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An integrated nanoaperture optical-fiber tweezer for developing single-photon sources

Jamal M. Ehtaiba

Published Jan 1, 2020• 0 citations
OpenAlex

Abstract

In this thesis, an approach for developing single-photon sources at the 1550nm wavelength will be demonstrated, based on optical trapping of luminescent upconverting nanoparticles. A single-photon source is a source that emits a single photon at a time, and hence it is a source of quantum bits that constitutes the basic building units in quantum computers and quantum communications. The approach exploits the plasmonic properties of gold films and the waveguiding characteristics of single mode optical fibers (SMFs). We start by planar nanofabrication of subwavelength nanoapertures in a thin gold film based on finite difference time domain simulations for a peak transmission at the wavelength in question. Subsequently, using ultraviolet curable epoxy adhesion material, a nanoaperture patterned on a gold film can be transferred to an SMF tip forming a nanoantenna enhanced optical fiber tweezer (NAFT). As a final step in building the optical tweezer, a test of the capability of the integrated optical fiber tweezer to trap 20 nm, and 30nm polystyrene nanospheres, as well as luminescent upconverting nanoparticles (UCNPs), has been experimentally realized with encouraging results. In addition to the optical trapping of the luminescent nanoparticles, the nano aperture antenna can improve light coupling into the low loss optical fiber guiding channel. Also, it could have a positive influence on enhancing the photon emission rate through the Purcell effect. Furthermore, we have combined NAFT with a low insertion loss wave splitter, a wavelength-division multiplexer (WDM), to allow measuring the 1550nm photon-emission statistics on a cooled superconducting nanowire single-photon detector (SNSPD) at ~ 2.4o K. Eventually, nanoantenna enhanced optical fiber tweezers can play an essential role in optical trapping towards developing single-photon sources and the emerging technology of quantum information processing, computation, and cryptography.

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Isolating Nanocrystals with an Individual Erbium Emitter: A Route to a Stable Single-Photon Source at 1550 nm Wavelength

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Single-photon emitters based on individual atoms or individual atomic-like defects are highly sought-after components for future quantum technologies. A key challenge in this field is how to isolate just one such emitter; the best approaches still have an active emitter yield of only 50% so that deterministic integration of single active emitters is not yet possible. Here, we demonstrate the ability to isolate individual erbium emitters embedded in 20 nm nanocrystals of NaYF 4 using plasmonic aperture optical tweezers. The optical tweezers capture the nanocrystal, whereas the plasmonic aperture enhances the emission of the Er and allows the measurement of discrete emission rate values corresponding to different numbers of erbium ions. Three separate synthesis runs show near-Poissonian distribution in the discrete levels of emission yield that correspond to the expected ion concentrations, indicating that the yield of active emitters is approximately 80%. Fortunately, the trap allows for selecting the nanocrystals with only a single emitter, and so this gives a route to isolating and integrating single emitters in a deterministic way. This demonstration is a promising step toward single-photon quantum information technologies that utilize single ions in a solid-state medium, particularly because Er emits in the low-loss fiber-optic 1550 nm telecom band.

