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APL Photonics

Nonlinear control of coherent absorption and its optical signal processing applications

Angelos Xomalis, Yongmin Jung, Iosif Demirtzioglou, Cosimo Lacava, Eric Plum, David John Richardson, Periklis Petropoulos, Nikolay I. Zheludev

Published Oct 1, 2019• 11 citations
Publisher

Abstract

All-optical data processing continues to attract significant interest as a way to overcome the electronic signal processing bottleneck of fiber telecommunication networks. Nonlinear optical devices such as limiters and saturable absorbers rely on intensity-dependent attenuation of light. However, making such devices using intensity-dependent multiphoton dissipation processes is an issue as these make complete absorption and transmission impossible. Here, we show that nonlinear phase retardation in an optical fiber can control the dissipation of coherent light waves interacting on a thin plasmonic absorber from total absorption to perfect transmission. The fiber’s instantaneous Kerr nonlinearity and the femtosecond coherent absorption time scale make this approach ultrafast. We report proof-of-principle demonstrations of all-optical intensity discrimination, power limiting, pulse restoration, pulse splitting, and signal transfer between carrier wavelengths within a fiber circuit. Our results indicate that nonlinear control of coherent absorption can imitate and outperform saturable and multiphoton absorption in terms of bandwidth and contrast.

DOI
10.1063/1.5123547

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•Jan 1, 2008•0 citations
All-optical data processing continues to attract significant interest as a way to overcome the electronic signal processing bottleneck of fiber telecommunication networks. Nonlinear optical devices such as limiters and saturable absorbers rely on intensity-dependent attenuation of light. However, making such devices using intensity-dependent multiphoton dissipation processes is an issue as these make complete absorption and transmission impossible. Here, we show that nonlinear phase retardation in an optical fiber can control the dissipation of coherent light waves interacting on a thin plasmonic absorber from total absorption to perfect transmission. The fiber’s instantaneous Kerr nonlinearity and the femtosecond coherent absorption time scale make this approach ultrafast. We report proof-of-principle demonstrations of all-optical intensity discrimination, power limiting, pulse restoration, pulse splitting, and signal transfer between carrier wavelengths within a fiber circuit. Our results indicate that nonlinear control of coherent absorption can imitate and outperform saturable and multiphoton absorption in terms of bandwidth and contrast.
Recently, coherent control of the optical response of thin films in standing waves has attracted considerable attention, ranging from applications in excitation-selective spectroscopy and nonlinear optics to all-optical image processing. Here, we show that integration of metamaterial and optical fibre technologies allows the use of coherently controlled absorption in a fully fiberized and packaged switching metadevice. With this metadevice, which controls light with light in a nanoscale plasmonic metamaterial film on an optical fibre tip, we provide proof-of-principle demonstrations of logical functions XOR, NOT and AND that are performed within a coherent fibre network at wavelengths between 1530 and 1565 nm. The metadevice has been tested at up to 40 gigabits per second and sub-milliwatt power levels. Since coherent absorption can operate at the single-photon level and with 100 THz bandwidth, we argue that the demonstrated all-optical switch concept has potential applications in coherent and quantum information networks.
Large distance implementation of quantum communication technologies requires coherent control of single photons in optical fiber networks. Here we demonstrate the phenomenon of coherent perfect absorption of single photons in a fully fiberized ultrathin plasmonic metamaterial fabricated at the end facet of an optical fiber. Continuous control of single-photon absorption probability is achieved by driving the network between the regimes of coherent total absorption and coherent total transmission. To circumvent phase fluctuations inherent to optical fiber networks, we implemented a reference-based postselection technique which yielded interference fringe visibility comparable to that of free space experiments. Coherent absorption of quantum light in fiber environment provides new opportunities for dissipative single-photon switching, filtering, and measurement, as well as for manipulation of entangled, weak coherent, and NOON states in optical fiber networks.
