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Physical Review Letters

Thermal diffusivity and chaos in metals without quasiparticles

Richard A. Davison, Subir Sachdev A, Michael Andrew Blake

Published Nov 1, 2017• 0 citations
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Abstract

We study the thermal diffusivity D[subscript T] in models of metals without quasiparticle excitations (“strange metals”). The many-body quantum chaos and transport properties of such metals can be efficiently described by a holographic representation in a gravitational theory in an emergent curved spacetime with an additional spatial dimension. We find that at generic infrared fixed points D[subscript T] is always related to parameters characterizing many-body quantum chaos: the butterfly velocity v[subscript B] and Lyapunov time τ[subscript L] through D[subscript T]∼v[subscript B][superscript 2]τ[subscript L]. The relationship holds independently of the charge density, periodic potential strength, or magnetic field at the fixed point. The generality of this result follows from the observation that the thermal conductivity of strange metals depends only on the metric near the horizon of a black hole in the emergent spacetime and is otherwise insensitive to the profile of any matter fields.

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We study the thermal diffusivity D[subscript T] in models of metals without quasiparticle excitations (“strange metals”). The many-body quantum chaos and transport properties of such metals can be efficiently described by a holographic representation in a gravitational theory in an emergent curved spacetime with an additional spatial dimension. We find that at generic infrared fixed points D[subscript T] is always related to parameters characterizing many-body quantum chaos: the butterfly velocity v[subscript B] and Lyapunov time τ[subscript L] through D[subscript T]∼v[subscript B][superscript 2]τ[subscript L]. The relationship holds independently of the charge density, periodic potential strength, or magnetic field at the fixed point. The generality of this result follows from the observation that the thermal conductivity of strange metals depends only on the metric near the horizon of a black hole in the emergent spacetime and is otherwise insensitive to the profile of any matter fields.
Significance All high-temperature superconductors exhibit a remarkable “strange metal” state above their critical temperatures. A theory of the strange metal is a prerequisite for a deeper understanding of high-temperature superconductivity, but the ubiquitous quasiparticle theory of normal metals cannot be extended to the strange metal. Instead, strange metals exhibit many-body chaos over the shortest possible time allowed by quantum theory. We characterize the quantum chaos in a model of fermions at nonzero density coupled to an emergent gauge field. We find a universal relationship between the chaos parameters and the experimentally measurable thermal diffusivity. Our results establish a connection between quantum dephasing and energy transport in states of quantum matter without quasiparticles.
Essentially all high temperature superconductors display a ``strange metal'' regime above their critical temperatures, where electrical and thermal transport cannot be explained within the traditional Fermi liquid paradigm of quasiparticle excitations. This paper focuses on the first, and newly discovered, solvable theory of a disordered metal without quasiparticle excitations, obtained by extending the Sachdev-Ye-Kitaev (SYK) models to finite spatial dimensions. The complete thermoelectric conductivity matrix is computed, and a surprising exact relation is found between the Seebeck coefficient and the derivative of the thermodynamic entropy with respect to the density. These computations are then compared with holographic theories which map strange metals onto black holes in theories of quantum gravity with one extra spatial dimension.
We model strange metals as quantum liquids without quasiparticle excitations, but with slow momentum relaxation and with slow diffusive dynamics of a conserved charge and energy. General expressions are obtained for electrical, thermal, and thermoelectric transport in the presence of an applied magnetic field using the memory matrix formalism. In the appropriate limits, our expressions agree with previous hydrodynamic and holographic results. We discuss the relationship of such results to thermoelectric and Hall transport measurements in the strange-metal phase of the hole-doped cuprates.
We study a relation between the thermal diffusivity (D T ) and two quantum chaotic properties, Lyapunov time (τ L ) and butterfly velocity (v B ) in strongly correlated systems by using a holographic method. Recently, it was shown that Ei:=DT,i/(vB,i2τL)(i=x,y) {\mathbb{E}}_i:={D}_{T,i}/\left({v}_{{}^{B,i}}^2{\tau}_L\right)\left(i=x,y\right) Ei​:=DT,i​/(vB,i2​τL​)(i=x,y) is universal in the sense that it is determined only by some scaling exponents of the IR metric in the low temperature limit regardless of the matter fields and ultraviolet data. Inspired by this observation, by analyzing the anisotropic IR scaling geometry carefully, we find the concrete expressions for Ei {\mathbb{E}}_i Ei​ in terms of the critical dynamical exponents z i in each direction, Ei=zi/2(zi−1) {\mathbb{E}}_i={z}_i/2\left({z}_i-1\right) Ei​=zi​/2(zi​−1) . Furthermore, we find the lower bound of Ei {\mathbb{E}}_i Ei​ is always 1/2, which is not affected by anisotropy, contrary to the η/s case. However, there may be an upper bound determined by given fixed anisotropy.
Since the mid-eighties there has been an accumulation of metallic materials whose thermodynamic and transport properties differ significantly from those predicted by Fermi liquid theory. Examples of these so-called non-Fermi liquids include the strange metal phase of high transition temperature cuprates, and heavy fermion systems near a quantum phase transition. We report on a class of non-Fermi liquids discovered using gauge/gravity duality. The low energy behavior of these non-Fermi liquids is shown to be governed by a nontrivial infrared (IR) fixed point which exhibits nonanalytic scaling behavior only in the temporal direction. Within this class we find examples whose single-particle spectral function and transport behavior resemble those of strange metals. In particular, the contribution from the Fermi surface to the conductivity is inversely proportional to the temperature. In our treatment these properties can be understood as being controlled by the scaling dimension of the fermion operator in the emergent IR fixed point.
This dissertation is a study of various aspects of metals with strong interactions between electrons, with a particular emphasis on the problem of charge transport through them. We consider the physics of clean or weakly-disordered metals near some quantum critical points, and highlight novel transport regimes that could be relevant to experiments. We then develop a variety of exactly-solvable lattice models of strongly interacting non-Fermi liquid metals using novel non-perturbative techniques based on the Sachdev-Ye-Kitaev models, and relate their physics to that of the ubiquitous “strange metal” normal state of most correlated-electron superconductors, providing controlled theoretical insight into the possible mechanisms behind it. Finally, we use ideas from the field of quantum chaos to study mathematical quantities that can provide evidence for the existence of quasiparticles (or the lack thereof) in quantum many-body systems, in the context of metals with correlated electrons.