Nano Letters•Dec 31, 2019•37 citations
In this thesis, an approach for developing single-photon sources at the 1550nm wavelength will be demonstrated, based on optical trapping of luminescent upconverting nanoparticles. A single-photon source is a source that emits a single photon at a time, and hence it is a source of quantum bits that constitutes the basic building units in quantum computers and quantum communications. The approach exploits the plasmonic properties of gold films and the waveguiding characteristics of single mode optical fibers (SMFs). We start by planar nanofabrication of subwavelength nanoapertures in a thin gold film based on finite difference time domain simulations for a peak transmission at the wavelength in question. Subsequently, using ultraviolet curable epoxy adhesion material, a nanoaperture patterned on a gold film can be transferred to an SMF tip forming a nanoantenna enhanced optical fiber tweezer (NAFT). As a final step in building the optical tweezer, a test of the capability of the integrated optical fiber tweezer to trap 20 nm, and 30nm polystyrene nanospheres, as well as luminescent upconverting nanoparticles (UCNPs), has been experimentally realized with encouraging results. In addition to the optical trapping of the luminescent nanoparticles, the nano aperture antenna can improve light coupling into the low loss optical fiber guiding channel. Also, it could have a positive influence on enhancing the photon emission rate through the Purcell effect. Furthermore, we have combined NAFT with a low insertion loss wave splitter, a wavelength-division multiplexer (WDM), to allow measuring the 1550nm photon-emission statistics on a cooled superconducting nanowire single-photon detector (SNSPD) at ~ 2.4o K. Eventually, nanoantenna enhanced optical fiber tweezers can play an essential role in optical trapping towards developing single-photon sources and the emerging technology of quantum information processing, computation, and cryptography.
Single photon sources are desired for quantum computing and communication applications. Ideally, these sources would provide single photons on demand at the low-loss fiber optical communication wavelength of 1550 nm. Single Erbium ions provide a good candidate for such sources because they emit at the right wavelength and they are very stable, however, the challenges remain of isolating a single emitter, coupling its emission to optical fiber and enhancing its emission rate. Nanoaperture optical tweezers provide a pathway to solving these issues by trapping and identifying single emitters, enhancing their emission rate and providing efficient coupling to an optical fiber. Recently, we have made progress in each of these areas (trapping, enhancing and coupling), which will be reviewed in this talk.
Single-photon sources are required for quantum technologies and can be created from individual atoms and atom-like defects. Erbium ions produce single photons at low-loss fiber optic wavelengths, but they have low emission rates, making them challenging to isolate reliably. Here, we tune the size of gold double nanoholes (DNHs) to enhance the emission of single erbium emitters, achieving 50× enhancement over rectangular apertures previously demonstrated. This produces enough enhancement to show emission from single nanocrystals at wavelengths not seen in our previous work, i.e., 400 and 1550 nm. We observe discrete levels of emission for nanocrystals with low numbers of emitters and demonstrate isolating single emitters. We describe how the trapping time is proportional to the enhancement factor for a given DNH structure, giving us an independent way to measure the enhancement. This shows a promising path to achieving single emitter sources at 1550 nm.
This dissertation explores the integration and interfacing of a variety of photonic devices with optical waveguides, aiming to minimize the optical losses and physical footprint of such systems. The specific investigations include interfacing solid-core and hollow-core optical fibers, development of a monolithic single-photon source based on a quantum dot embedded in a semiconductor nanowire aligned with a single-mode fiber, a proposal for a waveguide-integrated power limiter that can protect detectors in a quantum key distribution (QKD) network, and integrating superconducting-nanowire single photon detectors (SNSPD) with laser-written waveguides. \n \nHollow-core photonic-crystal fibers (HCPCFs), which can allow simultaneous tight confinement of both photons and atoms in their hollow core, offer a platform for enhancing interactions between light and atomic ensembles. However, interfacing HCPCFs with conventional solid core (SC) fibers presents a unique set of challenges including significant losses in the joint region due to partial melting and deformation of the photonic crystal during the conventional arc-fusion splicing process. We address this issue with a lithographically defined, vacuum-compatible on-chip structure acting as a mechanical splicer that allows efficient injection of light from a SC fiber to a HCPCF and vice versa, with maximum observed light injection efficiency from a single-mode SC fiber into a HCPCF of 90%. \n \nSingle photon sources (SPS) are often required in photonic quantum information applications. Among various candidates, quantum dots (QD) embedded in tapered semiconductor nanowires have demonstrated excellent progress so far to realize a SPS. However, the overall collection efficiency of the emitted photon into a single mode fiber remains as one of the major challenges, mainly due to loss in the intermediate optical components. We design a complete scheme for high efficiency light coupling from such quantum dot to a single mode fiber. We optimize the geometry of the tapered nanowire to achieve a low numerical aperture Gaussian output mode profile from the wire tip and use a lithographically defined structure to