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A Survey of Characteristics and Signatures of A Few Low-Temperature Phases of Quantum Matter

Daniel Ish

Published Jan 1, 2018• 0 citations
OpenAlex

Abstract

We study two distinct systems along a similar theme. In one, we present new theoretical studies of the optical properties of the $J_2$-$\\lambda$ model for the materieal FeSc$_2$S$_4$, which places it close to a quantum critical point on the disordered side of a quantum phase transition between a N\\'{e}el ordered phase and a ``Spin-Orbital Liquid" in which spins and orbitals are entangled, quenching the magnetization. We compute the dispersion relation for the quasiparticle excitations and the form of the collective response to electric field. We argue that the latter directly probes a low energy excitation continuum characteristic of quantum criticality, and that our results reinforce the consistency of this model with experiment. In the other, through a mixture of analytic and numerical techniques, we explore the optimal approximation by a free Majorana state to individual disorder realizations of the Sachdev-Ye-Kitaev model, along with a generalization of it. We elucidate the properties of the known time-reversal symmetry breaking phase in the generalized model, finding strong evidence of "spin glass" order. For the Sachdev-Ye-Kitaev model itself, our results are inconclusive but suggest a similar order may be present at $T = 0$.

Related papers

Quantum spin glasses and Sachdev-Ye-Kitaev models

Subir Sachdev A

A brief survey of some random quantum models with infinite-range couplings is presented, ranging from the quantum Ising model to the Sachdev-Ye-Kitaev model. The Sachdev-Ye-Kitaev model was the first to realize an extensive zero temperature entropy without requiring an exponentially large ground state degeneracy. This phenomenon is closely linked to the absence of a particle-like interpretation of its low energy spectrum--its spectral functions are not those of bosons or fermions but are instead "Planckian", meaning they are universal functions of energy/temperature. A remarkable consequence of these properties is that the SYK model provides an effective low energy theory of non-supersymmetric charged or rotating black holes in 3+1 dimensions, leading to new results on the density of many-body quantum states of such black holes. For applications to non-quasiparticle metallic states of quantum materials, an extension of the SYK model, known as the two-dimensional Yukawa-Sachdev-Ye-Kitaev model, is required. The 2dYSYK model describes quantum phase transitions in metals with spatial inhomogeneity in the position of the quantum critical point. This extension has led to a universal theory of the strange metal state observed in numerous correlated electron compounds, including copper-oxide based high temperature superconductors.

arXiv:2402.17824•Feb 27, 2024•1 citation

Sachdev-Ye-Kitaev Models and Beyond: A Window into Non-Fermi Liquids

Debanjan Chowdhury, Antoine Georges, Olivier Parcollet +1 more

We present a review of the Sachdev-Ye-Kitaev (SYK) model of compressible quantum many-body systems without quasiparticle excitations, and its connections to various theoretical studies of non-Fermi liquids in condensed matter physics. The review is placed in the context of numerous experimental observations on correlated electron materials. Strong correlations in metals are often associated with their proximity to a Mott transition to an insulator created by the local Coulomb repulsion between the electrons. We explore the phase diagrams of a number of models of such local electronic correlation, employing a dynamical mean field theory in the presence of random spin exchange interactions. Numerical analyses and analytical solutions, using renormalization group methods and expansions in large spin degeneracy, lead to critical regions which display SYK physics. The models studied include the single-band Hubbard model, the $t$-$J$ model and the two-band Kondo-Heisenberg model in the presence of random spin exchange interactions. We also examine non-Fermi liquids obtained by considering each SYK model with random four-fermion interactions to be a multi-orbital atom, with the SYK-atoms arranged in an infinite lattice. We connect to theories of sharp Fermi surfaces without any low-energy quasiparticles in the absence of spatial disorder, obtained by coupling a Fermi liquid to a gapless boson; a systematic large $N$ theory of such a critical Fermi surface, with SYK characteristics, is obtained by averaging over an ensemble of theories with random boson-fermion couplings. Finally, we present an overview of the links between the SYK model and quantum gravity and end with an outlook on open questions.

