This PhD thesis reports on the development of a wide variety of theoretical and experimental capabilities in the field of quantum information processing using trapped ions. The presentation is organized in two distinct parts. The first part presents a series of published articles containing theoretical results, and their experimental validation, advancing a range of tools and techniques in error-resilient quantum control and robust verification procedures. One of the fundamental challenges in realizing a general purpose quantum computer is the management of error in fragile quantum systems. A familiar aspect of this challenge is decoherence, a process by which the system looses its stored quantum information, rendering it useless for subsequent computation. This collection of works focuses on reducing sources of quantum decoherence and precisely quantifying residual errors in real quantum systems dominated by realistic temporally-correlated noise processes, of central importance in any future architecture for quantum computing. The second part focuses on the design, construction and characterization of a complex experimental system capable of supporting a broad calls of quantum simulation experiments with hundreds of spin qubits using 9Be+ ions in a Penning trap. The trap design is optimized to suppress non-harmonic trapping potentials while providing wide optical access for engineering enhanced spin-motion coupling across large ion crystals. A superconducting magnet, equipped with a fully closed-cycle dual LN2/LHe recondensor, provides the magnetic field for trapping and produces the 55-GHz Zeeman-split qubit states suitable for microwave control. A custom UV laser system for driving the relevant transitions in neutral and ionized beryllium, as well as UV-compatible fibers and in-bore optomechanics for delivering microwave and laser beams to the trap, is presented. The thesis concludes with a brief outlook towards future theoretical and experimental studies, and extensions of the experimental setup
This PhD thesis reports on the development of a wide variety of theoretical and experimental capabilities in the field of quantum information processing using trapped ions. The presentation is organized in two distinct parts. The first part presents a series of published articles containing theoretical results, and their experimental validation, advancing a range of tools and techniques in error-resilient quantum control and robust verification procedures. One of the fundamental challenges in realizing a general purpose quantum computer is the management of error in fragile quantum systems. A familiar aspect of this challenge is decoherence, a process by which the system looses its stored quantum information, rendering it useless for subsequent computation. This collection of works focuses on reducing sources of quantum decoherence and precisely quantifying residual errors in real quantum systems dominated by realistic temporally-correlated noise processes, of central importance in any future architecture for quantum computing. The second part focuses on the design, construction and characterization of a complex experimental system capable of supporting a broad calls of quantum simulation experiments with hundreds of spin qubits using 9Be+ ions in a Penning trap. The trap design is optimized to suppress non-harmonic trapping potentials while providing wide optical access for engineering enhanced spin-motion coupling across large ion crystals. A superconducting magnet, equipped with a fully closed-cycle dual LN2/LHe recondensor, provides the magnetic field for trapping and produces the 55-GHz Zeeman-split qubit states suitable for microwave control. A custom UV laser system for driving the relevant transitions in neutral and ionized beryllium, as well as UV-compatible fibers and in-bore optomechanics for delivering microwave and laser beams to the trap, is presented. The thesis concludes with a brief outlook towards future theoretical and experimental studies, and extensions of the experimental setup
In the search for new computational paradigms past the impending end of Moore’s law quantum information processing based on cold trapped ions has emerged as a promising candidate. This thesis presents on the design, construction and testing of a setup for analog quantum simulation experiments using Be ion crystals in a Penning trap. At the heart of the experiment is a specialized Penning trap with wide optical access for engineering Ising-type interactions. The trap sits inside a superconducting magnet which runs continuously with minimal losses through a novel dual-stage reliquefier system. During this thesis, mechanical and optical subsystems for this ion trap quantum simulator were designed and built. Two laser systems based on nonlinear frequency conversion were set up to generate light for photoionization, Doppler cooling, state preparation, readout, and Raman interactions. In parallel, a method was devised to produce ultraviolet-solarization resistant fiber patch cords for pointing-stable light delivery. Inbore optomechanics and a collaboratively designed precision six-axis positioning device were constructed for beam delivery and trap alignment, respectively. These optomechanics co-locate custom-designed millimeterwave delivery systems as well as numerically optimized, diffraction-limited imaging optics for fluorescence readout. Using these subsystems, we validate interferometrically the motional stability of the setup from the mHz to kHz region during pulse-tube operation. First-ever light-ion interaction serves to validate calculations of interaction frequencies, optomechanics operation, and imaging performance, while coherent qubit interaction allows for this to be done on the millimeter wave setup, where initial Rabi flopping times of 18 us were observed. Site-resolved imaging of rapidly rotating ion crystals demonstrates critical phase-locked operation of the apparatus; positioning the experiment for future upgrades towards a full analog quantum simulator.
