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arXiv:2106.13464

Chip-scale Spontaneous Quasi-Phase-Matched Micro-Racetrack Resonator

Tingge Yuan, Yian Liu, Xiongshuo Yan, Haowei Jiang, Hao Li, Ge, Rui, Yuping Chen, Xianfeng Chen, Qiang Lin

Published Jun 25, 2021• 0 citations
arXivHTMLPDF

Abstract

Due to their capacity for non-classical light generation, high-efficiency second-order nonlinear parametric processes play an important role in quantum photonic technology, and chip-scale realization of these processes is recognized as the key to building efficient light sources for integrated quantum photonic circuits. To achieve ultra-high nonlinear conversion efficiency, traditional method uses quasi-phase matching (QPM) technology. However, QPM requires electric field poling, which is incompatible with the CMOS fabrication process, and this hinders the wafer-scale production of integrated photonic circuits. In this paper, we demonstrate efficient spontaneous quasi-phase matched (SQPM) frequency conversion in a micro-racetrack resonator. Our approach does not involve poling, but exploits the anisotropy of the ferroelectric crystals to allow the phase-matching condition to be fulfilled spontaneously as the TE-polarized light circulates in a specifically designed racetrack resonator. SQPM second harmonic generation is observed with a normalized intracavity conversion efficiency of 0.85%/W, corresponding to the 111st-order QPM. This could theoretically reach 186,000%/W by first-order QPM. In this case such high intracavity conversion efficiency can be implemented in practice with an optimized outward coupling. Our configurable SQPM approach will benefit the application of nonlinear frequency conversion in chip-scale integrated photonics with CMOS-compatible fabrication processes, and is applicable to other on-chip nonlinear processes such as quantum frequency conversion or frequency-comb generation.

