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Entanglement transfer from electron spins to photons

Verónica Cerletti, Oliver Gywat, Daniel Loss

Published Nov 9, 2004• 0 citations
OpenAlex

Abstract

We show that electron recombination in spin light-emitting diodes provides an efficient method to transfer entanglement from electron spins onto pairs of polarization-entangled photons. Because of the interplay of quantum mechanical selection rules and interference, maximally entangled electron pairs are converted into maximally entangled photon pairs with unity fidelity for a continuous set of observation directions. We describe the dynamics of the conversion process using a master-equation approach and show that the implementation of our scheme is feasible with current experimental techniques.

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Coherent transfer of spin and entanglement in optoelectronics

Verónica Cerletti

In the last few years there has been a growing interest in the possible applications of quantum properties of different physical systems in well established technologies. This was motivated by the miniaturization of electronic devices. For very small systems, the laws of quantum mechanics start to govern their behavior and it is then to expect that for instance electronic components reach their "quantum limit". A good example of the introduction of quantum properties into conventional technologies is the case of the electron spin, which offers an alternative to electron-charge for the storage and transport of information in electronics. The idea of using electron spins in electronics gave rise to the new and exciting field of spintronics and was encouraged by experiments that showed coherent spin transport over long distances (over hundred micrometers) in semiconductors and long electron spin dephasing times. In addition to its applications in conventional technologies, the use of the electron spin as information-carrier has been suggested for the new field of quantum information processing. An important advantage of the electron spin with respect to other quantum information-carriers proposed is that it can profit from the well developed semiconductor industry and its related technologies. For the long-range transport of information, however, the highly interacting environment in solid-state devices represents a difficulty to the use of electron spins. In contrast, photons are very weekly coupled to their environment, and therefore more suitable for the transfer of information over long distances (on the order of kilometers), required, for instance, in quantum communication. Furthermore, the technology needed for the transport of photons over such long distances is well developed. Thus, an efficient transfer of quantum information between electron spins and photons is highly desirable. \n \nIn this dissertation, we show that the transfer of entanglement, a quantum correlation, from electron spins to the polarization of photons is not only theoretically possible, but also feasible under realistic experimental conditions. We study the transport of an entangled pair of electron spins through Fermi leads which split them spatially until they reach spin-LEDs, semiconductor structures containing quantum dots. In these structures, the electrons optically recombine with holes, producing then photons. We analyze the polarization state of the out-coming photons and give the conditions for which the entanglement of the electron spins is fully recovered in the photon-polarizations. We further show that it is possible to produce four-photon entanglement. \n \nWe also include in this work the study of coherent spin-transfer between quantum dots layers bridged by molecules. This study was motivated by an experiment showing that the molecules act not only as binders to construct the multilayer structures, but also as "wires" for the information through electron spins in the quantum dots. We show that a two-site Hamiltonian captures some of the essential features of the experiment. We calculate the dependence of the experimentally observed Faraday rotation (FR) signal as a function of probe energy on microscopic parameters such as spin transfer probabilities. The Faraday angle is related to the difference in the dielectric response for different polarizations of the light. We calculate the dielectric response functions of coupled quantum dots and derive an analytical expression for the FR angle in terms of electron transfer probabilities and Heisenberg exchange splittings.

