surfaces. Herein, we present a study of this atom-surface interaction in both Rubidium and Caesium atoms, demonstrating that the interaction follows a power law of 1/rα1/r^\alpha1/rα, where α=3.02±0.06\alpha = 3.02 \pm 0.06α=3.02±0.06. We also study Rabi oscillations at high densities, driving GHz Rabi oscillations in a Rb vapour at densities up to 101710^{17}1017~cm−3^{-3}−3. We find that the results do not have sufficient agreement with an optical Bloch simulation, but Maxwell Bloch simulations indicate the possible presence of simultons; simultaneously propagating solitons. Such phenomena have not yet been observed out of crystalline media. We also present a study of causality relations in atomic media. We first discuss the equivalency of the Hilbert transform to the Kramers-Kronig relations, well known in signal processing, but rarely applied in atomic physics. We then demonstrate that the Hilbert transform can be applied to atomic transmission spectra to quickly generate refractive index spectra. The final section of this thesis fully details the successful design and fabrication of vapour cells with a thickness of 500-1500~nm. The cells are assembled using a combination of traditional scientific glass blowing techniques and thermally annealed optically contacted plates. We fully outline the production process, and then present evidence of their successful functionality and longevity.
Alkali vapours, such as rubidium, are being used extensively in several important fields of research such as slow and stored light nonlinear optics quantum computation, atomic clocks and magnetometers. Recently, there is a growing effort towards miniaturizing traditional centimetre-size vapour cells. Owing to the significant reduction in device dimensions, light–matter interactions are greatly enhanced, enabling new functionalities due to the low power threshold needed for nonlinear interactions. Here, taking advantage of the mature platform of silicon photonics, we construct an efficient and flexible platform for tailored light–vapour interactions on a chip. Specifically, we demonstrate light–matter interactions in an atomic cladding waveguide, consisting of a silicon nitride nano-waveguide core with a rubidium vapour cladding. We observe the efficient interaction of the electromagnetic guided mode with the rubidium cladding and show that due to the high confinement of the optical mode, the rubidium absorption saturates at powers in the nanowatt regime. Alkali vapours are increasingly useful in photonic research and metrology applications, and they provide a useful test bed for investigating light–matter interaction. Stern et al. integrate silicon nitride waveguides with alkali vapours to study light–matter interactions on a chip-scale platform.