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Optics and Spectroscopy

Nonlinear control of the propagation of optical pulses in doped optical fibers

A. V. Prokhorov, N. V. Korol’kova, Sergei M Arakelyan

Published Oct 1, 2005• 2 citations
Publisher

Abstract

Results of study of nonlinear processes occurring during the propagation of light pulses in optical fibers doped with atoms of rare-earth elements under conditions of atomic coherence and interference are presented. For a three-level Λ scheme of interaction, the linear (χ (1) ) and nonlinear (χ (3) ) susceptibilities of such a medium are calculated. It is shown that the coefficients of Kerr nonlinearity and nonlinear absorption can reach extremely large values and can be negative. The competition between linear and nonlinear processes in the Λ scheme allows one to obtain compensation regimes when the coefficients of dispersion or absorption of the optical fiber material vanish. The efficient control of the optical properties of such a system over wide limits proves to be possible owing to variations in the parameters of light pulses at the input of the medium. The necessary conditions for realizing regimes with “slow” light, as well as for self-compression of a probing pulse on ultimately small spatial scales in a doped optical fiber, were obtained.

DOI
10.1134/1.2113378

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arXiv:physics/0209036•Physical Review A•Jun 17, 2003•28 citations
Results of study of nonlinear processes occurring during the propagation of light pulses in optical fibers doped with atoms of rare-earth elements under conditions of atomic coherence and interference are presented. For a three-level Λ scheme of interaction, the linear (χ (1) ) and nonlinear (χ (3) ) susceptibilities of such a medium are calculated. It is shown that the coefficients of Kerr nonlinearity and nonlinear absorption can reach extremely large values and can be negative. The competition between linear and nonlinear processes in the Λ scheme allows one to obtain compensation regimes when the coefficients of dispersion or absorption of the optical fiber material vanish. The efficient control of the optical properties of such a system over wide limits proves to be possible owing to variations in the parameters of light pulses at the input of the medium. The necessary conditions for realizing regimes with “slow” light, as well as for self-compression of a probing pulse on ultimately small spatial scales in a doped optical fiber, were obtained.
Numerical solutions are obtained of the full self-consistent system of equations for the counter, rotating polarization components of the field of a short optical pulse propagating in a nonlinear birefringent fiber and in the ensemble of the energy-level degenerate doped resonance atoms implanted in the fiber material. In every cross section of the fiber, the ellipticity of the polarized wave experiences a complex evolution in time accompanied by rapid changes of the azimuthal angle due to the interplay of the dispersion and the Kerr nonlinear self-and cross-phase modulation. The reciprocal effect of the impurities on the traveling pulse causes oscillations of the pulse envelope that can completely distort the shape of the input signal, while the resonance absorption can drive the birefringence process from the nonlinear regime back to the linear one.
Optical solitons are expected to play a key role in single-mode optical-fiber communication systems. However, they are still degraded by the linear fiber loss. Therefore, in order to be realistically feasible, soliton-based systems will need repeaters to enhance the signal, and, from a practical point of view, optical amplifiers are preferable to electro-optical ones. The use of Raman nonlinearity,1 and, more recently, the use of rare-earth-doped fibers,2 have been proposed for such optical amplification. We have numerically simulated pulse propagation through singlemode silica fibers doped with passive two-level atoms in an attempt to cancel the linear fiber loss by the well known doping resonant nonlinearities. Our first results, from experiments carried out in a variety of circum-stances, indicate that the linear rate of loss may be diminished with a proper choice of parameters but that the doped fiber by itself is unable to support steady propagation.
This thesis deals with the study of propagation effects experienced by weak light pulses as they propagate in atomic media driven by strong pulses. We explore both the ultra-short and long pulse regime and investigate the phenomena that arise at these different time scales. In the short pulse regime, a strongly driven two level atomic system presents transient light shifts, and non-adiabatic transitions occur between these adiabatic levels. We have studied a method to probe these light shifts in real time by propagating a weak probe through the medium. The light shifts enrich the spectrum of the probe and the probe gets shaped as a result. In this way a strongly driven two-level system can act as an active pulse shaper, and can introduce oscillations in the temporal profile of an ultra-short pulse at a time scale shorter than the pulse duration. We also show that by driving the system with two time delayed non-resonant strong fields, the non-adiabatic effects can be rendered phase dependent. This gives very sensitive phase control of the excited state population and can be used to formulate new techniques in interferometry. In the long pulse regime we present a new method of slowing light that can be realized in a double