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Journal of Experimental and Theoretical Physics Letters

Ultrashort Optical Pulses and Their Generation in Resonant Media (Scientific Summary)

Rostislav M. Arkhipov, Mikhail V. Arkhipov, A. A. Shimko, A. V. Pakhomov, Nikolay N. Rosanov

Published Jul 1, 2019• 49 citations

Abstract

Our recent studies of methods for obtaining ultrashort light pulses and analysis of the impact of ultrashort optical pulses on classical and quantum micro-objects with the identification of the determining role of the degree of unipolarity of pulses (maximum for strictly unipolar pulses) in the efficiency of direct laser acceleration of charged particles and excitation of atoms and molecules have been reviewed. Special attention has been paid to the coherent mode locking regime in lasers, which is implemented when the laser pulse duration is less than the relaxation time of the working transition in media with resonance amplification and absorption (laser analog of the phenomenon of self-induced transparency). Experimental data on coherent mode locking in a titanium-sapphire laser with a cell with rubidium vapor at self-induced transparency in rubidium have been presented. The interaction of ultrashort pulses in resonant media has also been analyzed.

DOI: 10.1134/s0021364019130071

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A review is given of the investigations of the coherent interaction of light pulses with resonantly absorbing two-level media. An analysis is made of the self-induced transparency discovered by McCall and Hahn and of its importance in quantum electronics. Bleached states associated with the phase modulation are considered in detail. A comparison is made with the theory of nonlinear waves of different physical origin. A review is given of some possible physical applications associated with the discriminatory nature of the transmission and delay of light in the self-induced transparency effect.

Resonant and near-resonant two-photon excitations with ultrashort laser pulses of forbidden atomic transitions give access to a wide class of nonlinear-optical processes such as two-photon absorption, stimulated Raman scattering, four-wave sum- and difference-frequency mixing. The latter has proofed to be a powerful tool for efficient femtosecond pulse generation in the VUV-spectral range [1]. Nevertheless, up to now only few experimental results have been obtained which allow the direct observation of the coherent dynamics in two-photon induced radiation-matter interactions (see experimental papers [2-5] and monograph [6]).

Exact single-soliton solutions of the modified system of Maxwell-Bloch equations, in which the dipole-dipole interactions of the atoms of a dense resonant medium are taken into account, are obtained. Two propagation regimes are analyzed: “coherent,” where the pulse duration is much shorter than both relaxation times ( T p ≪ T 1 , T 2 ), and “incoherent,” where the pulse duration falls between the relaxation times ( T 2 ≪ T p ≪ T 1 ). It is predicted, for the first time, that soliton propagation of an ultrashort pulse is possible in a dense resonant absorbing medium in an incoherent interaction regime. The differences between the amplitude and phase characteristics of the solitons considered and the corresponding characteristics of the solitons for McCall-Hahn self-induced transparency are noted.

Abstract We study the interaction of two counterpropagating unipolar video pulses of electromagnetic radiation in a dense resonant two-level medium. The pulse durations are less than one oscillation period of an atomic transition. We show that a polariton cluster (i.e. the compact long-living strongly coupled state of electromagnetic field and matter polarization) is created, when two unipolar pulses collide in a resonant medium of the frequency ω0 (the pulses correspond to self-induced transparency solitons of the same amplitudes and opposite polarities). We have studied for the first time the conditions of maximal excitation of a resonant polarization in the polariton cluster volume. We show that there exist optimal durations and amplitudes of the recording pulses. We studied the processes of double and multiple recording and erasing of an optical memory cell in a thin layer of a resonant medium (quantum dots). We demonstrated that the pulse rate of the recording-erasing pulses can reach 60 000 GHz and higher, which happens under the coherent regime of the interaction between the electromagnetic field and polarization of the medium.

A review is given of recent theoretical investigations on coherent propagation and nonlinear interaction of multifrequency ultrashort radiation pulses in resonantly absorbing media. An analysis is made of frequency conversion by parametric interaction and stimulated Raman scattering of laser pulses in resonant three-level media. New ways of controlling the parameters of coherent pulses and the use of multifrequency pulses in the spectroscopy of multilevel media are discussed. The experimental capabilities of the investigated effects are considered.