align the SMF collecting the emitted photons. A graded-index multimode fiber acting as a lens is spliced on the SMF end for high efficiency coupling of light from the nanowire into the fiber. \n \nExtremely sensitive photonic devices are often used in quantum optics applications for detection and manipulation of signals with very low power. To prevent malfunction or even damage to these sensitive devices by excess incident power, we propose an optical power limiter based on a pair of cavities integrated with optical waveguides. Such power limiter can be used to protect sensitive electro-optical devices and prevent certain types of attacks on QKD systems. \n \nLastly, a 2D photonic lattice formed by laser-written waveguides in bulk glass can be used as an analogue quantum simulator. We explore the integration of SNSPDs with laser-written waveguides with the goal of making this platform fully on-chip.
Optical nano-antennae have been integrated with semiconductor lasers to intensify light at the nanoscale and photodiodes to enhance photocurrent. In quantum optics, plasmonic metal structures have been used to enhance nonclassical light emission from single quantum dots. Absorption and detection of single photons from free space could also be enhanced by nanometallic antennae, but this has not previously been demonstrated. Here, we use nano-optical transmission effects in a one-dimensional gold structure, combined with optical cavity resonance, to form optical nano-antennae, which are further used to couple single photons from free space into a 80-nm-wide superconducting nanowire. This antenna-assisted coupling enables a superconducting nanowire single-photon detector with 47% device efficiency at the wavelength of 1550 nm and 9-μm-by-9-μm active area while maintaining a reset time of only 5 ns. We demonstrate nanoscale antenna-like structures to achieve exceptional efficiency and speed in single-photon detection.
The physics of single photons is fascinating, by manipulating them we can observe and probe quantum effects. Doing so requires the fabrication and utilization of single photon sources, of which many types have been developed including quantum dots, trapped atoms and ions, and color centers. On the other end of the experiments, single photon detectors play a role of utmost importance, and while several types of detectors exist, superconducting nanowire single photon detectors are now the state-of-the-art technology. By offering near unity detection efficiency from the ultra-violet to the mid-infrared light spectrum, with negligible noise and excellent time resolution, they made possible many experiments that were previously technologically unfeasible. The same appealing characteristics have found a use in applications outside of the quantum optics framework, with notably light detection and ranging, biomedical imaging or CMOS circuits testing.In this thesis a controlled growth method for tailoring the characteristics of niobium titanium nitride in the framework of superconducting nanowire single photon detectors was developed. Reactive co-sputter deposition of niobium titanium nitride was shown to be a versatile method, both in terms of the degree of control over the material composition, and in the choice of substrates that it allows. Unity internal detection efficiency of detectors at telecom wavelengths was achieved by optimizing the niobium content in the material. The influence of lattice matching on the critical temperatures of films deposited at room temperature was investigated. The fabrication of superconducting nanowire single photon detectors on aluminum nitride-on-sapphire, on lithium niobate nano-waveguides, on gallium arsenide, and the integration on SiN waveguides was achieved. The material was used to fabricate detectors with optimized response for any linear polarization of the incoming photons by using a fractal architecture. Another method was proposed to achieve the same results by encapsulating meandering detectors in a high index dielectric material, resulting in a decrease of the permittivity mismatch between the nanowire material and its surrounding and therefore optimizing the efficiency for both orthogonal linear polarizations.Finally, detectors were fabricated from films developed in this work, and were operated to enable the implementation of polarization-based entanglement distribution in optical fibers in a real-conditions scenario, over a record distance of 96 km. This paves the way for the development of quantum communication networks using existing optical fiber links.
Single-photon emitters based on individual atoms or individual atomic-like defects are highly sought-after components for future quantum technologies. A key challenge in this field is how to isolate just one such emitter; the best approaches still have an active emitter yield of only 50% so that deterministic integration of single active emitters is not yet possible. Here, we demonstrate the ability to isolate individual erbium emitters embedded in 20 nm nanocrystals of NaYF 4 using plasmonic aperture optical tweezers. The optical tweezers capture the nanocrystal, whereas the plasmonic aperture enhances the emission of the Er and allows the measurement of discrete emission rate values corresponding to different numbers of erbium ions. Three separate synthesis runs show near-Poissonian distribution in the discrete levels of emission yield that correspond to the expected ion concentrations, indicating that the yield of active emitters is approximately 80%. Fortunately, the trap allows for selecting the nanocrystals with only a single emitter, and so this gives a route to isolating and integrating single emitters in a deterministic way. This demonstration is a promising step toward single-photon quantum information technologies that utilize single ions in a solid-state medium, particularly because Er emits in the low-loss fiber-optic 1550 nm telecom band.