arXiv:2109.05037•Sep 10, 2021•14 citations

Universal Aspects of Quantum-Critical Dynamics in and Out of Equilibrium

Julia Steinberg

Quantum phase transitions occur strictly at zero temperature and are accessed by varying a physical parameter such as a magnetic field or chemical potential. While these transitions themselves are experimentally inaccessible, the existence of a zero temperature quantum critical point has remarkable effects on the dynamical properties of interacting quantum many-body systems at finite temperatures. In this thesis, we study dynamics in four strongly interacting many-body systems near quantum critical points in the context of NMR relaxation, quantum quenches, many-body quantum chaos, and charge diffusion. In chapter 1, we begin by revisiting the issue of NMR relaxation in the quantum disordered phase of Ising spin chains. We find that the imaginary part of the spin susceptibility at low frequences is dominated by rare quantum processes which leads to an NMR relaxation rate that scales as $1/T_{1}\sim \exp(-\frac{2\Delta}{T})$ near the quantum critical point rather than the previously conjectured $1/T_{1}\sim \exp(-\frac{\Delta}{T})$. These results resolve certain discrepancies between the energy scales measured with different experimental probes in the quantum disordered paramagnetic phase of the Ising chain system $\text{CoNb}_{2}\text{O}_{6}$. In chapter 2, we study the non-equilibrium dynamics of Sachdev-Ye-Kitaev (SYK) models with $q$ body interactions after a quantum quench, considering a quench protocol which drives the system from an initial state with long-lived quasiparticle excitations to a final state lacking any long-lived quasiparticle excitations. For $q=4$, we find that the timescale for the system to locally thermalize $\tau_{eq}\sim\frac{\hbar}{k_{B}T}$ and for $q\rightarrow \infty$ we find that the system thermalizes instantaneously. In chapter 3, we study the real time dynamics of quantum electrodynamics in 2+1 dimensions with $N_{f}$ flavors of fermions. We focus on thermalization and the onset of many-body quantum chaos and compute the quantum Lyapunov exponent in a $\frac{1}{N_{f}}$ expansion. We briefly comment on chaos, locality, and gauge invariance. Finally, in Chapter 4 we consider whether the butterfly velocity - a speed at which quantum information propagates - may provide a fundamental bound on diffusion constants in dirty incoherent metals by computing the charge diffusion constant and the butterfly velocity in charge-neutral holographic matter with long wavelength ``hydrodynamic" disorder. In this limit, we find that the butterfly velocity does not set a sharp lower bound for the charge diffusion constant.

•May 13, 2020•0 citations

Exploring Symmetry and Field-induced Phenomena in Kitaev Materials

Jacob Aaron Simmons Gordon

A large part of modern condensed matter concerns non-local or global properties of systems under the broad term of topology. Closely intertwined with certain senses of topology are symmetries of the system, which physically constrain our description and offer non-perturbative insights into material properties. The range of possible phases of matter is greatly enriched by quantum mechanics, including certain types of non-local entanglement that cannot be understood in the usual symmetry-breaking paradigm of local order parameters. Beyond weakly interacting topology we find the stronger notion of \textit{topological order} in correlated systems, a prominent example being the $S = \tfrac{1}{2}$ Kitaev honeycomb model in a weak magnetic field.Through a remarkable combination of lattice geometry, strong spin-orbit coupling, and electron interactions, several material candidates have been put forward to realize Kitaev physics, including the $4d$ Mott insulator $\alpha$-RuCl$_{3}$ which offers tantalizing experimental hints of topological order. In this thesis we explore several aspects of Kitaev candidates and related systems under two broad themes. One involves symmetry-informed and constrained observables, including a proposed singularity in a thermodynamic quantity accompanying phase transitions between two Ising topological orders (ITOs). The ITO physics realized by the Kitaev model requires time-reversal symmetry to be broken, and much of the non-trivial physics is found at finite magnetic field. To this end, we study a microscopic spin model appropriate for $\alpha$-RuCl$_{3}$ and show that it exhibits an interesting field-induced paramagnetic state between the low- and high-field magnetic orders, consistent with recent experimental findings. We determine several properties of a lower-dimensional spin-$S$ analogue of the Kitaev model, including a multi-critical point at finite field separating different topological phases. Finally, we derive quantum state purities of entangled photons emitted from a spin-triplet superconducting heterostructure and discuss its use in a new paradigm of entangled spectroscopy.

