Observation of Coherent Oscillations in a Single Electron Spin

Katja C. Nowack

Christoph Schlegel, Joris van Slageren, M. Manoli +2 more

Direct evidence of quantum coherence in a single-molecule magnet in a frozen solution is reported with coherence times as long as T{2}=630+/-30 ns. We can strongly increase the coherence time by modifying the matrix in which the single-molecule magnets are embedded. The electron spins are coupled to the proton nuclear spins of both the molecule itself and, interestingly, also to those of the solvent. The clear observation of Rabi oscillations indicates that we can manipulate the spin coherently, an essential prerequisite for performing quantum computations.

Pu Huang, Jingwei Zhou, Fang Fang +4 more

We demonstrate quantum coherent control of a single electron spin in a NV center in diamond using the Landau-Zener-Stuckelberg interferometry at room temperature. Interference pattern is observed oscillating as a function of microwave frequency. The decays in the visibility of the interference are well explained by numerical simulation which includes the thermal fluctuations of the nuclear bath which shows that Landau-Zener-Stuckelberg interferometry can be used for probing electron spin decoherence processes.

Yuxi Jiang, Amirehsan Alizadehherfati, Christine Falter +6 more

Coherent spin-photon interfaces are essential for scalable quantum networks, but their realization requires optically bright transitions, long-lived spin coherence, and complete coherent control. Donor-bound electron spins in II-VI semiconductors offer an attractive platform for optically active spin qubits because they combine strong donor-bound exciton transitions in a direct-bandgap material with a potentially nuclear-spin-free environment. However, coherent control of an individual optically active donor spin has remained elusive. Here we demonstrate optical initialization, coherent control, and readout of a single donor-bound electron spin in ZnSe. Using spin-selective donor-bound exciton optical transitions, we initialize the electron spin and directly resolve its spin-relaxation dynamics. We achieve coherent spin control with off-resonant picosecond optical pulses, as demonstrated by spin Rabi oscillations and Ramsey interference. We further coherently drive two spin-selective optical transitions and observe high-contrast coherent population trapping, demonstrating the formation of an optically controlled dark state. At higher driving strengths, multiple dark resonances reveal the hyperfine interaction between the electron and the I = 3/2 Cl nucleus. These results establish the first coherent optical control of a single donor electron spin in a II-VI semiconductor and identify isolated optical donors as a promising platform for solid-state optically active qubits.

D. V. Averin, K. K. Likharev

Chandrasekhar Ramanathan, James D. Lee, Paola Cappellaro +2 more