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Analyzing photon-counting based entanglement generation between solid-state spin qubits by unraveling the master equation

Stephen C. Wein, Jia-Wei Ji, Yu-Feng Wu, Faezeh Kimiaee Asadi, Roohollah Ghobadi, Christoph Simon

Published Apr 9, 2020• 0 citations
OpenAlex

Abstract

We analyze and compare three different schemes that can be used to generate entanglement between spin qubits in optically-active single solid-state quantum systems. Each scheme is based on first generating entanglement between the spin degree of freedom and either the photon number, the time bin, or the polarization degree of freedom of photons emitted by the systems. We compute the time dynamics of the entanglement generation process by unraveling a Markovian master equation into a set of propagation superoperators conditioned on the cumulative detector photocount. We then use the conditional density operator solutions to compute the efficiency and fidelity of the final spin-spin entangled state while accounting for spin decoherence, optical pure dephasing, spectral diffusion, photon loss, detector dark counts, and detector photon number resolution limitations. We find that the limit to fidelity for each scheme is restricted by the mean wavepacket overlap of photons from each source, but that these bounds are different for each scheme. We also compare the performance of each scheme as a function of the distance between spin qubits.

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We analyze and compare three different schemes that can be used to generate entanglement between spin qubits in optically-active single solid-state quantum systems. Each scheme is based on first generating entanglement between the spin degree of freedom and either the photon number, the time bin, or the polarization degree of freedom of photons emitted by the systems. We compute the time dynamics of the entanglement generation process by unraveling a Markovian master equation into a set of propagation superoperators conditioned on the cumulative detector photocount. We then use the conditional density operator solutions to compute the efficiency and fidelity of the final spin-spin entangled state while accounting for spin decoherence, optical pure dephasing, spectral diffusion, photon loss, detector dark counts, and detector photon number resolution limitations. We find that the limit to fidelity for each scheme is restricted by the mean wavepacket overlap of photons from each source, but that these bounds are different for each scheme. We also compare the performance of each scheme as a function of the distance between spin qubits.
We analyze and compare three different schemes that can be used to generate entanglement between spin qubits in optically active single solid-state quantum systems. Each scheme is based on first generating entanglement between the spin degree of freedom and the photon number, the time bin, or the polarization degree of freedom of photons emitted by the systems. We compute the time evolution of the entanglement generation process by decomposing the dynamics of a Markovian master equation into a set of propagation superoperators conditioned on the cumulative detector photon count. We then use the conditional density operator solutions to compute the efficiency and fidelity of the final spin-spin--entangled state while accounting for spin decoherence, optical pure dephasing, spectral diffusion, photon loss, phase errors, detector dark counts, and detector photon number resolution limitations. We find that the limit to fidelity for each scheme is restricted by the mean wave-packet overlap of photons from each source but that these bounds are different for each scheme. We also compare the performance of each scheme as a function of the distance between spin qubits.
Solid-state quantum emitters, such as quantum dots, color centers, rare-earth dopants, and organic molecules, offer qubit systems that integrate well with chip-scale photonic and electronic devices. To fully harness their potential for quantum applications requires the generation of entanglement between two remote qubits with high fidelity and efficiency. In this article, we compare the performance of three common photon-mediated entanglement schemes under realistic noise for solid-state quantum emitters, including optical dephasing and spectral diffusion. We identify the optimal scheme across different noise regimes and calculate the measurement parameters needed to achieve the highest entanglement fidelity at a given rate. Additionally, we explore the effects of temporal and spectral filtering in enhancing entanglement fidelity. Our findings provide practical guidelines for selecting optimal entanglement schemes and outline the measurement strategies for achieving better entanglement fidelity.