two-level system interacting with two orthogonally polarized light pulses that propagate along different axis. Spatio-temporal dependence of the total polarization induces a grating in the ground Zeeman coherence. The stronger of the two fields (the control field) is diffracted from this grating into the direction of the weak probe field compensating for the absorption of this latter field. A transparency window is thus created in the absorption spectrum of the probe leading to the slowing down of light. The transparency window exhibits characteristics similar to the one obtained by EIT (electromagnetic induced transparency) method. However, the important difference between our method and the traditional EIT method, is that ours doesn't rely on realizing dark state in the system. This may open the possibility of slowing down light in more complex atomic media. Moreover, when the linear absorptive response of the medium is cancelled in this manner, the nonlinear response becomes more important. In the situation where fields propagate in the same direction and have same frequency, two regimes have been investigated. For small optical depths, the effective susceptibility behaves as chi_lin exp[2 i phi] (with phi the phase difference between two fields). This renders phase control of the medium response, and the medium can be changed from an absorber to an amplifier, with normal or anomalous dispersion, by adjusting the relative phase phi.  In the regime of large optical thickness, phase saturation takes place and the effective susceptibility turns into chi_lin*, changing an absorber into an amplifier without effecting the dispersive response (chi_lin is linear susceptibility).
The influence of Kerr nonlinearity and Doppler broadening on the slow light propagation of a dispersive atomic medium is revisited using a four-level ?-type (87Rb) atomic system under the condition of electromagnetically induced transparency (EIT). The medium exhibits an EIT process which is accompanied by normal dispersion, i.e.,?sub-luminal (slow light) pulse propagation. In the presence of Kerr nonlinearity and the Doppler broadening effect the dispersion property of the proposed atomic medium is modified, which leads to enhancement of the positive group index of the medium. The combined effect of Kerr nonlinearity and Doppler broadening on slow light propagation inside the medium is the major motivation for this work.
In the framework of the nonlinear Λ model, propagation of solitons was analysed in atomic vapours and Bose-Einstein condensates. The complicated nonlinear interplay between fast and slow-light solitons in a Λ-type medium was shown to facilitate control of its optical transparency and formation of optical gates. An exact analytical description was given for the deceleration, stopping and revival of slow-light solitons in the experimentally relevant non-adiabatic regime. A stopping slow-light soliton imprints a localized immobile polarization pattern in the medium, which, as explicitly demonstrated here, can be used as a bit of readable optical memory. The whole process can be controlled with the background field and an auxiliary laser field. The latter regulates the signal velocity, while the slow-light soliton can be stopped by switching off the former. The location and shape of the imprinted memory bit were also determined. With few assumptions characteristic of slow light, the Λ model was reduced to a simpler nonlinear model that also describes two-dimensional dilatonic gravity. Exact solutions could now be derived also in the presence of relaxation. Spontaneous decay of the upper atomic level was found to be strongly suppressed, and the spatial form of the decelerating slow-light soliton was preserved, even if the optical relaxation time was much shorter than the typical time scale of the soliton. The effective relaxation coefficient of the slow-light soliton was significantly smaller than that of an arbitrary optical pulse. Such features are obviously of great importance when this kind of system is applied, in practice, to information processing. A number of experimentally observable properties of the solutions reported were found to be in good agreement with recent experimental results, and a few suggestions are also made for future experiments.
We investigate a light-pulse propagation with negative group velocity in a nonlinear coherent medium. We show that the necessary conditions for nonlinear superluminal effects to be observable are realized in a three-level $\ensuremath{\Lambda}$ system interacting with a linearly polarized laser field in the presence of a static magnetic field. The initially prepared Zeeman coherence cancels the resonant absorption of the medium almost completely, but preserves its dispersion anomalous and very high. In this medium the light pulse propagates superluminally in the sense that the peak of the transmitted pulse exits the medium before the peak of the incident pulse enters. At the same time the pulse group velocity is intensity dependent, which leads to the self-steepening of the pulse trailing edge due to the fact that the more intense parts of the pulse travel slower. This is in contrast with the shock wave generation in a nonlinear medium with normal dispersion. The predicted effect can be easily observed in the well-known schemes employed in the studies of nonlinear magneto-optical rotation. The upper bound of sample length is found from the criterion that the pulse self-steepening and group-advance time are observable without pulse distortion caused by the group-velocity dispersion.