•Jun 1, 2023•0 citations

Low-dimensional quantum systems from novel constituents

Chengshu Li

Recent decades have seen a proliferation of unconventional quasiparticles in condensed matter systems. Majorana fermions, theoretically predicted in several setups and of great interest in topological quantum computation, are a focus of intense research efforts. Higher-spin moments, relevant for both solid-state compounds and cold atoms, are of great theoretical interest as they interpolate between the quantum and classical limits but sometimes show surprising behavior. In the meantime, successful fabrication and characterization of low-dimensional systems have brought new phenomenology and physical insights. In this dissertation I will theoretically explore a few low-dimensional models using Majorana fermions and higher-spin moments as building blocks. I will first discuss a generalized family of the celebrated Sachdev-Ye-Kitaev model, a zero-dimensional all-to-all Majorana model that exhibits non-Fermi liquid behavior and is holographically dual to a black hole. The generalized model has a phase transition between a non-Fermi liquid and a disordered Fermi liquid. Then I will discuss the Heisenberg model with higher spins, with a focus on chaos and information scrambling. Using matrix-product-state-based methods, we are able to obtain numerical results for spin up to 4 and characterize the Lyapunov growth. After that I will discuss a generalization of the Hubbard model to Majorana fermions on the honeycomb lattice. Unlike previous similar models, we find topological phases with (anti-)chiral edge modes for weak interaction. Finally I will show a construction of explicit supersymmetric Majorana model on the kagome lattice, where a family of exact solutions is found and the nature of supersymmetry breaking is explored.

•Jan 1, 2021•0 citations

Excitation spectra of quantum matter without quasiparticles. I. Sachdev-Ye-Kitaev models

Maria Tikhanovskaya, Haoyu Guo, Subir Sachdev A +1 more

We study the low-frequency spectra of complex Sachdev-Ye-Kitaev models at general densities. The analysis applies also to $\mathrm{SU}(M)$ magnets with random exchange at large $M$. The spectral densities are computed by numerical analysis of the saddle-point equations on the real frequency $\ensuremath{\omega}$ axis at zero temperature $T$. The asymptotic low-$\ensuremath{\omega}$ behaviors are found to be in excellent agreement with the scaling dimensions of irrelevant operators which perturb the conformally invariant critical states. Of possible experimental interest is our computation of the universal spin spectral weight of the $\mathrm{SU}(M)$ magnets at low $\ensuremath{\omega}$ and $T$; this includes a contribution from the time reparametrization mode, which is the boundary graviton of the holographic dual. This analysis is extended to a random $t\ensuremath{-}J$ model in the following paper [M. Tikhanovskaya et al., following paper, Phys. Rev. B 103, 075142 (2021)].

