Due to their capacity for non-classical light generation, high-efficiency second-order nonlinear parametric processes play an important role in quantum photonic technology, and chip-scale realization of these processes is recognized as the key to building efficient light sources for integrated quantum photonic circuits. To achieve ultra-high nonlinear conversion efficiency, traditional method uses quasi-phase matching (QPM) technology. However, QPM requires electric field poling, which is incompatible with the CMOS fabrication process, and this hinders the wafer-scale production of integrated photonic circuits. In this paper, we demonstrate efficient spontaneous quasi-phase matched (SQPM) frequency conversion in a micro-racetrack resonator. Our approach does not involve poling, but exploits the anisotropy of the ferroelectric crystals to allow the phase-matching condition to be fulfilled spontaneously as the TE-polarized light circulates in a specifically designed racetrack resonator. SQPM second harmonic generation is observed with a normalized intracavity conversion efficiency of 0.85%/W, corresponding to the 111st-order QPM. This could theoretically reach 186,000%/W by first-order QPM. In this case such high intracavity conversion efficiency can be implemented in practice with an optimized outward coupling. Our configurable SQPM approach will benefit the application of nonlinear frequency conversion in chip-scale integrated photonics with CMOS-compatible fabrication processes, and is applicable to other on-chip nonlinear processes such as quantum frequency conversion or frequency-comb generation.
Abstract It is shown that cascaded nonlinear optical frequency conversion over an intermediate wavelength, subjected to dissipation, behaves similarly to population transfer via a decaying state in a three-state non-Hermitian quantum system. The intermediate dissipation leads to a fixed phase relationship between the input signal wave and the wave at the target frequency, what finally stabilizes both waves preventing any spatial oscillation of their powers. The cascaded conversion acts as a stable wave splitter between the input and target waves, the latter being nearly immune to power fluctuations of the pumps. A case of a simultaneous cascade of the sum frequency generation and the difference frequency generation processes is discussed as an example. A possible implementation, based on aperiodically engineered quasi-phase-matching in lithium niobate, is proposed.
Efficient generation of entangled photons typically relies on spontaneous parametric down-conversion (SPDC) in phase-matched macroscopic nonlinear media. However, generating entanglement under phase-matching constraints requires additional bulk optics or interferometers. In contrast, ultrathin van der Waals semiconductors - such as transition metal dichalcogenides (TMDs) - exhibit strong enough optical nonlinearities for SPDC to be observed from subwavelength-thick media, thereby bypassing conventional phase-matching constraints. In this microscopic domain, the intrinsic crystal symmetry governs the nonlinear optical response, enabling the native generation of polarization-entangled photon pairs. However, generating these states efficiently has been fundamentally restricted by the material's coherence length (
Lc), which limits the attainable conversion efficiency. Here, we investigate periodically-poled TMDs (PPTMDs) designed to scale up this interaction via quasi-phase matching. We demonstrate that mechanically flipping the sign of the nonlinearity at precise intervals of
Lc introduces quasi-phase matching, that scales the pair-production rate while preserving the pristine, symmetry-generated polarization entanglement, with fidelities exceeding 99%. Backed by a rigorous theoretical model, our work clarifies the interplay between crystal symmetry and propagation effects in thin nonlinear media, providing a new avenue for engineering quantum light in nanophotonic systems.