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Scientific Reports

Single electron-photon pair creation from a single polarization-entangled photon pair

Kazuyuki Kuroyama, Marcus Larsson, Sadashige Matsuo, Takafumi Fujita, Sascha R. Valentin, Arne Ludwig, Andreas Dirk Wieck, A. Oiwa, Seigo Tarucha

Published Nov 29, 2017• 12 citations
Publisher

Abstract

Quantum entanglement between different forms of qubits is an indication of the universality of quantum mechanics. Entanglement transfer between light and matter, especially photon and spin, has long been studied as the central concept, but it remains technically challenging for single photons and spins. In this paper, we show paired generation of a single electron in a GaAs quantum dot and a single photon from a single polarization-entangled photon pair. We measure temporal coincidence between the single photo-electron detection and the single photon detection. Considering a single photon polarization is converted to an electron spin via an optical selection rule, the present result indicates the capability of photon to spin entanglement transfer. This may be useful to explore the physics of entanglement transfer and also for applications to quantum teleportation based quantum communication.

DOI
10.1038/s41598-017-16899-w

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Quantum entanglement between different forms of qubits is an indication of the universality of quantum mechanics. Entanglement transfer between light and matter, especially photon and spin, has long been studied as the central concept, but it remains technically challenging for single photons and spins. In this paper, we show paired generation of a single electron in a GaAs quantum dot and a single photon from a single polarization-entangled photon pair. We measure temporal coincidence between the single photo-electron detection and the single photon detection. Considering a single photon polarization is converted to an electron spin via an optical selection rule, the present result indicates the capability of photon to spin entanglement transfer. This may be useful to explore the physics of entanglement transfer and also for applications to quantum teleportation based quantum communication.
We demonstrate paired generation of a single photo-electron in a quantum dot and a single photon from a single polarization-entangled photon pair that is generated by spontaneous parametric down conversion. The electron is reated in a GaAs quantum dot via inter-band resonantexcitation by irradiating one of the paired photons on the dot, while the remaining photon is detected by a single photon counter. Because the paired photons are generated simultaneously, the photo-electron and the remaining photon should be observed as a coincident event if the traveling distance is equivalent between them. The coincidence is probabilistic due to the probabilistic generation of the paired photon. We observe the probability of finding the photon with the photo-electron detection substantially higher then that without the photo-electron detection and derive the coincident rate comparable to the emission rate of the original photon pairs.
We show that electron recombination using positively charged excitons in single quantum dots provides an efficient method to transfer entanglement from electron spins onto photon polarizations. We propose a scheme for the production of entangled four-photon states of GHZ type. From the GHZ state, two fully entangled photons can be obtained by a measurement of two photons in the linear polarization basis, even for quantum dots with observable fine structure splitting for neutral excitons and significant exciton spin decoherence. Because of the interplay of quantum mechanical selection rules and interference, maximally entangled electron pairs are converted into maximally entangled photon pairs with unity fidelity for a continuous set of observation directions. We describe the dynamics of the conversion process using a master-equation approach and show that the implementation of our scheme is feasible with current experimental techniques.
We show that electron recombination in spin light-emitting diodes provides an efficient method to transfer entanglement from electron spins onto pairs of polarization-entangled photons. Because of the interplay of quantum mechanical selection rules and interference, maximally entangled electron pairs are converted into maximally entangled photon pairs with unity fidelity for a continuous set of observation directions. We describe the dynamics of the conversion process using a master-equation approach and show that the implementation of our scheme is feasible with current experimental techniques.
We investigate entanglement transfer from a system of two spin-entangled electron-hole pairs, each placed in a separate single mode cavity, to the photons emitted due to cavity leakage. Dipole selection rules and a splitting between the light hole and the heavy hole subbands are the crucial ingredients establishing a one-to-one correspondence between electron spins and circular photon polarizations. To account for the measurement of the photons as well as dephasing effects, we choose a stochastic Schrödinger equation and a conditional master equation approach, respectively. The influence of interactions with the environment as well as asymmetries in the coherent couplings on the photon entanglement is analysed for two concrete measurement schemes. The first one is designed to violate the Clauser-Horne-Shimony-Holt (CHSH) inequality, while the second one employs the visibility of interference fringes to prove the entanglement of the photons. Because of the spatial separation of the entangled electronic system over two quantum dots, a successful verification of entangled photons emitted by this system would imply the detection of nonlocal spin entanglement of massive particles in a solid state structure.
Entanglement plays a central role in fundamental tests of quantum mechanics as well as in the burgeoning field of quantum information processing. Particularly in the context of quantum networks and communication, an outstanding challenge is the efficient generation of entanglement between stationary (spin) and flying (photon) qubits. In this talk, I will first show the observation of quantum entanglement between a semiconductor quantum dot spin and the color of a propagating optical photon [1]. The demonstration of entanglement relies on the use of fast single-photon detection which allows us to project the photon into a superposition of its two frequency components. Our results extend the previous demonstrations of single-spin-photon entanglement in trapped ions, neutral atoms and nitrogen vacancy centers to the domain of artificial atoms in semiconductor nano-structures that allow for integration of electronic and photonic elements.
Quantum state transfer from flying photons to stationary matter qubits is an important element in the realization of quantum networks. Self-assembled semiconductor quantum dots provide a promising solid-state platform hosting both single photon and spin, with an inherent light-matter interface. Here, we develop a method to coherently and actively control the single-photon frequency bins in superposition using electro-optic modulators, and measure the spin-photon entanglement with a fidelity of 0.796±0.020. Further, by Greenberger-Horne-Zeilinger-type state projection on the frequency, path, and polarization degrees of freedom of a single photon, we demonstrate quantum state transfer from a single photon to a single electron spin confined in an InGaAs quantum dot, separated by 5 m. The quantum state mapping from the photon's polarization to the electron's spin is demonstrated along three different axes on the Bloch sphere, with an average fidelity of 78.5%.