A fiber optic-based all-optical amplifier is designed by using the coherent perfect absorption phenomenon. For this purpose, we use a deposited chromium thin layer as an absorbent material on the cross-section of a PM fiber. By placing another fiber in front of the deposited one, we show that by controlling the relative phase between the two counter-propagating beams, total absorbance can be controlled. In the interaction of two beams with unequal intensities, absorption control can be associated with amplification for the weaker beam. By using this mechanism, the effect of an external phase-shifting parameter can be amplified. Furthermore, it is possible to amplify a small signal riding on a CW background through this all-optical procedure.
Results of study of nonlinear processes occurring during the propagation of light pulses in optical fibers doped with atoms of rare-earth elements under conditions of atomic coherence and interference are presented. For a three-level Λ scheme of interaction, the linear (χ (1) ) and nonlinear (χ (3) ) susceptibilities of such a medium are calculated. It is shown that the coefficients of Kerr nonlinearity and nonlinear absorption can reach extremely large values and can be negative. The competition between linear and nonlinear processes in the Λ scheme allows one to obtain compensation regimes when the coefficients of dispersion or absorption of the optical fiber material vanish. The efficient control of the optical properties of such a system over wide limits proves to be possible owing to variations in the parameters of light pulses at the input of the medium. The necessary conditions for realizing regimes with “slow” light, as well as for self-compression of a probing pulse on ultimately small spatial scales in a doped optical fiber, were obtained.
The four-wave mixing produced with two ultrashort phase-locked !-3! laser pulses propagating coherently in a two-level system in the infrared spectral region is shown to depend on the pulses relative phase. The Maxwell-Bloch equations are solved beyond the rotating-wave approximation to account for field frequencies which are largely detuned from the atomic resonance. The relative phase dominating the efficiency of the coupling to the 5! anti-Stokes Raman component is determined by sign of the total ac Stark shift induced in the system, in such a way that the phase influence disappears precisely where the ac Stark effect due to both pulses is compensated. This fundamental quantum interference effect can be the basis for nonlinear ultrafast optical spectroscopy techniques. Phenomena arising from the coherent control of nonlinear interactions are of importance in fields as diverse as optoelectronics and materials research, in high harmonic generation, in photoionization or molecular dissociation, and in biological applications such as spectroscopy and imaging, among others [1, 2, 3, 4, 5, 6, 7]. Optical quantum coherent control is based on the fact that the phases of interfering transition amplitudes in light-matter interactions can be controlled through the optical phase of coherent light sources that drive the interaction, in such a way that the transition rates to final states and the dynamics at various stages of the process can be modified [1]. In a recent paper [8], a theoretical investigation on the quantum coherent control of the optical transient four-wave mixing of two intense phase-locked femtosecond laser pulses of central angular frequencies ω and 3ω propagating in a two-level atom (TLA) was reported. It was shown how the nonlinear (χ (3) ) coupling to the antiStokes Raman field at frequency 5ω depends critically on the initial relative phase φ of the propagating pulses. In Ref. [8], the study was centered to intense pulses in the visible and ultraviolet spectral regions, with frequencies at resonance or lower than the atomic transition. The phenomena observed in [8], however, can be scaled to various laser and material parameters. In the infrared spectral range, for instance, experiments on ultrafast molecular dynamics are frequently performed by help of twocolor pump probe nonlinear spectroscopy techniques. In this type of studies, due to the high intensities inherent to ultrashort (subpicosecond) pulses, nonlinear effects such as stimulated Raman processes may become important and are often utilized as a complementary tool to gain information [9]. In this Letter, we address the conditions for quantum coherent control of transient four-wave mixing interactions with two phase-locked ω-3ω femtosecond laser pulses in the mid-IR spectral region. Our purpose is to reveal the basic physics for a strict two-level medium and to this end the Maxwell-Bloch TLA will be considered. We will study pulses with a duration of 300 fs (with a w 5w