This dissertation is a study of various aspects of metals with strong interactions between electrons, with a particular emphasis on the problem of charge transport through them. We consider the physics of clean or weakly-disordered metals near some quantum critical points, and highlight novel transport regimes that could be relevant to experiments. We then develop a variety of exactly-solvable lattice models of strongly interacting non-Fermi liquid metals using novel non-perturbative techniques based on the Sachdev-Ye-Kitaev models, and relate their physics to that of the ubiquitous “strange metal” normal state of most correlated-electron superconductors, providing controlled theoretical insight into the possible mechanisms behind it. Finally, we use ideas from the field of quantum chaos to study mathematical quantities that can provide evidence for the existence of quasiparticles (or the lack thereof) in quantum many-body systems, in the context of metals with correlated electrons.
We study the thermal diffusivity D[subscript T] in models of metals without quasiparticle excitations (“strange metals”). The many-body quantum chaos and transport properties of such metals can be efficiently described by a holographic representation in a gravitational theory in an emergent curved spacetime with an additional spatial dimension. We find that at generic infrared fixed points D[subscript T] is always related to parameters characterizing many-body quantum chaos: the butterfly velocity v[subscript B] and Lyapunov time τ[subscript L] through D[subscript T]∼v[subscript B][superscript 2]τ[subscript L]. The relationship holds independently of the charge density, periodic potential strength, or magnetic field at the fixed point. The generality of this result follows from the observation that the thermal conductivity of strange metals depends only on the metric near the horizon of a black hole in the emergent spacetime and is otherwise insensitive to the profile of any matter fields.
Strange metals—ubiquitous in correlated quantum materials—transport electrical charge at low temperatures but not by the individual electronic quasiparticle excitations, which carry charge in ordinary metals. In this work, we consider two-dimensional metals of fermions coupled to quantum critical scalars, the latter representing order parameters or fractionalized particles. We show that at low temperatures ( T ), such metals generically exhibit strange metal behavior with a T -linear resistivity arising from spatially random fluctuations in the fermion-scalar Yukawa couplings about a nonzero spatial average. We also find a T ln(1/ T ) specific heat and a rationale for the Planckian bound on the transport scattering time. These results are in agreement with observations and are obtained in the large N expansion of an ensemble of critical metals with N fermion flavors.
Quantum phase transitions occur strictly at zero temperature and are accessed by varying a physical parameter such as a magnetic field or chemical potential. While these transitions themselves are experimentally inaccessible, the existence of a zero temperature quantum critical point has remarkable effects on the dynamical properties of interacting quantum many-body systems at finite temperatures. In this thesis, we study dynamics in four strongly interacting many-body systems near quantum critical points in the context of NMR relaxation, quantum quenches, many-body quantum chaos, and charge diffusion. In chapter 1, we begin by revisiting the issue of NMR relaxation in the quantum disordered phase of Ising spin chains. We find that the imaginary part of the spin susceptibility at low frequences is dominated by rare quantum processes which leads to an NMR relaxation rate that scales as
1/T1∼exp(−T2Δ) near the quantum critical point rather than the previously conjectured
1/T1∼exp(−TΔ). These results resolve certain discrepancies between the energy scales measured with different experimental probes in the quantum disordered paramagnetic phase of the Ising chain system
CoNb2O6. In chapter 2, we study the non-equilibrium dynamics of Sachdev-Ye-Kitaev (SYK) models with
q body interactions after a quantum quench, considering a quench protocol which drives the system from an initial state with long-lived quasiparticle excitations to a final state lacking any long-lived quasiparticle excitations. For
q=4, we find that the timescale for the system to locally thermalize
τeq∼kBTℏ and for
q→∞ we find that the system thermalizes instantaneously. In chapter 3, we study the real time dynamics of quantum electrodynamics in 2+1 dimensions with
Nf flavors of fermions. We focus on thermalization and the onset of many-body quantum chaos and compute the quantum Lyapunov exponent in a
Nf1 expansion. We briefly comment on chaos, locality, and gauge invariance. Finally, in Chapter 4 we consider whether the butterfly velocity - a speed at which quantum information propagates - may provide a fundamental bound on diffusion constants in dirty incoherent metals by computing the charge diffusion constant and the butterfly velocity in charge-neutral holographic matter with long wavelength ``hydrodynamic" disorder. In this limit, we find that the butterfly velocity does not set a sharp lower bound for the charge diffusion constant.
Strange or bad metallic transport, defined by incompatibility with the conventional quasiparticle picture, is a theme common to many strongly correlated materials, including high-temperature superconductors. The Hubbard model represents a minimal starting point for modeling strongly correlated systems. Here we demonstrate strange metallic transport in the doped two-dimensional Hubbard model using determinantal quantum Monte Carlo calculations. Over a wide range of doping, we observe resistivities exceeding the Mott-Ioffe-Regel limit with linear temperature dependence. The temperatures of our calculations extend to as low as 1/40 of the noninteracting bandwidth, placing our findings in the degenerate regime relevant to experimental observations of strange metallicity. Our results provide a foundation for connecting theories of strange metals to models of strongly correlated materials.
Abstract The mysterious metallic phase showing T-linear resistivity and a universal scattering rate 1 / τ = α P k B T / ℏ with a universal prefactor α P ∼ 1 and logarithmic-in-temperature singular specific heat coefficient, the so-called ‘Planckian metal phase’ was observed in various overdoped high- T c cuprate superconductors over a finite range in doping. Revealing the mystery of the Planckian metal state is believed to be the key to understanding the mechanism for high- T c superconductivity. Here, we propose a generic microscopic mechanism for this state based on quantum-critical local bosonic charge Kondo fluctuations coupled to both spinon and a heavy conduction-electron Fermi surface within the heavy-fermion formulation of the slave-boson t–J model. By a controlled perturbative renormalization group analysis, we examine the competition between the pseudogap phase, characterized by Anderson’s Resonating-Valence-Bond spin-liquid, and the Fermi-liquid state, modeled by the electron hopping (effective charge Kondo effect). We find a quantum-critical metallic phase with a universal Planckian ℏ ω / k B T scaling in scattering rate near an extended localized-delocalized (pseudogap-to-Fermi liquid) charge-Kondo breakdown transition. The d-wave superconducting ground state emerges near the transition. Unprecedented qualitative and quantitative agreements are reached between our theoretical predictions and various experiments, including optical conductivity, universal doping-independent field-to-temperature scaling in magnetoresistance, specific heat coefficient, marginal Fermi-liquid spectral function observed in ARPES, and Fermi surface reconstruction observed in Hall coefficients in various overdoped cuprates. Our mechanism offers a microscopic understanding of the quantum-critical Planckian metal phase observed in cuprates and its link to the pseudogap, d-wave superconducting, and Fermi liquid phases. It offers a promising route for understanding how d-wave superconductivity emerges from such a strange metal phase in cuprates–one of the long-standing open problems in condensed matter physics since 1990s–as well as shows a broader implication for the Planckian strange metal states observed in other correlated unconventional superconductors.