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Journal of Experimental and Theoretical Physics

Investigation of the absorption spectrum of a two-level system subjected to intense two-photon excitation

V. A. Khodovoǐ, N. A. Chigir

Published Jan 1, 1978• 0 citations
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Il Nuovo Cimento•Apr 1, 1965•7 citations
We investigate how the quantum control of a two-level system (TLS) coupled to photons can modify and tune the TLS's photon absorption spectrum. Tuning and controlling the emission and the absorption are of great interest, e.g., for the development of efficient interfaces between stationary and flying qubits in modern architectures for quantum computation and quantum communication. We consider periodic pulse control, where the TLS is subjected to a periodic sequence of the near-resonant Rabi driving pulses, each pulse implementing a ${180}^{\ensuremath{\circ}}$ rotation. For small interpulse delays, the absorption spectrum features a pronounced peak of stimulated emission at the pulse frequency, similar satellite peaks with smaller spectral weights, and the net absorption peaks on the sides. As long as the detuning between the carrier frequency of the driving and the TLS transition frequency remains moderate, this spectral shape shows little change. Therefore, the pulse control allows shifting the absorption peak to a desired position and locks the overall absorption spectrum to the carrier frequency of the driving pulses. A detailed description of the spectrum and its evolution as a function time, the interpulse spacing, and the detuning is presented.
Abstract Theoretical and experimental investigations are made of two‐photon absorption spectra of trivalent rare‐earth ions in crystals. Effective cross‐sections, selection rules, and relative intensities of the components are found. The most intensive two‐photon transitions are established. Two‐photon excitation spectra of luminescence of Er3+ and Ho3+ ions in CaF2 are obtained and effective excitation cross‐sections are measured using a tunable dye laser (715 to 850 nm). It is shown that the spectra have a peculiar structure which differs considerably from that of the one‐photon absorption spectra. The experimental results agree with theory. It is established that one of the levels in Ho3+ is the level 5G6 rather than 3K7 usually assumed.
Measurements of the absolute generalized cross sections for the non-resonant two-photon excitation of discrete states of barium atoms are presented. They are based on the detection of an ion current due to absorption of a third photon in two processes of both resonant and non-resonant two-photon excitation of the same discrete level. Also considered is the appearance of additional lines in the two-photon absorption spectrum due to superradiance of the dye laser, the anomalous width of some of the two-photon resonances and the use of two-photon resonances for calibration purposes in investigation of autoionization resonances.