Quantum computation is a promising technology owing to the unique physical nature of quantum systems. Quantum computers have the potential to be as much as exponentially more efficient than today’s most powerful classical computer at certain tasks. One of the major challenges the scientific community must overcome, arises due to the intrinsic tendency of quantum information to be highly susceptible to environmental noise. This thesis presents work in developing and characterizing methods for precision quantum control in the presence of decoherence inducing noise, using trapped 171Yb+ ions as a model experimental platform. A flexible , robust microwave system is used to access the 12.6 GHz hyperfine qubit manifold in the outer S-shell orbital. The low phase noise characteristics of a microwave oscillator allow free-evolution coherence times in excess of three seconds, and operational fidelities F > 99.99%, characterized by randomized benchmarking. Starting from this relatively clean baseline, control techniques may be implemented in order to simulate a variety of realistic, time-dependent noise models, via arbitrary IQ modulation of the microwave source. A formalism for calculating the spectral noise filter functions of piece-wise constant control sequences is developed. The efficacy of this formalism is demonstrated by experimentally characterizing a variety of control protocols in the presence of engineered noise.
Abstract A major obstacle in the way of practical quantum computing is achieving scalable and robust high-fidelity entangling gates. To this end, quantum control has become an essential tool, as it can make the entangling interaction resilient to sources of noise. Nevertheless, it may be difficult to identify an appropriate quantum control technique for a particular need given the breadth of work pertaining to robust entanglement. To this end, we attempt to consolidate the literature by providing a non-exhaustive summary and critical analysis. The quantum control methods are separated into two categories: schemes which extend the robustness to (i) spin or (ii) motional decoherence. We choose to focus on extensions of the σ x ⊗ σ x Mølmer–Sørensen interaction using microwaves and a static magnetic field gradient. Nevertheless, some of the techniques discussed here can be relevant to other trapped ion architectures or physical qubit implementations. Finally, we experimentally realize a proof-of-concept interaction with simultaneous robustness to spin and motional decoherence by combining several quantum control methods presented in this manuscript.
We provide an introduction to the use of ion crystals in a Penning trap for experiments in quantum information. Macroscopic Penning traps allow for the containment of a few to a few million atomic ions whose internal states may be used in quantum information experiments. Ions are laser Doppler cooled, and the mutual Coulomb repulsion of the ions leads to the formation of crystalline arrays. The structure and dimensionality of the resulting ion crystals may be tuned using a combination of control laser beams and external potentials. We discuss the use of two-dimensional 9Be+ ion crystals for experimental tests of quantum control techniques. Our primary qubit is the 124 GHz ground-state electron spin flip transition, which we drive using microwaves. An ion crystal represents a spatial ensemble of qubits, but the effects of inhomogeneities across a typical crystal are small, and as such we treat the ensemble as a single effective spin. We are able to initialize the qubits in a simple state and perform a projective measurement on the system. We demonstrate full control of the qubit Bloch vector, performing arbitrary high-fidelity rotations ($\tau_{\pi}\sim$200 μs). Randomized Benchmarking demonstrates an error per gate (a Pauli-randomized π/2 and π pulse pair) of 8±1×10−4. Ramsey interferometry and spin-locking measurements are used to elucidate the limits of qubit coherence in the system, yielding a typical free-induction decay coherence time of $T_{2}\sim$2 ms, and a limiting $T_{1\rho}\sim$688 ms. These experimental specifications make ion crystals in a Penning trap ideal candidates for novel experiments in quantum control. As such, we briefly describe recent efforts aimed at studying the error-suppressing capabilities of dynamical decoupling pulse sequences, demonstrating an ability to extend qubit coherence and suppress phase errors. We conclude with a discussion of future avenues for experimental exploration, including the use of additional nuclear-spin-flip transitions for effective multiqubit protocols, and the potential for Coulomb crystals to form a useful testbed for studies of large-scale entanglement.
