Controlled decoherence of free electrons due to Coulomb interaction with a truly macroscopic environment, the electron (and phonon) gas inside a semiconducting plate, is studied experimentally. The quantitative results are compared with different theoretical models. The experiment confirms the main features of the theory of decoherence and can be interpreted in terms of which-path information. In contrast to previous model experiments on decoherence, the obtained interferograms directly visualize the transition from quantum to classical.
Controlled decoherence of free electrons due to Coulomb interaction with a truly macroscopic environment, the electron (and phonon) gas inside a semiconducting plate, is studied experimentally. The quantitative results are compared with different theoretical models. The experiment confirms the main features of the theory of decoherence and can be interpreted in terms of which-path information. In contrast to previous model experiments on decoherence, the obtained interferograms directly visualize the transition from quantum to classical.
A controlled decoherence environment is studied experimentally by free electron interaction with semiconducting and metallic plates. The results are compared with physical models based on decoherence theory to investigate the quantum-classical transition. The experiment is consistent with decoherence theory and rules out established Coulomb interaction models in favor of plasmonic excitation models. In contrast to previous decoherence experiments, the present experiment is sensitive to the onset of decoherence.
Abstract The performance of modern quantum devices in communication, metrology or microscopy relies on the quantum–classical interaction which is generally described by the theory of decoherence. Despite the high relevance for long coherence times in quantum electronics, decoherence mechanisms mediated by the Coulomb force are not well understood yet and several competing theoretical models exist. Here, we present an experimental study of the Coulomb-induced decoherence of free electrons in a superposition state in a biprism electron interferometer close to a semiconducting and metallic surface. The decoherence was determined through a contrast loss at different beam path separations, surface distances and conductibilities. To clarify the current literature discussion, four theoretical models were compared to our data. We could rule out three of them and got good agreement with a theory based on macroscopic quantum electrodynamics. The results will enable the determination and minimization of specific decoherence channels in the design of novel quantum instruments.
An experiment in which decoherence, i.e. the transition from quantum to classical behaviour, can be studied in detail was proposed by Anglin and Zurek [1] and has now been realized. An electron beam in a biprism interferometer is split into two parts both of which travel over a plate made of a highly resistive material at the same, small height. The induced charges inside the plate move along with the beam electron, therefore a current results which encounters ohmic resistance. This process leads to a disturbance in the electron and phonon gas in the plate. As this disturbance is different for the two parts of the beam, entanglement between beam electron and plate is formed. The strength of decoherence, represented by the visibility of the interference fringes, varies as a function of two parameters, the height above the plate and the lateral separation of the beams. Allowing electrons of different height to reach the fluorescent screen successively, 'photos' of the quantum-classical border (continuous decrease of contrast with decreasing height above the plate) are built up.
Quantum theory is often cited as being one of the most empirically validated theories in terms of its predictive power and precision. These attributes have led to numerous scientific discoveries and technological advancements. However, the precise relationship between quantum and classical physics remains obscure. The prevailing description is known as decoherence theory, where classical physics emerges from a more general quantum theory through environmental interaction. Sometimes referred to as the decoherence program, it does not solve the quantum measurement problem. We believe experiments performed between the microscopic and macroscopic world may help finish the program. The following considers a free electron that interacts with a surface (the environment), providing a controlled decoherence mechanism. There are non-decohering interactions to be examined and quantified before the weaker decohering effects are filtered out. In the first experiment, an electron beam passes over a surface that’s illuminated by low-power laser light. This induces a surface charge redistribution causing the electron deflection. This phenomenon’s parameters are investigated. This system can be well understood in terms of classical electrodynamics, A second experiment tests decoherence theory by introducing a nanofabricated diffraction grating before the surface. The electron undergoes diffraction through the grating, but as the electron passes over the surface it’s predicted by various physical models that the electron will lose its wave interference property. Image charge based models, which predict a larger loss of contrast than what is observed, are falsified (despite experiencing an image charge force). A theoretical study demonstrates how a loss of contrast may not be due to the irreversible process decoherence, but dephasing (a reversible process due to randomization of the wavefunction’s phase). To resolve this ambiguity, a correlation function on an ensemble of diffraction patterns is analyzed after an electron undergoes either process in a path integral calculation. The diffraction pattern is successfully recovered for dephasing, but not for decoherence, thus verifying it as a potential tool in experimental studies to determine the nature of the observed process.
In the interaction between a quantum mechanical electron wave and a wall, loss of interference contrast is observed. It is of general interest to identify the mechanism and categorize its nature as dephasing or decoherence. Decoherence is of fundamental importance for the transition between the classical and quantum boundary, while dephasing is often an experimental detriment that needs to be understood and overcome. We find that the loss of contrast is attributed to a local charge distribution induced by secondary emission: a dephasing mechanism. This mechanism is expected to be present for many materials, is clearly visible for copper oxide, and can mask decoherence mechanisms. The local charge distribution on the wall causes a loss of contrast and electron beam deformation. A model based on Coulomb interaction with the surface charge gives good agreement for both features. Our model can thus be used to improve the experimental design and lead to separate out decoherence phenomena in the electron-wall system.
Electron microscopes provide a powerful platform for exploring physical phenomena with nanoscale resolution, based on the interaction of free electrons with the excitations of a sample such as phonons, excitons, bulk plasmons, and surface plasmons. The interaction usually results in the absorption or emission of such excitations, which can be detected directly through cathodoluminescence or indirectly through electron energy loss spectroscopy (EELS). However, as we show here, the underlying interaction of a free electron and an arbitrary optical excitation goes beyond what was predicted or measured so far, due to the interplay of entanglement and decoherence of the electron-excitation system. The entanglement of electrons and optical excitations can provide new analytical tools in electron microscopy. For example, it can enable measurements of optical coherence, plasmonic lifetimes, and electronic length scales in matter (such as the Bohr radius of an exciton). We show how these can be achieved using common configurations in electron diffraction and EELS, revealing significant changes in the electron’s coherence, as well as in other quantum information theoretic measures such as purity. Specifically, we find that the purity after interaction with nanoparticles can only take discrete values, versus a continuum of values for interactions with surface plasmons. We quantify the post-interaction density matrix of the combined electron-excitation system by developing a framework based on macroscopic quantum electrodynamics. The framework enables a quantitative account of decoherence due to excitations in any general polarizable material (optical environment). This framework is thus applicable beyond electron microscopy. Particularly in electron microscopy, our work enriches analytical capabilities and informs the design of quantum information experiments with free electrons, allowing control over their quantum states and their decoherence by the optical environment.