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Polychromatic, continuous-wave mirrorless lasing from monochromatic pumping of cesium vapor

D. Antypas, Oleg Tretiak, Dmitry Budker, A. M. Akulshin

Published Jan 1, 2019• 19 citations
OpenAlex

Abstract

We report on the studies of simultaneous continuous-wave mirrorless lasing on multiple optical transitions, realized by pumping hot cesium (Cs) vapor with laser light resonant with the 6S1/2→8P3/2 transition. The multiplicity of the decay paths for the excited atoms to their ground state is responsible for the emergence of lasing in a number of transitions, observed here in at least seven wavelengths in the infrared and at two wavelengths in the blue. We study the properties of the fields generated in the Cs vapor such as optical power, directionality, and optical linewidth.

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We report on the studies of simultaneous continuous-wave mirrorless lasing on multiple optical transitions, realized by pumping hot cesium (Cs) vapor with laser light resonant with the 6S1/2→8P3/2 transition. The multiplicity of the decay paths for the excited atoms to their ground state is responsible for the emergence of lasing in a number of transitions, observed here in at least seven wavelengths in the infrared and at two wavelengths in the blue. We study the properties of the fields generated in the Cs vapor such as optical power, directionality, and optical linewidth.

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We report on observations of coherent, sustained oscillations in the absorption of continuous-wave light at 388 nm that excites the 6 S 1/2 → 8 P 3/2 transition in cesium (Cs) vapor. The oscillation frequency is close to the spacing of hyperfine levels of the 8 P 3/2 level that are excited simultaneously by the 388 nm field. We observe a threshold behavior of the oscillation amplitude with pump power and suggest that the effect is associated with infrared directional emission due to amplified spontaneous emission (ASE) from the 8 P 3/2 → 8 S 1/2 transition that is assisted by retro-reflections from cell windows. The effect may be used to probe a lasing process in an atomic vapor, by checking the temporal properties of the pump field transmitted through the vapor.

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We demonstrate the generation of coherent and collimated blue light (CBL) based on cesium (Cs) 6S1/2(F = 4)→6P3/2(F' = 5)→6D5/2(F'' = 6)→7P3/2(F' = 5)→6S1/2(F = 4) diamond-type atomic system in a heated vapor cell. Two infrared pumping lasers with wavelengths at 852 nm (6S1/2→6P3/2) and 917 nm (6P3/2→6D5/2), provide step-wise excitation to the 6D5/2 excited state, and induce strong two-photon coherence between the 6S1/2 state and 6D5/2 state. The atoms undergo a double cascade accompanied with the amplified spontaneous emission at 15.1 μm via the 7P3/2 intermediate excited state, and produce a beam of 455 nm (7P3/2→6S1/2) CBL with highly spatiotemporal coherence through a parametric four-wave mixing process. We investigate the influence of experimental parameters such as polarization combination of the two pumping lasers, and their power, and the temperature of Cs vapor cell on the CBL. Especially, we add a beam of 894 nm laser operating at the 6S1/2(F = 3) →6P1/2 transition as repumping laser, which can pump atoms back to the 6S1/2(F = 4) state from the 6S1/2(F = 3) state, thus significantly improving the power of CBL. This technique of the CBL enhancement via optical pumping is also useful for the other alkali metal atoms.

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Mirrorless lasers avoid cavity-pulling effects by generating stimulated emission directly from an atomic gain medium without an optical cavity. However, most superradiant or superfluorescent emissions are transient, limiting their use as steady atom-referenced optical sources. Here, we demonstrate a continuous-wave dual-wavelength mirrorless laser in thermal rubidium vapor. A frequency-stabilized 420 nm laser pumps the 5S1/2→6P3/2 transition and generates directional infrared lasing at 1323 and 1367 nm through the non-cascaded 6S1/2→5P1/2 and 6S1/2→5P3/2 transitions. The emissions exhibit threshold-like pump-power dependence and a near-fundamental transverse mode, supporting CW mirrorless laser in a traveling-wave atomic gain medium. Heterodyne detection gives a 1367 nm linewidth of 32.5 kHz, which is 38 times narrower than the natural linewidth. This work establishes a linewidth-narrowed, cavity-free, atom-referenced dual-wavelength laser platform for precision spectroscopy, optical frequency references, and quantum sensing.