Quantum computers hold the potential of solving problems that are intractable using classical means. Yet, to date no quantum computer has actually solved a problem of general interest that could not have been solved otherwise. Bridging this gap from promised theoretical usefulness to practical relevance is an interdisciplinary challenge, requiring experimental progress, solutions of classical software challenges as well as advances in quantum algorithm design. It is these final two points in which this thesis aims to contribute. One of the most promising quantum computing architectures is based on trapping ions in surface-electrode ion-traps. In order to productively operate such trapped-ion quantum computers, we develop and benchmark a compiler that optimizes ion shuttling sequences in order to efficiently map abstract quantum circuits onto a physical trapped-ion chip. This is a necessary component of the infrastructure of a quantum computing setup, however it is alone not sufficient to execute arbitrary quantum algorithms. In particular, a very promising class of quantum algorithms are so-called hybrid quantum-classical algorithms which leverage the computational resources of both quantum and classical computers. To effectively implement such algorithms, a suitable software setup is necessary to allow for tight interplay between the two types of computers without wasting precious coherence time. To solve this challenge, we propose, implement and benchmark our setup for Interpreted Quantum-Classical Computations (IQCCs), demonstrating its feasibility for trapped-ion quantum computers. For the second part of this thesis we focus on the development of quantum algorithms that make use of this setup. As a first application, we investigate quantum simulations of gauge theories. Such theories are prevalent throughout modern physics and are characterized by local constraints that the dynamics are subject to. Errors in noisy simulations of such theories results in these constraints being violated and the simulations becoming unphysical. We show that this problem can be remedied by measuring gauge operators, decoding possible errors on a classical computer and actively correcting them, which reduces simulation errors. Additionally we interpret the scheme as a sympathetic cooling setup, which allows thermal control of the simulation. We finally turn to the task of preparing ground states of frustration-free Hamiltonians in quantum computers. Studying ground states of various systems is of paramount importance for solving optimization problems and understanding phenomena such as magnetism, superconductivity and superfluidity. We frame the ground-state preparation problem as an error correction problem, wherein energy is measured locally, measurements are decoded and corrections are applied to reduce the energy. In physically relevant examples we show up to exponentially improved runtimes over previous, similar algorithms and give a general run-time bound in terms of the Hamiltonian gap.
Trapped ions are a powerful and flexible platform used for scientific applications ranging from studies of fundamental physics and precision spectroscopy to quantum simulation and quantum information processing. These applications are enabled by the excellent control that can be exerted over the long-lived atomic states of trapped ions using electromagnetic fields. In crystals containing multiple ions, the shared motion is used as a mediator to couple the atomic states of distant ions. This thesis focuses on improving the control over ion motion, and in particular for crystals that contain multiple ion species. The first set of experiments discussed in this thesis is the application of a ground-state cooling method known as electromagnetically-induced-transparency (EIT) cooling to 25Mg+. This ion has a complex hyperfine structure which enables the implementation of a long-lived qubit. By demonstrating EIT cooling on 25Mg+, it is shown that such qubit ions are also compatible with this resource-efficient sub-Doppler cooling method. The normal modes of trapped-ion motion are well-described by quantum harmonic oscillators, and the second set of experiments described in this thesis covers the direct, rapid, and parametric coupling between two harmonic oscillators in the motion modes of multi-ion crystals. This coupling can be used to indirectly cool ion modes that are otherwise difficult or inefficient to cool. It can also be used to perform mid-circuit non-destructive readout of trapped-ion motion, which is useful for the study of states encoded in the ion motion, such as those used for bosonic error correction.