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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Extension of the Ion Optical Clock to Multi-Ion Systems

Kazuhiro Hayasaka

Published Jun 1, 2019• 0 citations
Publisher

Abstract

The optical clock is a fundamental applications of the coherence of ultracold atoms. Most of the implementations with trapped ions are based on the single-ion optical clock by Dehmelt [1], and some of them have successfully achieved inaccuracies in the 10-18level [2]. The idea has been extended to systems consisting of many neutral atoms by Katori with proper engineering on light shift associated with the optical lattice [3]. The enhanced stability is the great advantage obtained by multiple atoms. Extension of the single-ion system to multi-ion systems requires considerations on the inhomogeneous electric quadrupole shift originating from non-uniform electric field gradient at the location of each ion. A straightforward approach is to use ion species with null quadrupole moment such as In+, Al+[4]. We present another approach using ions with non-zero quadrupole moment. In the approach we use a planar surface trap to arrange the ions in an equally-spaced manner to vanish the inhomogeneous shift. We show that a clock with multiple Ca+ions can be operated even without a reference cavity for the clock laser, and that superradiant clock is expected when the ions are coupled to a cavity.

DOI
10.1109/cleoe-eqec.2019.8871750

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The optical clock is a fundamental applications of the coherence of ultracold atoms. Most of the implementations with trapped ions are based on the single-ion optical clock by Dehmelt [1], and some of them have successfully achieved inaccuracies in the 10-18level [2]. The idea has been extended to systems consisting of many neutral atoms by Katori with proper engineering on light shift associated with the optical lattice [3]. The enhanced stability is the great advantage obtained by multiple atoms. Extension of the single-ion system to multi-ion systems requires considerations on the inhomogeneous electric quadrupole shift originating from non-uniform electric field gradient at the location of each ion. A straightforward approach is to use ion species with null quadrupole moment such as In+, Al+[4]. We present another approach using ions with non-zero quadrupole moment. In the approach we use a planar surface trap to arrange the ions in an equally-spaced manner to vanish the inhomogeneous shift. We show that a clock with multiple Ca+ions can be operated even without a reference cavity for the clock laser, and that superradiant clock is expected when the ions are coupled to a cavity.
Scaling trapped-ion optical clocks to hundreds of ions remains a major challenge due to inhomogeneous frequency shifts in large ion crystals. Here, we propose a circular surface-trap architecture for a multi-ion optical clock with hundreds of ions. The rotational symmetry of the ion crystal suppresses the main sources of inhomogeneity, quadrupole shift.We investigate the feasibility of a clock based on a ring crystal of 400 40Ca+^{40}\mathrm{Ca}^{+}40Ca+ ions and propose a suitable experimental setup configuration. We have shown that circular configuration of ions leads to suppression by two orders of magnitude of the quadrupole shift comparing to the linear trap. Combined with stray-field compensation and dynamical decoupling techniques, this architecture provides a pathway toward multi-ion optical clocks with fractional frequency uncertainty at the 10−1810^{-18}10−18 level and an expected 20-fold improvement in frequency stability compared to single ion clocks.
Trapped-ion optical clocks are capable of achieving systematic fractional frequency uncertainties of 10−1810^{-18}10−18 and possibly below. However, the stability of current ion clocks is fundamentally limited by the weak signal of single-ion interrogation. We present an operational, versatile platform for extending clock spectroscopy to arrays of Coulomb crystals consisting of several tens of ions, while allowing systematic shifts as low as 10−1910^{-19}10−19. The concept is applicable to all clock transitions with low differential electric quadrupole moments. We observe 3D excess micromotion amplitudes of all individual ions inside a Coulomb crystal with nm resolution and prove that the related frequency shifts can be controlled simultaneously at the 10−1910^{-19}10−19 level. Using this method, we demonstrate regions of 400400400 μ\muμm and 222 mm length in our trap array with time dilation shifts due to micromotion close to 1×10−191\times10^{-19}1×10−19 and below 10−1810^{-18}10−18, respectively. Further measurements of the trapping environment and cooling dynamics calculations for mixed In+{}^++ / Yb+{}^++ crystals show that achievable clock uncertainties due to multi-ion operation in our setup are below 1×10−191\times10^{-19}1×10−19. This work will enable clock operation with multiple ions and open up the possibility of new interrogation schemes which allow optical clock stabilities beyond classical limits.
Abstract We present a novel method for engineering an optical clock transition that is robust against external field fluctuations and is able to overcome limits resulting from field inhomogeneities. The technique is based on the application of continuous driving fields to form a pair of dressed states essentially free of all relevant shifts. Specifically, the clock transition is robust to magnetic field shifts, quadrupole and other tensor shifts, and amplitude fluctuations of the driving fields. The scheme is applicable to either a single ion or an ensemble of ions, and is relevant for several types of ions, such as 40 Ca + , 88 Sr + , 138 Ba + and 176 Lu + . Taking a spherically symmetric Coulomb crystal formed by 400 40 Ca + ions as an example, we show through numerical simulations that the inhomogeneous linewidth of tens of Hertz in such a crystal together with linear Zeeman shifts of order 10 MHz are reduced to form a linewidth of around 1 Hz. We estimate a two-order-of-magnitude reduction in averaging time compared to state-of-the art single ion frequency references, assuming a probe laser fractional instability of 10 − 15 . Furthermore, a statistical uncertainty reaching 2.9 × 10−16 in 1 s is estimated for a cascaded clock scheme in which the dynamically decoupled Coulomb crystal clock stabilizes the interrogation laser for an 27 Al + clock.
An optical clock based upon a single mercury ion in a radio-frequency trap has the potential for both high stability and high accuracy. The systematic uncertainty of this frequency standard is limited by contributions due to two types of external fields. The clock has previously been operated with a magnetic bias field that destabilizes dark states that limit the rates of laser cooling and state detection. This bias field has previously resulted in a substantial second-order Zeeman shift. We now destabilize the dark states with a polarization-scrambling technique that allows us to operate with only a minimal magnetic field. The second uncertainty that we address here is the magnitude of the quadrupole shift due to the interaction of stray electric-field gradients with the quadrupole moment of the ion. We describe the steps that we are taking to evaluate this shift in the near future. 1
To date, optical clocks based on singly trapped ions and ultracold neutral atoms trapped in the Stark-shift-free optical lattices are regarded as promising candidates for future atomic clocks. Since 2006, “optical lattice clocks” have been evaluated close to the Cs clocks' uncertainty limit internationally. One of the essential experimental challenges in the development of “optical lattice clocks” is to find out the better lattice geometries as well as interrogated atom species (including their quantum statistics) that bring out the potential performance of the clock scheme, taking into account the collisional frequency shift, the Black body radiation (BBR) shift, the atomic multipolar and hyperpolarizability effects.