Most phenomena around us can be explained by classical optics since photons interact weakly with atoms. When the interaction is strong enough where one photon affects the properties of other photons, we go to the regime of quantum photon-photon nonlinear optics. The work in this thesis explores this regime of physics. This paves the path to exploring strongly interacting many-body physics with photons which is still a largely unexplored domain. The ability to control strongly interacting photons is also of central importance in quantum science and engineering. We use the approach of Electromagnetically Induced Transparency (EIT) in atomic ensembles to create strong interactions and demonstrate coherent control between single photons. Using EIT, we coherently map single photons onto the atoms which travel as coupled excitations of light and matter called dark-state polaritons. When the medium is optically dense, the polariton propagates as a massive particle with a velocity that is much smaller than the speed of light. These polaritons interact with each other via their atomic component. In this thesis, we show robust symmetry-protected collisions between photons that imprint a large phase of π/2 with little loss and extend the nature of photon-photon interactions to the repulsive regime, which are essential for quantum communication and metrology. We use the technique of photon blockade to make a fast optical detector of Rydberg states, directly demonstrating the use of quantum nonlinear optics for quantum computation. We also study the extensions of the attractive and repulsive photons for three particles shedding light into the formation of bound states and crystals of photons and paving the way to studying many-body physics of photons.Most phenomena around us can be explained by classical optics since photons interact weakly with atoms. When the interaction is strong enough where one photon affects the properties of other photons, we go to the regime of quantum photon-photon nonlinear optics. The work in this thesis explores this regime of physics. This paves the path to exploring strongly interacting many-body physics with photons which is still a largely unexplored domain. The ability to control strongly interacting photons is also of central importance in quantum science and engineering. We use the approach of Electromagnetically Induced Transparency (EIT) in atomic ensembles to create strong interactions and demonstrate coherent control between single photons. Using EIT, we coherently map single photons onto the atoms which travel as coupled excitations of light and matter called dark-state polaritons. When the medium is optically dense, the polariton propagates as a massive particle with a velocity that is much smaller than the speed of light. These polaritons interact with each other via their atomic component. In this thesis, we show robust symmetry-protected collisions between photons that imprint a large phase of π/2 with little loss and extend the nature of photon-photon interactions to the repulsive regime, which are essential for quantum communication and metrology. We use the technique of photon blockade to make a fast optical detector of Rydberg states, directly demonstrating the use of quantum nonlinear optics for quantum computation. We also study the extensions of the attractive and repulsive photons for three particles shedding light into the formation of bound states and crystals of photons and paving the way to studying many-body physics of photons.

Jan 1, 20210 citations

Photonic quantum transport in a nonlinear optical fiber

Mohammad Hafezi, Darrick E. Chang, Vladimir Gritsev +2 more

We theoretically study the transmission of few-photon quantum fields through a strongly nonlinear optical medium. We develop a general approach to investigate nonequilibrium quantum transport of bosonic fields through a finite-size nonlinear medium and apply it to a recently demonstrated experimental system where cold atoms are loaded in a hollow-core optical fiber. We show that when the interaction between photons is effectively repulsive, the system acts as a single-photon switch. In the case of attractive interaction, the system can exhibit either antibunching or bunching, associated with the resonant excitation of bound states of photons by the input field. These effects can be observed by probing statistics of photons transmitted through the nonlinear fiber.We theoretically study the transmission of few-photon quantum fields through a strongly nonlinear optical medium. We develop a general approach to investigate nonequilibrium quantum transport of bosonic fields through a finite-size nonlinear medium and apply it to a recently demonstrated experimental system where cold atoms are loaded in a hollow-core optical fiber. We show that when the interaction between photons is effectively repulsive, the system acts as a single-photon switch. In the case of attractive interaction, the system can exhibit either antibunching or bunching, associated with the resonant excitation of bound states of photons by the input field. These effects can be observed by probing statistics of photons transmitted through the nonlinear fiber.

arXiv:0907.5206Europhysics Letters (EPL)May 27, 201126 citations

Two-photon self-Kerr nonlinearities for quantum computing and quantum optics

Joshua Combes, Daniel J. Brod

The self-Kerr interaction is an optical nonlinearity that produces a phase shift proportional to the square of the number of photons in the field. At present, many proposals use nonlinearities to generate photon-photon interactions. For propagating fields these interactions result in undesirable features such as spectral correlation between the photons. Here we engineer a discrete network composed of cross-Kerr interaction regions to simulate a self-Kerr medium. The medium has effective long-range interactions implemented in a physically local way. We compute the one- and two-photon $S$ matrices for fields propagating in this medium. From these scattering matrices we show that our proposal leads to a high-fidelity photon-photon gate. In the limit where the number of nodes in the network tends to infinity, the medium approximates a perfect self-Kerr interaction in the one- and two-photon regime.The self-Kerr interaction is an optical nonlinearity that produces a phase shift proportional to the square of the number of photons in the field. At present, many proposals use nonlinearities to generate photon-photon interactions. For propagating fields these interactions result in undesirable features such as spectral correlation between the photons. Here we engineer a discrete network composed of cross-Kerr interaction regions to simulate a self-Kerr medium. The medium has effective long-range interactions implemented in a physically local way. We compute the one- and two-photon $S$ matrices for fields propagating in this medium. From these scattering matrices we show that our proposal leads to a high-fidelity photon-photon gate. In the limit where the number of nodes in the network tends to infinity, the medium approximates a perfect self-Kerr interaction in the one- and two-photon regime.

arXiv:1804.08531Physical Review ADec 10, 201822 citations

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matrices for fields propagating in this medium. From these scattering matrices we show that our proposal leads to a high-fidelity photon-photon gate. In the limit where the number of nodes in the network tends to infinity, the medium approximates a perfect self-Kerr interaction in the one- and two-photon regime.