DOI
10.48550/arxiv.2106.13464

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Due to their capacity for non-classical light generation, high-efficiency second-order nonlinear parametric processes play an important role in quantum photonic technology, and chip-scale realization of these processes is recognized as the key to building efficient light sources for integrated quantum photonic circuits. To achieve ultra-high nonlinear conversion efficiency, traditional method uses quasi-phase matching (QPM) technology. However, QPM requires electric field poling, which is incompatible with the CMOS fabrication process, and this hinders the wafer-scale production of integrated photonic circuits. In this paper, we demonstrate efficient spontaneous quasi-phase matched (SQPM) frequency conversion in a micro-racetrack resonator. Our approach does not involve poling, but exploits the anisotropy of the ferroelectric crystals to allow the phase-matching condition to be fulfilled spontaneously as the TE-polarized light circulates in a specifically designed racetrack resonator. SQPM second harmonic generation is observed with a normalized intracavity conversion efficiency of 0.85%/W, corresponding to the 111st-order QPM. This could theoretically reach 186,000%/W by first-order QPM. In this case such high intracavity conversion efficiency can be implemented in practice with an optimized outward coupling. Our configurable SQPM approach will benefit the application of nonlinear frequency conversion in chip-scale integrated photonics with CMOS-compatible fabrication processes, and is applicable to other on-chip nonlinear processes such as quantum frequency conversion or frequency-comb generation.
Spontaneous parametric down-conversion (SPDC) has been utilized in generating non-classical light, such as correlated photon pairs and squeezed light, significantly influencing optical quantum information research. Advances in thinfilm lithium niobate (TFLN) technologies have brought the benefits of χ(2)nonlinearity from bulk optics to integrated photonics. Targeting fully exploitation of high Electro-optic (EO) controllability and the periodic poled lithium niobate (PPLN), enabling quasi-phase matching (QPM), offer the realization especially under the X-cut based platform [1]–[3]. Moreover, the small footprint is also key figure of merit for efficient processing of SPDC spectrum. In this work, we demonstrate SPDC photon pair generation in a small footprint size with a 0.614 nm FSR at the IR wavelength, based on X-cut PPLN racetrack resonator.
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On-chip quantum information network requires qubit transfer between different wavelengths while preserving quantum coherence and entanglement, which needs broadband up-conversion available. Herein, we demonstrate a mode-hybridization based broadband nonlinear frequency conversion on X-cut thin film lithium niobate. With the spontaneous quasi-phase matching and quasi groupvelocity matching being simultaneously satisfied, broadband second harmonic generation with a 3-dB bandwidth up to 13 nm has been achieved in a micro-racetrack resonator. The same mechanism can work on the frequency conversion of the ultra-short pulse in the bent waveguide structure. This work will be beneficial to on-chip tunable frequency conversion and quantum light source generation on integrated photonic platforms, and further enable on-chip large-capacity multiplexing, multichannel optical information processing, and large quantum information networks.
Thanks to its high quadratic nonlinear susceptibilty and low propagation losses, thin film lithium niobate (TFLN) on insulator is an ideal platform for laser frequency conversion and generation of quantum states of light. Frequency conversion is usually achieved by quasi-phase matching (QPM) via electric-field poling. However, this scheme shows very high sensitivity to the dimensions of the waveguide, poling period and duty cycle, resulting in a lack of repeatability of the phase matched wavelength and efficiency, which in turn limits the spread of TFLN frequency converters in complex circuits and hinders wafer-scale production. Here we propose a layer-poled modal phase matching (MPM) that is 5 to 10 times more robust towards fabrication uncertainties and theoretically more efficient than conventional QPM. By selectively poling the bottom part of the waveguide all along its length, second harmonic is efficiently generated on a higher order waveguide's mode. We validate this approach by poling TFLN waveguides as a post-process after the fabrication in a foundry process. We perform a tolerance analysis and compare the experimental results with conventional QPM second harmonic generation process on the same waveguides. Then, we show how MPM can be exploited to obtain efficient intraband frequency conversion processes at telecom wavelengths by leveraging simultaneous second harmonic and difference frequency generation in the same waveguide.
The integration of second-order optical nonlinearities into scalable photonic platforms remains a key challenge due to their large sensitivity to fabrication variations. Here, we present a scalable quadratic nonlinear platform that harnesses the maturity and scalability of existing CMOS processes by heterogeneously integrating periodically poled lithium niobate (PPLN) onto a silicon photonics platform. A generic PPLN design enables frequency conversion on two distinct waveguide geometries with efficiencies comparable to LNOI rib waveguides. We achieve reproducible phase-matching across the full radius of a commercial 200 mm silicon photonics wafer, leveraging superior CMOS fabrication tolerances. Furthermore, we introduce a tuning mechanism for both blue- and red-shifting of the operating wavelength, fully compensating fabrication-induced offsets. This enables deterministic phase-matching over an entire wafer and yields a strategy for wafer-scale phase-matched quadratic nonlinearities. Finally, we realize printable photon-pair sources via spontaneous parametric down-conversion, highlighting the platform's potential for large-scale quantum optical circuits. These results pave the way for wafer-scale integration of second-order optical nonlinearities in large photonic systems.
Abstract Integrated photon-pair sources are crucial for scalable photonic quantum systems. Thin-film lithium niobate is a promising platform for on-chip photon-pair generation through spontaneous parametric down-conversion (SPDC). However, the device implementation faces practical challenges. Periodically poled lithium niobate (PPLN), despite enabling flexible quasi-phase matching, suffers from poor fabrication reliability and device repeatability, while conventional modal phase matching (MPM) methods yield limited efficiencies due to inadequate mode overlaps. Here, we introduce a layer-poled lithium niobate (LPLN) nanophotonic waveguide for efficient photon-pair generation. It leverages layer-wise polarity inversion through electrical poling to break spatial symmetry and significantly enhance nonlinear interactions for MPM, achieving a notable normalized second-harmonic generation (SHG) conversion efficiency of 4615% W-1 cm-2. Through a cascaded SHG and SPDC process, we demonstrate photon-pair generation with a normalized brightness of 3.1×106 Hz nm-1 mW-2 in a 3.3 mm long LPLN waveguide, surpassing existing on-chip sources under similar operating configurations. Crucially, our LPLN waveguides offer enhanced fabrication reliability and reduced sensitivity to geometric variations and temperature fluctuations compared to PPLN devices. We expect LPLN to become a promising solution for on-chip nonlinear wavelength conversion and non-classical light generation, with immediate applications in quantum communication, networking, and on-chip photonic quantum information processing.