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New Journal of Physics

Molecular interferometers: effects of Pauli principle on entangled-enhanced precision measurements

Peter Alexander Bouvrie, A. P. Majtey, Francisco Figueiredo, I. Roditi

Published Nov 25, 2019• 1 citation
Publisher

Abstract

Abstract Feshbach molecules forming a Bose–Einstein condensate (BEC) behave as non-ideal bosonic particles due to their underlying fermionic structure. We study the observable consequences of the fermion exchange interactions in the interference of molecular BECs for entangled-enhanced precision measurements. Our many-body treatment of the molecular condensate is based on an ansatz of composite two-fermion bosons which accounts for all possible fermion exchange correlations present in the system. The Pauli principle acts prohibitively on the particle fluctuations during the interference process leading to a loss of precision in phase estimations. However, we find that, in the regime where molecular dissociations do not jeopardize the interference dynamics, measurements of the phase can still be performed with a precision beyond the classical limit comparable to atomic interferometers. We also show that the effects of Pauli principle increases with the noise of the particle detectors such that molecular interferometers would require more efficient detectors.

DOI
10.1088/1367-2630/ab5b2f

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Abstract Feshbach molecules forming a Bose–Einstein condensate (BEC) behave as non-ideal bosonic particles due to their underlying fermionic structure. We study the observable consequences of the fermion exchange interactions in the interference of molecular BECs for entangled-enhanced precision measurements. Our many-body treatment of the molecular condensate is based on an ansatz of composite two-fermion bosons which accounts for all possible fermion exchange correlations present in the system. The Pauli principle acts prohibitively on the particle fluctuations during the interference process leading to a loss of precision in phase estimations. However, we find that, in the regime where molecular dissociations do not jeopardize the interference dynamics, measurements of the phase can still be performed with a precision beyond the classical limit comparable to atomic interferometers. We also show that the effects of Pauli principle increases with the noise of the particle detectors such that molecular interferometers would require more efficient detectors.
Any experimental realization of Bose-Einstein condensation (BEC) deals with composite bosons (cobosons), which are quasi-particles made of fermion pairs that suffer Pauli blocking. We evidence that the prime consequence of the Pauli exclusion principle is to prevent cobosons from having their centers of mass located at the same position within their spatial extension. We moreover predict a many-body effect induced by Pauli blocking that leads to high interference wave modes resulting from fermion exchanges between two colliding coboson condensates. These two effects can be detected by measuring spatial correlation functions. We here propose an original procedure to exactly derive such correlation functions for Frenkel-like cobosons characterized by just their momentum. We physically extend the obtained results to more complex Wannier-like cobosons that have an additional relative motion index. In addition to revealing the physics involved in results previously obtained for elementary boson condensates, we use Shiva diagrams to show how it is changed for cobosons. The predictions we here present, established for matter bosons, are directly applicable to experiments.
We show that an ansatz based on independent composite bosons [Phys. Rep. 463, 215 (2008)] accurately describes the condensate fraction of molecular Bose-Einstein condensates in ultracold Fermi gases. The entanglement between the fermionic constituents of a single Feshbach molecule then governs the many-particle statistics of the condensate, from the limit of strong interaction to close to unitarity. This result strengthens the role of entanglement as the indispensable driver of composite-boson behavior. The condensate fraction of fermion pairs at zero temperature that we compute matches excellently previous results obtained by means of fixed-node diffusion Monte Carlo methods and the Bogoliubov depletion approximation. This paves the way towards the exploration of the BEC-BCS crossover physics in mixtures of cold Fermi gases with an arbitrary number of fermion pairs as well as the implementation of Hong-Ou-Mandel--like interference experiments proposed within coboson theory.
Bose-Einstein condensate (BEC) is considered under conditions of Feshbach resonance in two-atom collisions due to a coupling of atomic pair and resonant molecular states. The association of condensate atoms can form a molecular BEC, and the molecules can dissociate to pairs of entangled atoms in two-mode squeezed states. Both entanglement and squeezing can be applied to quantum measurements and information processing. The processes in the atom-molecule quantum gas are analyzed using two theoretical approaches. The mean-field one takes into account deactivating collisions of resonant molecules with other atoms and molecules, neglecting quantum fluctuations. This method allows analysis of inhomogeneous systems, such as expanding BEC. The non-mean-field approach -- the parametric approximation -- takes into account both deactivation and quantum fluctuations. This method allows determination of optimal conditions for formation of molecular BEC and describes Bose-enhanced dissociation of molecular BEC, as well as entanglement and squeezing of the non-condensate atoms.
The use of Feshbach resonances for tuning the interparticle interaction in ultracold Fermi gases has led to remarkable developments, in particular to the creation and Bose-Einstein condensation of weakly bound diatomic molecules of fermionic atoms.These are the largest diatomic molecules obtained so far, with a size of the order of thousands of angstroms.They represent novel composite bosons, which exhibit features of Fermi statistics at short intermolecular distances.Being highly excited, these molecules are remarkably stable with respect to collisional relaxation, which is a consequence of the Pauli exclusion principle for identical fermionic atoms.The purpose of this review is to introduce theoretical approaches and describe the physics of molecular regimes in two-component Fermi gases and Fermi-Fermi mixtures, focusing attention on quantum statistical effects.
The use of Feshbach resonances for tuning the interparticle interaction in ultracold Fermi gases has led to remarkable developments, in particular to the creation and Bose-Einstein condensation of weakly bound diatomic molecules of fermionic atoms. These are the largest diatomic molecules obtained so far, with a size of the order of thousands of angstroms. They represent novel composite bosons, which exhibit features of Fermi statistics at short intermolecular distances. Being highly excited, these molecules are remarkably stable with respect to collisional relaxation, which is a consequence of the Pauli exclusion principle for identical fermionic atoms. The purpose of this review is to introduce theoretical approaches and describe the physics of molecular regimes in two-component Fermi gases and Fermi-Fermi mixtures, focusing attention on quantum statistical effects.
We have observed the interference between two Bose–Einstein condensates of weakly bound Feshbach molecules of fermionic 6 Li atoms. Two condensates are prepared in a double-well trap and, after release from this trap, overlap in expansion. We detect a clear interference pattern that unambiguously demonstrates the de Broglie wavelength of molecules. We verify that only the condensate fraction shows interference. With increasing interaction strength, the pattern vanishes because elastic collisions during overlap remove particles from the condensate wave function. For strong interaction, the condensates do not penetrate each other as they collide hydrodynamically.