Applied Physics Letters•Jul 13, 2026•0 citations
We report on the studies of simultaneous continuous-wave mirrorless lasing on multiple optical transitions, realized by pumping hot cesium (Cs) vapor with laser light resonant with the 6S1/2→8P3/2 transition. The multiplicity of the decay paths for the excited atoms to their ground state is responsible for the emergence of lasing in a number of transitions, observed here in at least seven wavelengths in the infrared and at two wavelengths in the blue. We study the properties of the fields generated in the Cs vapor such as optical power, directionality, and optical linewidth.
We report on the studies of simultaneous continuous-wave mirrorless lasing on multiple optical transitions, realized by pumping hot cesium (Cs) vapor with laser light resonant with the 6S1/2→8P3/2 transition. The multiplicity of the decay paths for the excited atoms to their ground state is responsible for the emergence of lasing in a number of transitions, observed here in at least seven wavelengths in the infrared and at two wavelengths in the blue. We study the properties of the fields generated in the Cs vapor such as optical power, directionality, and optical linewidth.
Population inversion on the 7S1/2− 6P3/2transition of cesium atoms is built by 455 nm diode laser pumping, and continuous-wave (cw) lasing is observed without the feedback on the gain medium from cavity mirrors. The stimulated emission at 1.47 µm infrared wavelength is restricted to a narrow angle along the direction of propagation of the pumping laser. Evidence of threshold-like characteristic is demonstrated in the cw mirrorless lasing dependence on pumping laser detuning, atomic density, and pumping light intensity. This compact structure can be used to generate mirrorless laser in a number of infrared wavelengths applied for the communication area. Moreover, it is expected to realize the narrow-linewidth optical frequency standard from an ultralow-finesse optical cavity.
We report on observations of coherent, sustained oscillations in the absorption of continuous-wave light at 388 nm that excites the 6 S 1/2 → 8 P 3/2 transition in cesium (Cs) vapor. The oscillation frequency is close to the spacing of hyperfine levels of the 8 P 3/2 level that are excited simultaneously by the 388 nm field. We observe a threshold behavior of the oscillation amplitude with pump power and suggest that the effect is associated with infrared directional emission due to amplified spontaneous emission (ASE) from the 8 P 3/2 → 8 S 1/2 transition that is assisted by retro-reflections from cell windows. The effect may be used to probe a lasing process in an atomic vapor, by checking the temporal properties of the pump field transmitted through the vapor.
We demonstrate the generation of coherent and collimated blue light (CBL) based on cesium (Cs) 6S1/2(F = 4)→6P3/2(F' = 5)→6D5/2(F'' = 6)→7P3/2(F' = 5)→6S1/2(F = 4) diamond-type atomic system in a heated vapor cell. Two infrared pumping lasers with wavelengths at 852 nm (6S1/2→6P3/2) and 917 nm (6P3/2→6D5/2), provide step-wise excitation to the 6D5/2 excited state, and induce strong two-photon coherence between the 6S1/2 state and 6D5/2 state. The atoms undergo a double cascade accompanied with the amplified spontaneous emission at 15.1 μm via the 7P3/2 intermediate excited state, and produce a beam of 455 nm (7P3/2→6S1/2) CBL with highly spatiotemporal coherence through a parametric four-wave mixing process. We investigate the influence of experimental parameters such as polarization combination of the two pumping lasers, and their power, and the temperature of Cs vapor cell on the CBL. Especially, we add a beam of 894 nm laser operating at the 6S1/2(F = 3) →6P1/2 transition as repumping laser, which can pump atoms back to the 6S1/2(F = 4) state from the 6S1/2(F = 3) state, thus significantly improving the power of CBL. This technique of the CBL enhancement via optical pumping is also useful for the other alkali metal atoms.
Mirrorless lasers avoid cavity-pulling effects by generating stimulated emission directly from an atomic gain medium without an optical cavity. However, most superradiant or superfluorescent emissions are transient, limiting their use as steady atom-referenced optical sources. Here, we demonstrate a continuous-wave dual-wavelength mirrorless laser in thermal rubidium vapor. A frequency-stabilized 420 nm laser pumps the 5S1/2→6P3/2 transition and generates directional infrared lasing at 1323 and 1367 nm through the non-cascaded 6S1/2→5P1/2 and 6S1/2→5P3/2 transitions. The emissions exhibit threshold-like pump-power dependence and a near-fundamental transverse mode, supporting CW mirrorless laser in a traveling-wave atomic gain medium. Heterodyne detection gives a 1367 nm linewidth of 32.5 kHz, which is 38 times narrower than the natural linewidth. This work establishes a linewidth-narrowed, cavity-free, atom-referenced dual-wavelength laser platform for precision spectroscopy, optical frequency references, and quantum sensing.