arXiv:2010.09742•Physical review. B./Physical review. B•Feb 24, 2021•34 citations
We study two distinct systems along a similar theme. In one, we present new theoretical studies of the optical properties of the J2J_2J2​-lambda\\lambdalambda model for the materieal FeSc2_22​S4_44​, which places it close to a quantum critical point on the disordered side of a quantum phase transition between a N\'{e}el ordered phase and a ``Spin-Orbital Liquid" in which spins and orbitals are entangled, quenching the magnetization. We compute the dispersion relation for the quasiparticle excitations and the form of the collective response to electric field. We argue that the latter directly probes a low energy excitation continuum characteristic of quantum criticality, and that our results reinforce the consistency of this model with experiment. In the other, through a mixture of analytic and numerical techniques, we explore the optimal approximation by a free Majorana state to individual disorder realizations of the Sachdev-Ye-Kitaev model, along with a generalization of it. We elucidate the properties of the known time-reversal symmetry breaking phase in the generalized model, finding strong evidence of "spin glass" order. For the Sachdev-Ye-Kitaev model itself, our results are inconclusive but suggest a similar order may be present at T=0T = 0T=0.
A brief survey of some random quantum models with infinite-range couplings is presented, ranging from the quantum Ising model to the Sachdev-Ye-Kitaev model. The Sachdev-Ye-Kitaev model was the first to realize an extensive zero temperature entropy without requiring an exponentially large ground state degeneracy. This phenomenon is closely linked to the absence of a particle-like interpretation of its low energy spectrum--its spectral functions are not those of bosons or fermions but are instead "Planckian", meaning they are universal functions of energy/temperature. A remarkable consequence of these properties is that the SYK model provides an effective low energy theory of non-supersymmetric charged or rotating black holes in 3+1 dimensions, leading to new results on the density of many-body quantum states of such black holes. For applications to non-quasiparticle metallic states of quantum materials, an extension of the SYK model, known as the two-dimensional Yukawa-Sachdev-Ye-Kitaev model, is required. The 2dYSYK model describes quantum phase transitions in metals with spatial inhomogeneity in the position of the quantum critical point. This extension has led to a universal theory of the strange metal state observed in numerous correlated electron compounds, including copper-oxide based high temperature superconductors.
We present a review of the Sachdev-Ye-Kitaev (SYK) model of compressible quantum many-body systems without quasiparticle excitations, and its connections to various theoretical studies of non-Fermi liquids in condensed matter physics. The review is placed in the context of numerous experimental observations on correlated electron materials. Strong correlations in metals are often associated with their proximity to a Mott transition to an insulator created by the local Coulomb repulsion between the electrons. We explore the phase diagrams of a number of models of such local electronic correlation, employing a dynamical mean field theory in the presence of random spin exchange interactions. Numerical analyses and analytical solutions, using renormalization group methods and expansions in large spin degeneracy, lead to critical regions which display SYK physics. The models studied include the single-band Hubbard model, the ttt-JJJ model and the two-band Kondo-Heisenberg model in the presence of random spin exchange interactions. We also examine non-Fermi liquids obtained by considering each SYK model with random four-fermion interactions to be a multi-orbital atom, with the SYK-atoms arranged in an infinite lattice. We connect to theories of sharp Fermi surfaces without any low-energy quasiparticles in the absence of spatial disorder, obtained by coupling a Fermi liquid to a gapless boson; a systematic large NNN theory of such a critical Fermi surface, with SYK characteristics, is obtained by averaging over an ensemble of theories with random boson-fermion couplings. Finally, we present an overview of the links between the SYK model and quantum gravity and end with an outlook on open questions.
Quantum phase transitions occur strictly at zero temperature and are accessed by varying a physical parameter such as a magnetic field or chemical potential. While these transitions themselves are experimentally inaccessible, the existence of a zero temperature quantum critical point has remarkable effects on the dynamical properties of interacting quantum many-body systems at finite temperatures. In this thesis, we study dynamics in four strongly interacting many-body systems near quantum critical points in the context of NMR relaxation, quantum quenches, many-body quantum chaos, and charge diffusion. In chapter 1, we begin by revisiting the issue of NMR relaxation in the quantum disordered phase of Ising spin chains. We find that the imaginary part of the spin susceptibility at low frequences is dominated by rare quantum processes which leads to an NMR relaxation rate that scales as 1/T1∼exp⁡(−2ΔT)1/T_{1}\sim \exp(-\frac{2\Delta}{T})1/T1​∼exp(−T2Δ​) near the quantum critical point rather than the previously conjectured 1/T1∼exp⁡(−ΔT)1/T_{1}\sim \exp(-\frac{\Delta}{T})1/T1​∼exp(−TΔ​). These results resolve certain discrepancies between the energy scales measured with different experimental probes in the quantum disordered paramagnetic phase of the Ising chain system CoNb2O6\text{CoNb}_{2}\text{O}_{6}CoNb2​O6​. In chapter 2, we study the non-equilibrium dynamics of Sachdev-Ye-Kitaev (SYK) models with qqq body interactions after a quantum quench, considering a quench protocol which drives the system from an initial state with long-lived quasiparticle excitations