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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Optomechanical Self-Structuring of Cold Atoms with Structured Light

Giuseppe Baio, Gordon R. M. Robb, Alison M. Yao, Gian‐Luca Oppo

Published Jun 1, 2019• 0 citations
Publisher

Abstract

The spontaneous emergence of spatiotemporal order is a prominent feature of physical systems driven far from equilibrium. Recent experimental works have provided paradigmatic examples in transverse nonlinear optics with cold atoms such as spatial (optomechanical) or magnetic ordering [1], [2]. In the first case, the bunching of atoms due to dipole forces provides positive feedback leading to multimode symmetry breaking.

DOI
10.1109/cleoe-eqec.2019.8872827

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The spontaneous emergence of spatiotemporal order is a prominent feature of physical systems driven far from equilibrium. Recent experimental works have provided paradigmatic examples in transverse nonlinear optics with cold atoms such as spatial (optomechanical) or magnetic ordering [1], [2]. In the first case, the bunching of atoms due to dipole forces provides positive feedback leading to multimode symmetry breaking.
We theoretically, numerically and experimentally investigate spontaneous transverse instabilities in cold atomic gases, arising from the action of dispersive light forces. Previous research focused on pattern-forming instabilities in hot gases where optical nonlinearities arise from the internal structure of the atoms and spatio-temporal structures are encoded in the populations and coherences of the medium. Dipole forces acting on the center-of-mass of laser-cooled atoms, being dependent on gradients of the optical intensity, are also nonlinear in nature: previous studies focused, for instance, on beam filamentation. Here we investigate the situation where a positive feedback loop is present in the system leading to a pattern-forming instability. We stress that the resulting spatial structures are encoded also in the spatial density distribution, effectively leading to the self-assembly of an optical atomic lattice.
Recent years have witnessed considerable interest in simulating the dynamics of complex many-body systems by well-controlled cold atom model systems. Among others, magnetic ordering phenomena draw a lot of attention. We demonstrated an unconventional approach to light mediated atomic interactions using laser light undergoing diffraction [1]. Diffractive propagation of periodically modulated light fields leads to an exchange between phase and amplitude modulated planes (Talbot effect) which can be used to couple atomic degrees of freedom. In a feedback scheme this can lead to the spontaneous formation of coupled lattices in the light field and the atomic degrees of freedom. After adiabatic elimination of the dynamics of the light field, one is left with light mediated atomic interactions. The coupling can occur via optomechanical nonlinearities [1] or via optical pumping [2]. In the latter case, the result is a spontaneous magnetic ordering in the atomic cloud, a spin or a magnetic dipole pattern [2]. We will provide further details on the latter as well as evidence for novel alignment patterns, corresponding to quadrupole states.
The study of transverse optical pattern formation has been studied extensively in nonlinear optics, with a recent experimental interest in studying the phenomenon using cold atoms, which can undergo real-space self-organization. Here, we describe our experimental observation of pattern formation in cold atoms, which occurs using less than 1 μW of applied power. We show that the optical patterns and the self-organized atomic structures undergo continuous symmetry breaking, which is characteristic of nonequilibrium phenomena in a multimode system. To theoretically describe pattern formation in cold atoms, we present a self-consistent model that allows for tight atomic bunching in the applied optical lattice. We derive the nonlinear refractive index of a gas of multilevel atoms in an optical lattice, and we derive the threshold conditions under which pattern formation occurs. We show that by using small detunings and sub-Doppler temperatures, one achieves intensity thresholds for pattern formation that are reduced by two orders of magnitude compared to warm atoms.
Summary form only given. Spontaneous optical pattern formation occurs in a variety of nonlinear systems [1], including hot atomic vapors [2]. On the other hand, the spatial self-organization of atomic ensembles due to opto-mechanical coupling has received a lot of interest in recent years [3].We report on the observation of transverse self-organization of a cold atomic cloud (issued from a magnetooptical trap) under the action of a single pump laser beam. Two symmetries (translation and rotation) in the plane orthogonal to the beam propagation direction are spontaneously broken. We use a simple optical feedback scheme [4], where the transmitted pump beam is retro-reflected to the atoms by a high-reflectivity mirror located at a distance d behind the cloud. This feedback loop transforms phase fluctuations of the transmitted wave into intensity fluctuations, which then react on the atomic medium. If the feedback is positive, a transverse instability can develop leading to the spontaneous apparition of patterns in the transmitted pump intensity profile, as shown in the figure below (left).Using a weak probe beam sent a few tens of μs after the e,tinction of the pump, we demonstrate that the instability also results in a transverse spatial ordering of the atomic medium as shown in the right image. The cold atoms thus e,perience strong spatial bunching due to the dipole force associated to the inhomogeneous intensity distribution. We identified two different instability regimes. For short pump durations (- 1 μs), high pump intensity and cloud optical density, the instability relies on the Kerr effect (electronic nonlinearity). For longer pump durations (- 100 μs), the instability is driven by the opto-mechanical effect, resulting in lower intensity and optical density thresholds than for the electronic nonlinearity. These observations are well reproduced by a theoretical model including the coupled dynamics of the light field and the atomic e,ternal degrees of freedom.
Self-organized phases in cold atoms as a result of light-mediated interactions can be induced by coupling to internal or external degrees of the atoms. There has been growing interest in the interaction of internal spin degrees of freedom with the optomechanical dynamics of the external center-of-mass motion. We present a model for the coupling between magnetic and optomechanical structuring in a $J=1/2\ensuremath{\rightarrow}{J}^{\ensuremath{'}}=3/2$ system in a single-mirror feedback scheme, which is representative of a larger class of diffractively coupled systems such as longitudinally pumped cavities and counterpropagating-beam schemes. For negative detunings, a linear stability analysis demonstrates that optical pumping and optomechanical driving cooperate to create magnetic ordering. However, for long-period transmission gratings the magnetic driving will strongly dominate the optomechanical driving, unless one operates very close to the existence range of the magnetic instability. At small lattice periods, in particular at wavelength-scale periods, the optomechanical driving will dominate.