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Journal of Applied Physics

Ion dynamics and oscillation frequencies in a linear combined trap

T. Nakamura, S. Ohtani, M. Wada, K. Okada, Ichiro Katayama, Hans A. Schuessler

Published Mar 1, 2001• 11 citations
Publisher

Abstract

Ion traps have been pivotal in opening new frontiers for the precision spectroscopy of stable ions. We report on the demonstration of an additional ion trap: the linear combined trap. This device is particularly well suited for trapping ions with unstable nuclei, due to its large range of stability parameters that facilitates external injection online to an accelerator. The motion of an ion in such a linear combined trap is investigated theoretically and experimentally. In the trap ions oscillate harmonically in the radial direction and move nearly harmonically between fixed boundaries along the longitudinal axis. The presence of a homogeneous magnetic field and the applied dc and rf electric fields, lead to a set of coupled Mathieu equations. Their approximate solutions exhibit motional frequencies, which are combinations of shifted macromotion frequencies and the cyclotron frequency. The dependence of these motional frequencies on the applied trapping fields was studied in detail. For the measurements we used small clouds of laser cooled B9e+ ions and crystallized B9e+ ions. The observed oscillation frequencies are compared to both the results of zeroth order analytical solutions and to numerical simulations in which the frequency spectrum was obtained from the ion orbits by using the fast fourier transform formalism. The various motional resonances were experimentally recorded by applying a weak dipole excitation field to one of the trap electrodes, and by simultaneously observing at resonance the changes in the fluorescence intensity. Depending on the detuning of the cooling laser the ions gain energy during the motional excitation process in such a way that they are shifted further in or out of optical resonance by the Doppler effect. This leads to either positive or negative ion motion signals at the various ion oscillation frequencies.

