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The dynamics of laser cooled ions in a quadrupole ion trap

Kishan Dholakia

Published Jan 1, 1994• 0 citations
OpenAlex

Abstract

This thesis describes experimental work performed on laser cooled magnesium ions, confined in a quadrupole ion trap operating in the Penning or the combined mode. Information is gained about the dynamical motion of the ions. This is done by analyzing the time delays between scattered fluorescence photons in the case of small ion clouds (generally less than ten ions). For larger clouds (upwards of 100 ions), a fraction of the ions is "tagged" and a subsequent study made of the time evolution of the fluorescence. We have developed an innovative, non-invasive method for measuring ion oscillation frequencies which is based on analyzing photon-photon correlations present in the emitted ion fluorescence. This technique has been used to measure all three Penning trap frequencies for a wide range of dc voltage. The data have been fitted to theory and we have obtained a global fit of these data to one set of trap parameters. We also demonstrate that our technique enables us to measure space-charge shifted values of the trap resonances. This method has also been applied to the combined trap and we report experimental verification of the predicted trap resonances for a wide range of trapping parameters. These data fit well to theory. This is for all three oscillation frequencies for one set of trap parameters consistent with the data for the Penning trap. \nFurther experiments are reported concerned with the dynamics of larger ion clouds in a Penning trap. A pulsed laser is used to "tag" a small number of the ions in large ion clouds. This removes those ions from the cooling cycle by placing them in a metastable state. Subsequently, we have monitored the time evolution of the fluorescence. By analyzing these data we have been able to determine cloud rotation frequencies for large ensembles of ions.

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Photon-correlation detection of ion-oscillation frequencies in quadrupole ion traps

Kishan Dholakia, G. Horváth, D. M. Segal +3 more

We present a method for measuring ion-oscillation frequencies in quadrupole traps (Paul, Penning, and combined traps). The method depends on a statistical analysis of the delays between detected fluorescence photons. We have used the method to verify the oscillation frequencies for magnesium ions in a Penning trap as a function of the dc voltage applied to the trap electrodes. We demonstrate that, as expected, the method measures the space-charge shifted (individual-ion) oscillation frequency and not the frequency at which the ion cloud as a whole moves. However, our data suggest that for most of our operating conditions, the space-charge shift is negligible. We also discuss the effect of the contact potential arising from areas of the trap electrodes that are coated by excess Mg from the atomic beam used. We show that this extra potential shifts the center of the Penning trap and makes it unstable for low values of the applied voltage.

Physical Review A•Jan 1, 1993•30 citations

A study of trapped ion dynamics by photon-correlation and pulse-probe techniques

J. Rink, Kishan Dholakia, G. Horváth +6 more

We demonstrate non‐evasive methods for observing ion and ion cloud oscillation frequencies in a quadrupole ion trap. These trap resonances are measured for small clouds using a photon correlation technique. For large clouds the rotation frequency can be detected with the help of an additional pulsed probe laser. We show applications of the photon correlation method such as estimating the dynamic properties of a combined trap and detecting ion crystals.

AIP conference proceedings•Jan 1, 1995•0 citations

Ion dynamics in perturbed quadrupole ion traps

G. Horváth, José Luis Hernández‐Pozos, Kishan Dholakia +3 more

We use the results of a Lagrangian formulation of the dynamics of ions in a Penning trap to calculate the motional frequencies of the ions as a function of the trapping parameters. We then add realistic perturbations to the ideal trapping fields in the formalism and deduce the effects of these perturbations on the ion motion. For an ideal trap there exist values of the applied trapping fields that result in a degeneracy in the ion oscillation frequencies associated with different types of motion. We show that this motional frequency degeneracy is lifted by the inclusion of the effect of a tilt of the trap axis with respect to the axis of the applied magnetic field, leading to an ``avoided crossing'' between the oscillation frequencies. We calculate typical ion orbits for trap parameters that give oscillation frequencies near the avoided crossing between the axial and modified cyclotron frequencies. We generalize the analysis to include the motion of ions in a combined (Penning-Paul) trap and perform an experiment to test the predictions of the theory for a degeneracy between the modified cyclotron frequency and the axial frequency for ${\mathrm{Mg}}^{+}$ ions held in a tilted combined trap. The oscillation frequencies are measured for a range of tilt angles using a photon-photon correlation technique. There is good agreement between the experimental results and the theoretical predictions. The method we describe may prove to be a useful means by which trap imperfections can be identified and subsequently removed.

