In the interaction between a quantum mechanical electron wave and a wall, loss of interference contrast is observed. It is of general interest to identify the mechanism and categorize its nature as dephasing or decoherence. Decoherence is of fundamental importance for the transition between the classical and quantum boundary, while dephasing is often an experimental detriment that needs to be understood and overcome. We find that the loss of contrast is attributed to a local charge distribution induced by secondary emission: a dephasing mechanism. This mechanism is expected to be present for many materials, is clearly visible for copper oxide, and can mask decoherence mechanisms. The local charge distribution on the wall causes a loss of contrast and electron beam deformation. A model based on Coulomb interaction with the surface charge gives good agreement for both features. Our model can thus be used to improve the experimental design and lead to separate out decoherence phenomena in the electron-wall system.
In the interaction between a quantum mechanical electron wave and a wall, loss of interference contrast is observed. It is of general interest to identify the mechanism and categorize its nature as dephasing or decoherence. Decoherence is of fundamental importance for the transition between the classical and quantum boundary, while dephasing is often an experimental detriment that needs to be understood and overcome. We find that the loss of contrast is attributed to a local charge distribution induced by secondary emission: a dephasing mechanism. This mechanism is expected to be present for many materials, is clearly visible for copper oxide, and can mask decoherence mechanisms. The local charge distribution on the wall causes a loss of contrast and electron beam deformation. A model based on Coulomb interaction with the surface charge gives good agreement for both features. Our model can thus be used to improve the experimental design and lead to separate out decoherence phenomena in the electron-wall system.
Abstract The performance of modern quantum devices in communication, metrology or microscopy relies on the quantum–classical interaction which is generally described by the theory of decoherence. Despite the high relevance for long coherence times in quantum electronics, decoherence mechanisms mediated by the Coulomb force are not well understood yet and several competing theoretical models exist. Here, we present an experimental study of the Coulomb-induced decoherence of free electrons in a superposition state in a biprism electron interferometer close to a semiconducting and metallic surface. The decoherence was determined through a contrast loss at different beam path separations, surface distances and conductibilities. To clarify the current literature discussion, four theoretical models were compared to our data. We could rule out three of them and got good agreement with a theory based on macroscopic quantum electrodynamics. The results will enable the determination and minimization of specific decoherence channels in the design of novel quantum instruments.
Quantum theory is often cited as being one of the most empirically validated theories in terms of its predictive power and precision. These attributes have led to numerous scientific discoveries and technological advancements. However, the precise relationship between quantum and classical physics remains obscure. The prevailing description is known as decoherence theory, where classical physics emerges from a more general quantum theory through environmental interaction. Sometimes referred to as the decoherence program, it does not solve the quantum measurement problem. We believe experiments performed between the microscopic and macroscopic world may help finish the program. The following considers a free electron that interacts with a surface (the environment), providing a controlled decoherence mechanism. There are non-decohering interactions to be examined and quantified before the weaker decohering effects are filtered out. In the first experiment, an electron beam passes over a surface that’s illuminated by low-power laser light. This induces a surface charge redistribution causing the electron deflection. This phenomenon’s parameters are investigated. This system can be well understood in terms of classical electrodynamics, A second experiment tests decoherence theory by introducing a nanofabricated diffraction grating before the surface. The electron undergoes diffraction through the grating, but as the electron passes over the surface it’s predicted by various physical models that the electron will lose its wave interference property. Image charge based models, which predict a larger loss of contrast than what is observed, are falsified (despite experiencing an image charge force). A theoretical study demonstrates how a loss of contrast may not be due to the irreversible process decoherence, but dephasing (a reversible process due to randomization of the wavefunction’s phase). To resolve this ambiguity, a correlation function on an ensemble of diffraction patterns is analyzed after an electron undergoes either process in a path integral calculation. The diffraction pattern is successfully recovered for dephasing, but not for decoherence, thus verifying it as a potential tool in experimental studies to determine the nature of the observed process.
We review different attempts to show the decoherence process in double-slit-like experiments both for charged particles (electrons) and for neutral particles with permanent dipole moments. Interference is studied when electrons or atomic systems are coupled to classical or quantum electromagnetic fields. The interaction between the particles and time-dependent fields induces a time-varying Aharonov phase. Averaging over the phase generates a suppression of fringe visibility in the interference pattern. We show that, for suitable experimental conditions, the loss of contrast for dipoles can be almost as large as the corresponding one for coherent electrons and therefore can be observed. We analyse different trajectories in order to show the dependence of the decoherence factor on the velocity of the particles.
An experiment in which decoherence, i.e. the transition from quantum to classical behaviour, can be studied in detail was proposed by Anglin and Zurek [1] and has now been realized. An electron beam in a biprism interferometer is split into two parts both of which travel over a plate made of a highly resistive material at the same, small height. The induced charges inside the plate move along with the beam electron, therefore a current results which encounters ohmic resistance. This process leads to a disturbance in the electron and phonon gas in the plate. As this disturbance is different for the two parts of the beam, entanglement between beam electron and plate is formed. The strength of decoherence, represented by the visibility of the interference fringes, varies as a function of two parameters, the height above the plate and the lateral separation of the beams. Allowing electrons of different height to reach the fluorescent screen successively, 'photos' of the quantum-classical border (continuous decrease of contrast with decreasing height above the plate) are built up.
Surface plasma waves arise from the collective oscillations of billions of electrons at the surface of a metal in unison. The simplest way to quantize these waves is by direct analogy to electromagnetic fields in free space, with the surface plasmon, the quantum of the surface plasma wave, playing the same role as the photon. It follows that surface plasmons should exhibit all of the same quantum phenomena that photons do, including quantum interference and entanglement. Unlike photons, however, surface plasmons suffer strong losses that arise from the scattering of free electrons from other electrons, phonons, and surfaces. Under some circumstances, these interactions might also cause “pure dephasing,” which entails a loss of coherence without absorption. Quantum descriptions of plasmons usually do not account for these effects explicitly, and sometimes ignore them altogether. In light of this extra microscopic complexity, it is necessary for experiments to test quantum models of surface plasmons. In this thesis, I describe two such tests that my collaborators and I performed. The first was a plasmonic version of the Hong-Ou-Mandel experiment, in which we observed two-particle quantum interference between plasmons with a visibility of 93 ± 1%. This measurement confirms that surface plasmons faithfully reproduce this effect with the same visibility and mutual coherence time, to within measurement error, as in the photonic case. The second experiment demonstrated path entanglement between surface plasmons with a visibility of 95 ± 2%, confirming that a path-entangled state can indeed survive without measurable decoherence. This measurement suggests that elastic scattering mechanisms of the type that might cause pure dephasing must have been weak enough not to significantly perturb the state of the metal under the experimental conditions we investigated. These two experiments add quantum interference and path entanglement to a growing list of quantum phenomena that surface plasmons appear to exhibit just as clearly as photons, confirming the predictions of the simplest quantum models.
Controlled decoherence of free electrons due to Coulomb interaction with a truly macroscopic environment, the electron (and phonon) gas inside a semiconducting plate, is studied experimentally. The quantitative results are compared with different theoretical models. The experiment confirms the main features of the theory of decoherence and can be interpreted in terms of which-path information. In contrast to previous model experiments on decoherence, the obtained interferograms directly visualize the transition from quantum to classical.