to a final state lacking any long-lived quasiparticle excitations. For q=4q=4q=4, we find that the timescale for the system to locally thermalize τeq∼ℏkBT\tau_{eq}\sim\frac{\hbar}{k_{B}T}τeq​∼kB​Tℏ​ and for q→∞q\rightarrow \inftyq→∞ we find that the system thermalizes instantaneously. In chapter 3, we study the real time dynamics of quantum electrodynamics in 2+1 dimensions with NfN_{f}Nf​ flavors of fermions. We focus on thermalization and the onset of many-body quantum chaos and compute the quantum Lyapunov exponent in a 1Nf\frac{1}{N_{f}}Nf​1​ expansion. We briefly comment on chaos, locality, and gauge invariance. Finally, in Chapter 4 we consider whether the butterfly velocity - a speed at which quantum information propagates - may provide a fundamental bound on diffusion constants in dirty incoherent metals by computing the charge diffusion constant and the butterfly velocity in charge-neutral holographic matter with long wavelength ``hydrodynamic" disorder. In this limit, we find that the butterfly velocity does not set a sharp lower bound for the charge diffusion constant.
A large part of modern condensed matter concerns non-local or global properties of systems under the broad term of topology. Closely intertwined with certain senses of topology are symmetries of the system, which physically constrain our description and offer non-perturbative insights into material properties. The range of possible phases of matter is greatly enriched by quantum mechanics, including certain types of non-local entanglement that cannot be understood in the usual symmetry-breaking paradigm of local order parameters. Beyond weakly interacting topology we find the stronger notion of \textit{topological order} in correlated systems, a prominent example being the S=12S = \tfrac{1}{2}S=21​ Kitaev honeycomb model in a weak magnetic field.Through a remarkable combination of lattice geometry, strong spin-orbit coupling, and electron interactions, several material candidates have been put forward to realize Kitaev physics, including the 4d4d4d Mott insulator α\alphaα-RuCl3_{3}3​ which offers tantalizing experimental hints of topological order. In this thesis we explore several aspects of Kitaev candidates and related systems under two broad themes. One involves symmetry-informed and constrained observables, including a proposed singularity in a thermodynamic quantity accompanying phase transitions between two Ising topological orders (ITOs). The ITO physics realized by the Kitaev model requires time-reversal symmetry to be broken, and much of the non-trivial physics is found at finite magnetic field. To this end, we study a microscopic spin model appropriate for α\alphaα-RuCl3_{3}3​ and show that it exhibits an interesting field-induced paramagnetic state between the low- and high-field magnetic orders, consistent with recent experimental findings. We determine several properties of a lower-dimensional spin-SSS analogue of the Kitaev model, including a multi-critical point at finite field separating different topological phases. Finally, we derive quantum state purities of entangled photons emitted from a spin-triplet superconducting heterostructure and discuss its use in a new paradigm of entangled spectroscopy.
Recent decades have seen a proliferation of unconventional quasiparticles in condensed matter systems. Majorana fermions, theoretically predicted in several setups and of great interest in topological quantum computation, are a focus of intense research efforts. Higher-spin moments, relevant for both solid-state compounds and cold atoms, are of great theoretical interest as they interpolate between the quantum and classical limits but sometimes show surprising behavior. In the meantime, successful fabrication and characterization of low-dimensional systems have brought new phenomenology and physical insights. In this dissertation I will theoretically explore a few low-dimensional models using Majorana fermions and higher-spin moments as building blocks. I will first discuss a generalized family of the celebrated Sachdev-Ye-Kitaev model, a zero-dimensional all-to-all Majorana model that exhibits non-Fermi liquid behavior and is holographically dual to a black hole. The generalized model has a phase transition between a non-Fermi liquid and a disordered Fermi liquid. Then I will discuss the Heisenberg model with higher spins, with a focus on chaos and information scrambling. Using matrix-product-state-based methods, we are able to obtain numerical results for spin up to 4 and characterize the Lyapunov growth. After that I will discuss a generalization of the Hubbard model to Majorana fermions on the honeycomb lattice. Unlike previous similar models, we find topological phases with (anti-)chiral edge modes for weak interaction. Finally I will show a construction of explicit supersymmetric Majorana model on the kagome lattice, where a family of exact solutions is found and the nature of supersymmetry breaking is explored.
We study the low-frequency spectra of complex Sachdev-Ye-Kitaev models at general densities. The analysis applies also to SU(M)\mathrm{SU}(M)SU(M) magnets with random exchange at large MMM. The spectral densities are computed by numerical analysis of the saddle-point equations on the real frequency $\ensuremath{\omega}$ axis at zero temperature TTT. The asymptotic low-$\ensuremath{\omega}$ behaviors are found to be in excellent agreement with the scaling dimensions of irrelevant operators which perturb the conformally invariant critical states. Of possible experimental interest is our computation of the universal spin spectral weight of the SU(M)\mathrm{SU}(M)SU(M) magnets at low $\ensuremath{\omega}$ and TTT; this includes a contribution from the time reparametrization mode, which is the boundary graviton of the holographic dual. This analysis is extended to a random $t\ensuremath{-}J$ model in the following paper [M. Tikhanovskaya et al., following paper, Phys. Rev. B 103, 075142 (2021)].