•Jan 1, 2005•0 citations
We show that electron recombination in spin light-emitting diodes provides an efficient method to transfer entanglement from electron spins onto pairs of polarization-entangled photons. Because of the interplay of quantum mechanical selection rules and interference, maximally entangled electron pairs are converted into maximally entangled photon pairs with unity fidelity for a continuous set of observation directions. We describe the dynamics of the conversion process using a master-equation approach and show that the implementation of our scheme is feasible with current experimental techniques.
We show that electron recombination using positively charged excitons in single quantum dots provides an efficient method to transfer entanglement from electron spins onto photon polarizations. We propose a scheme for the production of entangled four-photon states of GHZ type. From the GHZ state, two fully entangled photons can be obtained by a measurement of two photons in the linear polarization basis, even for quantum dots with observable fine structure splitting for neutral excitons and significant exciton spin decoherence. Because of the interplay of quantum mechanical selection rules and interference, maximally entangled electron pairs are converted into maximally entangled photon pairs with unity fidelity for a continuous set of observation directions. We describe the dynamics of the conversion process using a master-equation approach and show that the implementation of our scheme is feasible with current experimental techniques.
Quantum entanglement between different forms of qubits is an indication of the universality of quantum mechanics. Entanglement transfer between light and matter, especially photon and spin, has long been studied as the central concept, but it remains technically challenging for single photons and spins. In this paper, we show paired generation of a single electron in a GaAs quantum dot and a single photon from a single polarization-entangled photon pair. We measure temporal coincidence between the single photo-electron detection and the single photon detection. Considering a single photon polarization is converted to an electron spin via an optical selection rule, the present result indicates the capability of photon to spin entanglement transfer. This may be useful to explore the physics of entanglement transfer and also for applications to quantum teleportation based quantum communication.
We investigate entanglement transfer from a system of two spin-entangled electron-hole pairs, each placed in a separate single mode cavity, to the photons emitted due to cavity leakage. Dipole selection rules and a splitting between the light hole and the heavy hole subbands are the crucial ingredients establishing a one-to-one correspondence between electron spins and circular photon polarizations. To account for the measurement of the photons as well as dephasing effects, we choose a stochastic Schrödinger equation and a conditional master equation approach, respectively. The influence of interactions with the environment as well as asymmetries in the coherent couplings on the photon entanglement is analysed for two concrete measurement schemes. The first one is designed to violate the Clauser-Horne-Shimony-Holt (CHSH) inequality, while the second one employs the visibility of interference fringes to prove the entanglement of the photons. Because of the spatial separation of the entangled electronic system over two quantum dots, a successful verification of entangled photons emitted by this system would imply the detection of nonlocal spin entanglement of massive particles in a solid state structure.
We propose a unique scheme to generate entangled photon pairs by six semiconductor quantum dots in a structure of quantum cellular automata. By means of interdot electronic tunneling, single-electron spin manipulation, and auxiliary excitons, we can convert the entanglement from the charge degrees of freedom of the electrons to the spin degrees of freedom of the electrons, and then to the polarization of the photons. Our scheme presents a source of entangled photon pairs without using spin–spin coupling, which could work repeatedly, deterministically and efficiently. Both the experimental challenge and the feasibility with present technologies are discussed. In comparison with former relevant work, our proposal not only gives an alternative method to generate entangled photons, but is applicable to other quantum information processing tasks with free electrons.
The entanglement transfer from electrons localized in a pair of quantum dots to circularly polarized photons is governed by optical selection rules, enforced by conservation of angular momentum. We point out that the transfer cannot be achieved by means of unitary evolution unless the angular momentum of the two initial qubit states differs by 2 units of ℏ. In particular, for spin-entangled electrons, the difference in angular momentum is 1 unit—so the transfer fails. Nevertheless, the transfer can be successfully completed if the unitary evolution is followed by a measurement of the angular momentum of each quantum dot and post-processing of the photons using the measured values as input.
In the last few years there has been a growing interest in the possible applications of quantum properties of different physical systems in well established technologies. This was motivated by the miniaturization of electronic devices. For very small systems, the laws of quantum mechanics start to govern their behavior and it is then to expect that for instance electronic components reach their "quantum limit". A good example of the introduction of quantum properties into conventional technologies is the case of the electron spin, which offers an alternative to electron-charge for the storage and transport of information in electronics. The idea of using electron spins in electronics gave rise to the new and exciting field of spintronics and was encouraged by experiments that showed coherent spin transport over long distances (over hundred micrometers) in semiconductors and long electron spin dephasing times. In addition to its applications in conventional technologies, the use of the electron spin as information-carrier has been suggested for the new field of quantum information processing. An important advantage of the electron spin with respect to other quantum information-carriers proposed is that it can profit from the well developed semiconductor industry and its related technologies. For the long-range transport of information, however, the highly interacting environment in solid-state devices represents a difficulty to the use of electron spins. In contrast, photons are very weekly coupled to their environment, and therefore more suitable for the transfer of information over long distances (on the order of kilometers), required, for instance, in quantum communication. Furthermore, the technology needed for the transport of photons over such long distances is well developed. Thus, an efficient transfer of quantum information between electron spins and photons is highly desirable. \n \nIn this dissertation, we show that the transfer of entanglement, a quantum correlation, from electron spins to the polarization of photons is not only theoretically possible, but also feasible under realistic experimental conditions. We study the transport of an entangled pair of electron spins through Fermi leads which split them spatially until they reach spin-LEDs, semiconductor structures containing quantum dots. In these structures, the electrons optically recombine with holes, producing then photons. We analyze the polarization state of the out-coming photons and give the conditions for which the entanglement of the electron spins is fully recovered in the photon-polarizations. We further show that it is possible to produce four-photon entanglement. \n \nWe also include in this work the study of coherent spin-transfer between quantum dots layers bridged by molecules. This study was motivated by an experiment showing that the molecules act not only as binders to construct the multilayer structures, but also as "wires" for the information through electron spins in the quantum dots. We show that a two-site Hamiltonian captures some of the essential features of the experiment. We calculate the dependence of the experimentally observed Faraday rotation (FR) signal as a function of probe energy on microscopic parameters such as spin transfer probabilities. The Faraday angle is related to the difference in the dielectric response for different polarizations of the light. We calculate the dielectric response functions of coupled quantum dots and derive an analytical expression for the FR angle in terms of electron transfer probabilities and Heisenberg exchange splittings.