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arXiv:1603.06280 · Journal of the Optical Society of America B

Transverse optical and atomic pattern formation

Bonnie L. Schmittberger, Daniel J. Gauthier

Published Jun 24, 2016• 10 citations
arXivHTMLPDF

Abstract

The study of transverse optical pattern formation has been studied extensively in nonlinear optics, with a recent experimental interest in studying the phenomenon using cold atoms, which can undergo real-space self-organization. Here, we describe our experimental observation of pattern formation in cold atoms, which occurs using less than 1 μW of applied power. We show that the optical patterns and the self-organized atomic structures undergo continuous symmetry breaking, which is characteristic of nonequilibrium phenomena in a multimode system. To theoretically describe pattern formation in cold atoms, we present a self-consistent model that allows for tight atomic bunching in the applied optical lattice. We derive the nonlinear refractive index of a gas of multilevel atoms in an optical lattice, and we derive the threshold conditions under which pattern formation occurs. We show that by using small detunings and sub-Doppler temperatures, one achieves intensity thresholds for pattern formation that are reduced by two orders of magnitude compared to warm atoms.

DOI
10.1364/josab.33.001543

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The study of transverse optical pattern formation has been studied extensively in nonlinear optics, with a recent experimental interest in studying the phenomenon using cold atoms, which can undergo real-space self-organization. Here, we describe our experimental observation of pattern formation in cold atoms, which occurs using less than 1 μW of applied power. We show that the optical patterns and the self-organized atomic structures undergo continuous symmetry breaking, which is characteristic of nonequilibrium phenomena in a multimode system. To theoretically describe pattern formation in cold atoms, we present a self-consistent model that allows for tight atomic bunching in the applied optical lattice. We derive the nonlinear refractive index of a gas of multilevel atoms in an optical lattice, and we derive the threshold conditions under which pattern formation occurs. We show that by using small detunings and sub-Doppler temperatures, one achieves intensity thresholds for pattern formation that are reduced by two orders of magnitude compared to warm atoms.
The nonlinear interaction between light and atoms is an extensive field of study with a broad range of applications in quantum information science and condensed matter physics. Nonlinear optical phenomena occurring in cold atoms are particularly interesting because such slowly moving atoms can spatially organize into density gratings, which allows for studies involving optical interactions with structured materials. In this thesis, I describe a novel nonlinear optical effect that arises when cold atoms spatially bunch in an optical lattice. I show that employing this spatial atomic bunching provides access to a unique physical regime with reduced thresholds for nonlinear optical processes and enhanced material properties. Using this method, I observe the nonlinear optical phenomenon of transverse optical pattern formation at record-low powers. These transverse optical patterns are generated by a wave- mixing process that is mediated by the cold atomic vapor. The optical patterns are highly multimode and induce rich non-equilibrium atomic dynamics. In particular, I find that there exists a synergistic interplay between the generated optical pat- terns and the atoms, wherein the scattered fields help the atoms to self-organize into new, multimode structures that are not externally imposed on the atomic sample. These self-organized structures in turn enhance the power in the optical patterns. I provide the first detailed investigation of the motional dynamics of atoms that have self-organized in a multimode geometry. I also show that the transverse optical patterns induce Sisyphus cooling in all three spatial dimensions, which is the first observation of spontaneous three-dimensional cooling. My experiment represents a unique means by which to study nonlinear optics and non-equilibrium dynamics at ultra-low required powers.
Summary form only given. Spontaneous optical pattern formation occurs in a variety of nonlinear systems [1], including hot atomic vapors [2]. On the other hand, the spatial self-organization of atomic ensembles due to opto-mechanical coupling has received a lot of interest in recent years [3].We report on the observation of transverse self-organization of a cold atomic cloud (issued from a magnetooptical trap) under the action of a single pump laser beam. Two symmetries (translation and rotation) in the plane orthogonal to the beam propagation direction are spontaneously broken. We use a simple optical feedback scheme [4], where the transmitted pump beam is retro-reflected to the atoms by a high-reflectivity mirror located at a distance d behind the cloud. This feedback loop transforms phase fluctuations of the transmitted wave into intensity fluctuations, which then react on the atomic medium. If the feedback is positive, a transverse instability can develop leading to the spontaneous apparition of patterns in the transmitted pump intensity profile, as shown in the figure below (left).Using a weak probe beam sent a few tens of μs after the e,tinction of the pump, we demonstrate that the instability also results in a transverse spatial ordering of the atomic medium as shown in the right image. The cold atoms thus e,perience strong spatial bunching due to the dipole force associated to the inhomogeneous intensity distribution. We identified two different instability regimes. For short pump durations (- 1 μs), high pump intensity and cloud optical density, the instability relies on the Kerr effect (electronic nonlinearity). For longer pump durations (- 100 μs), the instability is driven by the opto-mechanical effect, resulting in lower intensity and optical density thresholds than for the electronic nonlinearity. These observations are well reproduced by a theoretical model including the coupled dynamics of the light field and the atomic e,ternal degrees of freedom.
The spontaneous formation of patterns in dynamical systems is a rich phenomenon that transcends scientific boundaries. Here, we report our observation of coupled optical–atomic pattern formation, which results in the creation of self-organized, multimode structures in free-space laser-driven cold atoms. We show that this process gives rise to spontaneous three-dimensional Sisyphus cooling even at very low light intensities and the emergence of self-organized structures on both sub- and super-wavelength scales.
Cold atomic clouds constitute highly resonant nonlinear optical media, whose refractive index can easily be tuned via the light frequency. When subjected to a retroreflected laser beam and under appropriate conditions, the cloud undergoes spontaneous symmetry breaking, and spatial patterns develop in the transverse cross section of the beam. We investigate the impact of the sign of the light detuning from the atomic resonance on these patterns, thus directly comparing pattern formation for self-focusing and self-defocusing nonlinearities. Our observations emphasize the need for a ``diffractively thick'' medium description of the light-cloud interaction in which diffraction and nonlinear propagation inside the sample are taken into account.
We report a new nonlinear optical process that occurs in a cloud of cold atoms at low-light-levels when the incident optical fields simultaneously polarize, cool, and spatially-organize the atoms. We observe an extremely large effective fifth-order nonlinear susceptibility of χ(⁵) = 7.6 × 10⁻¹⁵ (m/V)⁴, which results in efficient Bragg scattering via six-wave mixing, slow group velocities (∼ c/10⁵), and enhanced atomic coherence times (> 100 μs). In addition, this process is particularly sensitive to the atomic temperatures, and provides a new tool for in-situ monitoring of the atomic momentum distribution in an optical lattice. For sufficiently large light-matter couplings, we observe an optical instability for intensities as low as ∼ 1 mW/cm² in which new, intense beams of light are generated and result in the formation of controllable transverse optical patterns.