Physical Review A•Mar 1, 1998•28 citations

Ion dynamics and oscillation frequencies in a linear combined trap

T. Nakamura, S. Ohtani, M. Wada +3 more

Ion traps have been pivotal in opening new frontiers for the precision spectroscopy of stable ions. We report on the demonstration of an additional ion trap: the linear combined trap. This device is particularly well suited for trapping ions with unstable nuclei, due to its large range of stability parameters that facilitates external injection online to an accelerator. The motion of an ion in such a linear combined trap is investigated theoretically and experimentally. In the trap ions oscillate harmonically in the radial direction and move nearly harmonically between fixed boundaries along the longitudinal axis. The presence of a homogeneous magnetic field and the applied dc and rf electric fields, lead to a set of coupled Mathieu equations. Their approximate solutions exhibit motional frequencies, which are combinations of shifted macromotion frequencies and the cyclotron frequency. The dependence of these motional frequencies on the applied trapping fields was studied in detail. For the measurements we used small clouds of laser cooled B9e+ ions and crystallized B9e+ ions. The observed oscillation frequencies are compared to both the results of zeroth order analytical solutions and to numerical simulations in which the frequency spectrum was obtained from the ion orbits by using the fast fourier transform formalism. The various motional resonances were experimentally recorded by applying a weak dipole excitation field to one of the trap electrodes, and by simultaneously observing at resonance the changes in the fluorescence intensity. Depending on the detuning of the cooling laser the ions gain energy during the motional excitation process in such a way that they are shifted further in or out of optical resonance by the Doppler effect. This leads to either positive or negative ion motion signals at the various ion oscillation frequencies.

Journal of Applied Physics•Mar 1, 2001•11 citations

Quantum dynamics of small numbers of ions in a penning trap

G. Stutter

Laser-cooled trapped ions are one of the main systems used in experiments in the fields of quantum optics and quantum information. There are two commonly-used types of ion trap, the radiofrequency trap and the Penning trap. In general, the RF trap has been more widely used in quantum information experiments, meaning that the set of experimental tools for conducting these types of experiments in a Penning trap is currently less complete. The aim of the work presented in this thesis is to increase this array of tools. Our experiment uses 40Ca+ ions in a Penning trap alongside lasers. Spectroscopy has been performed on single Doppler cooled ions, and on ions that have been prepared close to their ground state of motion using a multiple-stage sideband cooling technique resulting in an average phonon occupation number of $\nzbar = 0.029\pm 0.011$ from an initial $\nzbar \approx 24$. This corresponds to a quantum ground state population of $97\%$, which is close to the sideband cooling limit in our system. An axial heating rate measurement of $\dot{\bar{n}}_z=\SI{0.56\pm0.52}{\per\second}$ has also been obtained, which is the lowest recorded to date, due in part to the large dimensions of our trap. Additionally improved control of the Penning trap radial motion has been demonstrated and the average phonon occupation number of the modified cyclotron motion has been reduced from $\ncbar\approx150$ after Doppler cooling to $\ncbar=0.6$ after sideband cooling. Some preliminary single-ion coherent operations have also been performed. In the future we hope that this system of ground state cooled ions in a Penning trap can be used to generate highly-entangled states in two or more ions, with a view to performing simple quantum error-correcting codes and eventually an analogue quantum simulation of spin systems.

•Nov 1, 2015•1 citation

Quantum optics with trapped and laser cooled magnesium ions

Richard Claude Thompson, David John Bate, Kishan Dholakia +2 more

We report recent experiments at Imperial College with magnesium ions confined in an ion trap and cooled by irradiation with a frequency-doubled dye laser. The work covers observation of quantum jumps in single ions in a Penning trap, measurement of oscillation frequencies in the combined trap, and a preliminary study of the spectrum of time intervals between consecutive detected photons. Theoretical considerations relevant to the experiments are also presented.