The desire to understand the interaction between light and matter has stimulated centuries of research, leading to technological achievements that have shaped our world. One contemporary frontier of research into light-matter interaction considers regimes where quantum effects dominate. By understanding and manipulating these quantum effects, a vast array of new quantum-enhanced technologies become accessible. In this thesis, I explore and analyze fundamental components and processes for quantum optical devices with a focus on solid-state quantum systems. This includes indistinguishable single-photon sources, deterministic sources of entangled photonic states, photon-heralded entanglement generation between remote quantum systems, and deterministic optically-mediated entangling gates between local quantum systems. For this analysis, I make heavy use of an analytic quantum trajectories approach applied to a general Markovian master equation of an optically-active quantum system, which I introduce as a photon-number decomposition. This approach allows for many realistic system imperfections, such as emitter pure dephasing, spin decoherence, and measurement imperfections, to be taken into account in a straightforward and comprehensive way.
Self-assembled quantum dots can act as an interface between single spins and photons. They combine the flexibility and scalability of semiconductor systems with near-perfect two level systems, emitting highly coherent single photons. In potential quantum information processing architectures based upon optical networks, quantum dots permit light-matter coupling between matter qubits and photonic links. Single trapped charge carriers in quantum dots can be addressed optically, generating spin-photon entanglement between the matter qubits and \lq flying' photon qubits, a key first step in creation of a network. Such an optically linked network of spins in quantum dots has yet to be realized. The semiconductor environment presents a key challenge; it broadens the spectrum of the emitted light, which reduces the fidelity of schemes based upon photon exchange or interference. In addition, these quantum dots are subject to hyperfine coupling to a bath of >>> 105^{5}5 nuclear spins. While this presents an opportunity to study the physics of a central spin in a spin bath, it degrades the spin coherence of a trapped electron or hole. The suggested gate operations to generate entanglement, and the spin measurements to verify a created state, rely upon photon detection. Thus a second limitation occurs due to low efficiency of detectors and photon collection probability. Recent developments in detector technology have enabled us to bring generation and verification of entangled states with quantum dots into the realm of possibility. This dissertation begins with a detailed study of the interaction of a single electron spin with the solid state environment of the quantum dot, analysing the intensity noise of scattered light under resonant excitation to uncover the timescales and relative amplitudes of identified noise sources. A technique for rapid characterization of samples is presented, focusing in particular upon comparison of spectral broadening of the optical transitions relevant to a spin-photon interface. Having identified the extent of environmental factors acting upon the quantum dots, we turn to a demonstration of photon-mediated entanglement between two distant electron spins using a probabilistic scheme. We are able to generate entangled states at 7 kHz, the fastest yet reported for photon-mediated protocols. The average state fidelity of the created Bell states is 63.5 ±\pm± 3.0 \%., violating the classical limit by over 4 standard deviations of the mean. In addition, we demonstrate full optical phase tuning of the Bell state ∣Ψ=12(∣↑∣↓+eiϕ∣↓∣↑)|{\Psi} = \frac{1}{\sqrt{2}}\left(|{\uparrow}|{\downarrow} + e^{i\phi}|{\downarrow}|{\uparrow} \right)∣Ψ=2​1​(∣↑∣↓+eiϕ∣↓∣↑). This is a proof of principle experiment, and sets a fidelity benchmark upon which gains can be made by mitigation of environmental dynamics.
Efficient generation of entanglement between a stationary matter-qubit and a propagating photonic-qubit is a scientific and technological challenge of utmost importance for the realisation of fully-fledged quantum networks. Solid-state quantum emitters in the telecom C-band are a promising platform due to the minimal absorption of photons at these wavelengths and deterministic generation of high purity single photon flying qubits. Here, we use an InAs/InP quantum dot to implement an optically active spin-qubit and demonstrate high fidelity spin initialisation and coherent spin control of the resident electron. Lastly, for the first time we demonstrate high-fidelity spin-photon entanglement in a solid-state system with direct emission into the telecom C-band and obtain a lower bound on the entanglement fidelity of 80.07 %.
Entanglement between light and matter combines the advantage of long distance transmission of photonic qubits with the storage and processing capabilities of atomic qubits. To distribute photonic states efficiently over long distances several schemes to encode qubits have been investigated-time-bin encoding being particularly promising due to its robustness against decoherence in optical fibers. Here, we demonstrate the generation of entanglement between a photonic time-bin qubit and a single collective atomic spin excitation (spin wave) in a cold atomic ensemble, followed by the mapping of the atomic qubit onto another photonic qubit. A magnetic field that induces a periodic dephasing and rephasing of the atomic excitation ensures the temporal distinguishability of the two time bins and plays a central role in the entanglement generation. To analyze the generated quantum state, we use largely imbalanced Mach-Zehnder interferometers to perform projective measurements in different qubit bases and verify the entanglement by violating a Clauser-Horne-Shimony-Holt Bell inequality.