DOI
10.1063/1.1345514

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Ion traps have been pivotal in opening new frontiers for the precision spectroscopy of stable ions. We report on the demonstration of an additional ion trap: the linear combined trap. This device is particularly well suited for trapping ions with unstable nuclei, due to its large range of stability parameters that facilitates external injection online to an accelerator. The motion of an ion in such a linear combined trap is investigated theoretically and experimentally. In the trap ions oscillate harmonically in the radial direction and move nearly harmonically between fixed boundaries along the longitudinal axis. The presence of a homogeneous magnetic field and the applied dc and rf electric fields, lead to a set of coupled Mathieu equations. Their approximate solutions exhibit motional frequencies, which are combinations of shifted macromotion frequencies and the cyclotron frequency. The dependence of these motional frequencies on the applied trapping fields was studied in detail. For the measurements we used small clouds of laser cooled B9e+ ions and crystallized B9e+ ions. The observed oscillation frequencies are compared to both the results of zeroth order analytical solutions and to numerical simulations in which the frequency spectrum was obtained from the ion orbits by using the fast fourier transform formalism. The various motional resonances were experimentally recorded by applying a weak dipole excitation field to one of the trap electrodes, and by simultaneously observing at resonance the changes in the fluorescence intensity. Depending on the detuning of the cooling laser the ions gain energy during the motional excitation process in such a way that they are shifted further in or out of optical resonance by the Doppler effect. This leads to either positive or negative ion motion signals at the various ion oscillation frequencies.
The parametric resonant behavior of ions inside a linear rf ion trap is studied both theoretically and experimentally. Theoretically, the resonant motion of ions inside an ideal ion trap is described by approximating the trapping rf field as a harmonic pseudopotential with the ions being excited by an additional quadrupolar ac voltage. The resulting damped Mathieu equation is studied and the regions of resonant instability are predicted by investigating the solutions. Experimentally, the parametric excitation of Mg+{\mathrm{Mg}}^{+}Mg+ ions is observed by subjecting the cloud of trapped ions to an additional quadrupolar ac field. The various ion motion resonances are detected through the disappearance of the laser-induced fluorescence signal. Weak damping is introduced by the presence of a low-pressure buffer gas. The experimental results are compared with the theoretical predictions.
This thesis describes experimental work performed on laser cooled magnesium ions, confined in a quadrupole ion trap operating in the Penning or the combined mode. Information is gained about the dynamical motion of the ions. This is done by analyzing the time delays between scattered fluorescence photons in the case of small ion clouds (generally less than ten ions). For larger clouds (upwards of 100 ions), a fraction of the ions is "tagged" and a subsequent study made of the time evolution of the fluorescence. We have developed an innovative, non-invasive method for measuring ion oscillation frequencies which is based on analyzing photon-photon correlations present in the emitted ion fluorescence. This technique has been used to measure all three Penning trap frequencies for a wide range of dc voltage. The data have been fitted to theory and we have obtained a global fit of these data to one set of trap parameters. We also demonstrate that our technique enables us to measure space-charge shifted values of the trap resonances. This method has also been applied to the combined trap and we report experimental verification of the predicted trap resonances for a wide range of trapping parameters. These data fit well to theory. This is for all three oscillation frequencies for one set of trap parameters consistent with the data for the Penning trap. \nFurther experiments are reported concerned with the dynamics of larger ion clouds in a Penning trap. A pulsed laser is used to "tag" a small number of the ions in large ion clouds. This removes those ions from the cooling cycle by placing them in a metastable state. Subsequently, we have monitored the time evolution of the fluorescence. By analyzing these data we have been able to determine cloud rotation frequencies for large ensembles of ions.
We use the results of a Lagrangian formulation of the dynamics of ions in a Penning trap to calculate the motional frequencies of the ions as a function of the trapping parameters. We then add realistic perturbations to the ideal trapping fields in the formalism and deduce the effects of these perturbations on the ion motion. For an ideal trap there exist values of the applied trapping fields that result in a degeneracy in the ion oscillation frequencies associated with different types of motion. We show that this motional frequency degeneracy is lifted by the inclusion of the effect of a tilt of the trap axis with respect to the axis of the applied magnetic field, leading to an ``avoided crossing'' between the oscillation frequencies. We calculate typical ion orbits for trap parameters that give oscillation frequencies near the avoided crossing between the axial and modified cyclotron frequencies. We generalize the analysis to include the motion of ions in a combined (Penning-Paul) trap and perform an experiment to test the predictions of the theory for a degeneracy between the modified cyclotron frequency and the axial frequency for Mg+{\mathrm{Mg}}^{+}Mg+ ions held in a tilted combined trap. The oscillation frequencies are measured for a range of tilt angles using a photon-photon correlation technique. There is good agreement between the experimental results and the theoretical predictions. The method we describe may prove to be a useful means by which trap imperfections can be identified and subsequently removed.
Single ions trapped and laser cooled provide ideal objects for high resolution spectroscopy and frequency standards. For the latter purpose we are investigating the 5s2 1S0 → 5s5p 3P0 transition of In+. With a natural linewidth of only 1.1 Hz this resonance offers very high resolution and is highly immune to frequency shifts due to external electromagnetic fields, because it connects two levels with vanishing electronic magnetic momenta [1]. The wavelength of this clock transition is 236.5 nm and is technically very convenient, since it coincides with the fourth harmonic of the 946 nm Nd:YAG laser line. So this intrinsically frequency stable solid-state laser can be used to excite the transition [2]. For laser cooling and fluorescence detection of the indium ion the 5s2 1So -> 5s5p 3P1 transition at 230.6 nm can be employed. The use of the relatively narrow intercombination line for laser cooling allows us to study optical sideband cooling in the strong binding regime, where the oscillation frequencies of the ion in the trap (around 1 MHz) are larger than the optical linewidth of 360 kHz. In this parameter range laser cooling is possible to the quantum ground state of the vibrational motion in the trap corresponding to a temperature of roughly 100 μK. The same low temperature was obtained with sideband cooling of a small Coulomb crystal consisting of two ions, creating an interesting new quantum few-particle system.
The accurate evaluation of the second-order Doppler frequency shift (SODFS) of trapped ions in a linear Paul trap has been studied with experiments and molecular dynamics (MD) simulations. The motion of trapped ions in the trap has three contributions, and we focus on the ion excess micromotion, which is rarely discussed when evaluating the SODFS of ions. Based on the hypothesis that the ion density is uniformly distributed in the radial direction, we propose a model to accurately evaluate the total SODFS for an ion ensemble with temperature less than 100 mK, which consists of three contributions of ion motion. The effectiveness of the model has been verified by MD simulation, and the experimental results of the excess micromotion of trapped ions are consistent with the theory. We believe that our model offers advantages in accurately evaluating the SODFS for the ion trap, especially those of laser-cooled ion microwave clocks based on large ion clouds.
We have studied the dynamics of one and two laser-cooled trapped 40Ca+ ions by applying electric fields of different nature along the axial direction of the trap, namely, driving the motion with a harmonic dipolar field, or with white noise. These two types of driving induce distinct motional states of the axial modes: a coherent oscillation with the dipolar field, or an enhanced Brownian motion due to an additional contribution to the heating rate from the electric noise. In both scenarios, the sensitivity of an isolated ion and a laser-cooled two-ion crystal has been evaluated and compared. The analysis and understanding of this dynamics is important towards the implementation of a novel Penning trap mass-spectroscopy technique based on optical detection, aiming at improving precision and sensitivity.