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Optics and Spectroscopy

Properties of resonance multilevel quantum systems in a strong light field: strong-collision model

Vladimir Leonardovich Derbov, Sergey K. Potapov, A. D. Novikov

Published Mar 1, 1987• 0 citations
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We study the deflection of an atomic system with a resonant multilevel energy structure in classical and quantized wave light fields. We obtain that the shape of the momentum distribution is very sensitive to the energy level structure, whereas its moments are not. Comparison with a two-level case is made. PACS: 32.80, 33.80, 42.50 During the last two decades a remarkable development in mechanically manipulating atomary particles with resonant laser light has taken place (for a review, see for example [1, 2] and references therein). In addition to trapping and cooling of particles, the deflection of particles by a laser beam offers interesting possibilities, for example, to construct atomic interferometers or beam splitters [2-4]. This problem has been studied extensively both theoretically [2, 5, 8] and experimentally [9-12]. The fact that the momentum distribution caused by the scattering is connected to the quantum statistical properties of the scattered light has been known for some time [13]. Recently, one has also realized that the quantum statistics of the light causing the scattering can be important [14]. At low photon numbers, for example, the initial field state strongly influences the resulting momentum distribution. A related effect is that a standing wave and two counterpropagating traveling plane waves of equal emplitudes cause a different diffraction pattern when fields are treated quantum mechanically [15]. Most previous work on the deflection of particles by light fields used two-level atoms. In this paper we study how resonant multilevel systems scatter when they traverse a plane wave. In practical applications, molecules or highly excited atoms have similar energy structures as the models we use in this work. In most cases, we assume that the Raman-Nath regime is valid, i.e., the kinetic energy of the particle can be neglected. However, the field coupling is assumed to be sufficiently strong to make multiple scattering events possible. Our results show that the final momentum distribution of a multi-level system can strongly deviate from that of a two-level atom. It is of interest that the momentum distributions for resonant ladder systems are in general superpositions of few or several distributions similar to that of a two-level system. We also study the expectation values related to the momentum distribution and show that the spread in momentum is remarkably independent of the system considered. The absorption and reabsorption of photons during the scattering process causes the photon distribution to be smoothed out, and for long times a steady state is reached. The cases we studied did not show a creation of sub-Poissonian light. Our model and assumptions are described and discussed in Sect. 1. Some of the general properties of the momentum distribution are discussed in Sect. 2. In Sect. 3 we derive the generating function of the moments of momentum change in Raman-Nath regime. The main part of the paper is contained in Sects. 4 and 5, in which the momentum distribution itself is discussed for several model systems. In Sect. 4 a semiclassical field is assumed and in Sect. 5 a quantum field is used. The effects of the scattering on the field photon statistics are studied in Sect. 6. The final discussion of the results is given in Sect. 7.

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We study the deflection of an atomic system with a resonant multilevel energy structure in classical and quantized wave light fields. We obtain that the shape of the momentum distribution is very sensitive to the energy level structure, whereas its moments are not. Comparison with a two-level case is made. PACS: 32.80, 33.80, 42.50 During the last two decades a remarkable development in mechanically manipulating atomary particles with resonant laser light has taken place (for a review, see for example [1, 2] and references therein). In addition to trapping and cooling of particles, the deflection of particles by a laser beam offers interesting possibilities, for example, to construct atomic interferometers or beam splitters [2-4]. This problem has been studied extensively both theoretically [2, 5, 8] and experimentally [9-12]. The fact that the momentum distribution caused by the scattering is connected to the quantum statistical properties of the scattered light has been known for some time [13]. Recently, one has also realized that the quantum statistics of the light causing the scattering can be important [14]. At low photon numbers, for example, the initial field state strongly influences the resulting momentum distribution. A related effect is that a standing wave and two counterpropagating traveling plane waves of equal emplitudes cause a different diffraction pattern when fields are treated quantum mechanically [15]. Most previous work on the deflection of particles by light fields used two-level atoms. In this paper we study how resonant multilevel systems scatter when they traverse a plane wave. In practical applications, molecules or highly excited atoms have similar energy structures as the models we use in this work. In most cases, we assume that the Raman-Nath regime is valid, i.e., the kinetic energy of the particle can be neglected. However, the field coupling is assumed to be sufficiently strong to make multiple scattering events possible. Our results show that the final momentum distribution of a multi-level system can strongly deviate from that of a two-level atom. It is of interest that the momentum distributions for resonant ladder systems are in general superpositions of few or several distributions similar to that of a two-level system. We also study the expectation values related to the momentum distribution and show that the spread in momentum is remarkably independent of the system considered. The absorption and reabsorption of photons during the scattering process causes the photon distribution to be smoothed out, and for long times a steady state is reached. The cases we studied did not show a creation of sub-Poissonian light. Our model and assumptions are described and discussed in Sect. 1. Some of the general properties of the momentum distribution are discussed in Sect. 2. In Sect. 3 we derive the generating function of the moments of momentum change in Raman-Nath regime. The main part of the paper is contained in Sects. 4 and 5, in which the momentum distribution itself is discussed for several model systems. In Sect. 4 a semiclassical field is assumed and in Sect. 5 a quantum field is used. The effects of the scattering on the field photon statistics are studied in Sect. 6. The final discussion of the results is given in Sect. 7.
The resonant response of a multilevel atomic system to strong coherent radiation is analyzed using an extension of the methods of time-independent scattering theory, adapted to the density-matrix formalism in order to include thermal bath effects. General steady-state expressions are derived for self-attenuation and resonance scattering rates in strong saturating fields, as functions of the coupling strengths, relaxation parameters, and frequency detunings. Formal expressions are given for radiative-damping and collision-broadening relaxation parameters, relating the latter to scattering amplitudes. Modifications of collision-broadening parameters by the presence of very strong fields are discussed. The Bloch equations are derived by transformation to the time domain, under specified conditions.
A theory of resonant light scattering from two level atoms in a gas is developed for an arbitrarily strong pump field. The Doppler effect and two body foreign gas collisions are considered. Elastic, inelastic (upward and downward), and the velocity changing collisions are retained in the general formulation. The impact approximation is not made, and the expressions for all (field dependent) collision rates are generated internally. Particular attention is paid to the lower state interaction, and a more complete parameterization of the theory is achieved. The general theory is non-Markovian and the quantum regression theorem is not used; it reduces to existing theories in special cases. It is shown that the coherent scattering is not a general property of the system if the lower state interaction is present; the "coherent" component acquires a small, but nonzero, width in the strong field region. This width could provide information about some new collision parameters.