Physica Scripta•Sep 1, 1992•13 citations
This thesis describes experimental work performed on laser cooled magnesium ions, confined in a quadrupole ion trap operating in the Penning or the combined mode. Information is gained about the dynamical motion of the ions. This is done by analyzing the time delays between scattered fluorescence photons in the case of small ion clouds (generally less than ten ions). For larger clouds (upwards of 100 ions), a fraction of the ions is "tagged" and a subsequent study made of the time evolution of the fluorescence. We have developed an innovative, non-invasive method for measuring ion oscillation frequencies which is based on analyzing photon-photon correlations present in the emitted ion fluorescence. This technique has been used to measure all three Penning trap frequencies for a wide range of dc voltage. The data have been fitted to theory and we have obtained a global fit of these data to one set of trap parameters. We also demonstrate that our technique enables us to measure space-charge shifted values of the trap resonances. This method has also been applied to the combined trap and we report experimental verification of the predicted trap resonances for a wide range of trapping parameters. These data fit well to theory. This is for all three oscillation frequencies for one set of trap parameters consistent with the data for the Penning trap. \nFurther experiments are reported concerned with the dynamics of larger ion clouds in a Penning trap. A pulsed laser is used to "tag" a small number of the ions in large ion clouds. This removes those ions from the cooling cycle by placing them in a metastable state. Subsequently, we have monitored the time evolution of the fluorescence. By analyzing these data we have been able to determine cloud rotation frequencies for large ensembles of ions.
We present a method for measuring ion-oscillation frequencies in quadrupole traps (Paul, Penning, and combined traps). The method depends on a statistical analysis of the delays between detected fluorescence photons. We have used the method to verify the oscillation frequencies for magnesium ions in a Penning trap as a function of the dc voltage applied to the trap electrodes. We demonstrate that, as expected, the method measures the space-charge shifted (individual-ion) oscillation frequency and not the frequency at which the ion cloud as a whole moves. However, our data suggest that for most of our operating conditions, the space-charge shift is negligible. We also discuss the effect of the contact potential arising from areas of the trap electrodes that are coated by excess Mg from the atomic beam used. We show that this extra potential shifts the center of the Penning trap and makes it unstable for low values of the applied voltage.
We use the results of a Lagrangian formulation of the dynamics of ions in a Penning trap to calculate the motional frequencies of the ions as a function of the trapping parameters. We then add realistic perturbations to the ideal trapping fields in the formalism and deduce the effects of these perturbations on the ion motion. For an ideal trap there exist values of the applied trapping fields that result in a degeneracy in the ion oscillation frequencies associated with different types of motion. We show that this motional frequency degeneracy is lifted by the inclusion of the effect of a tilt of the trap axis with respect to the axis of the applied magnetic field, leading to an ``avoided crossing'' between the oscillation frequencies. We calculate typical ion orbits for trap parameters that give oscillation frequencies near the avoided crossing between the axial and modified cyclotron frequencies. We generalize the analysis to include the motion of ions in a combined (Penning-Paul) trap and perform an experiment to test the predictions of the theory for a degeneracy between the modified cyclotron frequency and the axial frequency for Mg+{\mathrm{Mg}}^{+}Mg+ ions held in a tilted combined trap. The oscillation frequencies are measured for a range of tilt angles using a photon-photon correlation technique. There is good agreement between the experimental results and the theoretical predictions. The method we describe may prove to be a useful means by which trap imperfections can be identified and subsequently removed.
Ion traps have been pivotal in opening new frontiers for the precision spectroscopy of stable ions. We report on the demonstration of an additional ion trap: the linear combined trap. This device is particularly well suited for trapping ions with unstable nuclei, due to its large range of stability parameters that facilitates external injection online to an accelerator. The motion of an ion in such a linear combined trap is investigated theoretically and experimentally. In the trap ions oscillate harmonically in the radial direction and move nearly harmonically between fixed boundaries along the longitudinal axis. The presence of a homogeneous magnetic field and the applied dc and rf electric fields, lead to a set of coupled Mathieu equations. Their approximate solutions exhibit motional frequencies, which are combinations of shifted macromotion frequencies and the cyclotron frequency. The dependence of these motional frequencies on the applied trapping fields was studied in detail. For the measurements we used small clouds of laser cooled B9e+ ions and crystallized B9e+ ions. The observed oscillation frequencies are compared to both the results of zeroth order analytical solutions and to numerical simulations in which the frequency spectrum was obtained from the ion orbits by using the fast fourier transform formalism. The various motional resonances were experimentally recorded by applying a weak dipole excitation field to one of the trap electrodes, and by simultaneously observing at resonance the changes in the fluorescence intensity. Depending on the detuning of the cooling laser the ions gain energy during the motional excitation process in such a way that they are shifted further in or out of optical resonance by the Doppler effect. This leads to either positive or negative ion motion signals at the various ion oscillation frequencies.
Laser-cooled trapped ions are one of the main systems used in experiments in the fields of quantum optics and quantum information. There are two commonly-used types of ion trap, the radiofrequency trap and the Penning trap. In general, the RF trap has been more widely used in quantum information experiments, meaning that the set of experimental tools for conducting these types of experiments in a Penning trap is currently less complete. The aim of the work presented in this thesis is to increase this array of tools. Our experiment uses 40Ca+ ions in a Penning trap alongside lasers. Spectroscopy has been performed on single Doppler cooled ions, and on ions that have been prepared close to their ground state of motion using a multiple-stage sideband cooling technique resulting in an average phonon occupation number of $\nzbar = 0.029\pm 0.011$ from an initial $\nzbar \approx 24$. This corresponds to a quantum ground state population of 97%97\%97%, which is close to the sideband cooling limit in our system. An axial heating rate measurement of $\dot{\bar{n}}_z=\SI{0.56\pm0.52}{\per\second}$ has also been obtained, which is the lowest recorded to date, due in part to the large dimensions of our trap. Additionally improved control of the Penning trap radial motion has been demonstrated and the average phonon occupation number of the modified cyclotron motion has been reduced from $\ncbar\approx150$ after Doppler cooling to $\ncbar=0.6$ after sideband cooling. Some preliminary single-ion coherent operations have also been performed. In the future we hope that this system of ground state cooled ions in a Penning trap can be used to generate highly-entangled states in two or more ions, with a view to performing simple quantum error-correcting codes and eventually an analogue quantum simulation of spin systems.