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Conference on Lasers and Electro-Optics

Helicity in a Twist: Attosecond, Extreme Ultraviolet Vortex Beams with Designer Spin and Orbital Angular Momenta

Kevin M. Dorney, Laura Rego, Nathan J. Brooks, Julio San Román, Chen-Ting Liao, Jennifer L. Ellis, Dmitriy H. Zusin, Christian Gentry, Quynh L. Nguyen, Justin M. Shaw, Antonio Picón, Luis Plaja, Henry C. Kapteyn, Margaret M. Murnane, Carlos Hernández-García

Published May 5, 2019• 0 citations
Publisher

Abstract

High-harmonies-and attosecond pulses-with controllable spin and orbital angular momenta (SAM and OAM) are generated for the first time. The coupled SAM-OAM conservation laws enable exquisite control over the polarization of attosecond pulse trains. © 2019 The Author(s)
DOI
10.23919/cleo.2019.8749379

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In 1992, Les Allen and coworkers within Han Woerdman's group realized that light beams with an azimuthal phase dependence described by an additional exp(iℓθ) term, where ℓ can take any integer value and θ is the angular position within the beam, carry an orbital angular momentum. This orbital angular momentum is additional to the spin angular momentum associated with circular polarization. These azimuthally phased beams comprise ℓ intertwined helical phase fronts, skewed with respect to the beam axis, meaning that at all positions within the beam cross section, the wavefront normal and associated momentum density has a well-defined azimuthal component. The insight of Allen and coworkers was that for all beams described in this way, when integrated over the beam cross section, the orbital angular momentum (OAM) is ℓℏ per photon. Laguerre-Gaussian and high-order Bessel beams are both examples of mode families having these properties. A further feature of these beams is that the phase singularity on the beam axis precludes a nonzero on-axis intensity and therefore all such beams with ℓ ≠0 have an annular intensity cross section (see Fig. 4.1). The circulation of the optical momentum and energy around the singularity leads them also to be called optical vortices. The further recognition that beams carrying defined amounts of OAM could be created within the laboratory means that over the last 15 years they have formed the basis of many investigations, ranging from the transfer of OAM to microscopic particles (in optical spanners or optical wrenches) to studies of the fundamental properties of light in both the classical and quantum regimes. However, although OAM is an immensely useful concept, one must emphasize that all its properties are simply those predicted by standard electromagnetic theory. The purpose of this chapter is to consider how sets of helical laser modes carrying OAM can be used for information transfer.

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In 1992, Les Allen and coworkers within Han Woerdman's group realized that light beams with an azimuthal phase dependence described by an additional exp(iℓθ) term, where ℓ can take any integer value and θ is the angular position within the beam, carry an orbital angular momentum. This orbital angular momentum is additional to the spin angular momentum associated with circular polarization. These azimuthally phased beams comprise ℓ intertwined helical phase fronts, skewed with respect to the beam axis, meaning that at all positions within the beam cross section, the wavefront normal and associated momentum density has a well-defined azimuthal component. The insight of Allen and coworkers was that for all beams described in this way, when integrated over the beam cross section, the orbital angular momentum (OAM) is ℓℏ per photon. Laguerre-Gaussian and high-order Bessel beams are both examples of mode families having these properties. A further feature of these beams is that the phase singularity on the beam axis precludes a nonzero on-axis intensity and therefore all such beams with ℓ ≠0 have an annular intensity cross section (see Fig. 4.1). The circulation of the optical momentum and energy around the singularity leads them also to be called optical vortices. The further recognition that beams carrying defined amounts of OAM could be created within the laboratory means that over the last 15 years they have formed the basis of many investigations, ranging from the transfer of OAM to microscopic particles (in optical spanners or optical wrenches) to studies of the fundamental properties of light in both the classical and quantum regimes. However, although OAM is an immensely useful concept, one must emphasize that all its properties are simply those predicted by standard electromagnetic theory. The purpose of this chapter is to consider how sets of helical laser modes carrying OAM can be used for information transfer.
We investigate the propagation of an optical vector vortex weakly interacting with a coherently prepared atomic medium (phaseonium) in a three-level ΛΛΛ configuration. The vector beam consists of vortex pulse pairs with right- and left-circular polarizations, corresponding to opposite spin angular momentum (SAM), and carrying opposite orbital angular momentum (OAM) charges ±l\pm l±l. We show that during the propagation of the vortex pairs, analytically obtained in the linear regime, the medium inherits the topology of the vortex pair, mapping the OAM onto a spatially structured atomic coherence. This mapping produces 2∣l∣−2|l|-2∣l∣−fold azimuthal transparency structures that reshape the beam intensity from a ring into a petal-like pattern. The OAM-structured atomic coherence induces a corresponding optical anisotropy within the medium, which feeds back into the propagating vector beam, resulting in optical spin-orbit coupling manifested as SAM exchange, rotation, and evolution of polarization textures. Depending on the initial ground-state population of the phaseonium, the polarization state evolves between left-circular, linear, and right-circular polarizations.
The exchange of orbital angular momentum (OAM) between paraxial optical vortex and a Bose-Einstein condensate (BEC) of atomic gases is well known. In this paper, we develop a theory for the microscopic interaction between matter and an optical vortex beyond paraxial approximation. We show how superposition of vortex states of BEC can be created with a focused optical vortex. Since the polarization or spin angular momentum (SAM) of the optical field is coupled with OAM of the field, in this case, these angular momenta can be transferred to the internal electronic and external center-of-mass motion of atoms provided both the motions are coupled. We propose a scheme for producing the superposition of matter-wave vortices using Gaussian and a focused Laguerre-Gaussian beam. We study how two-photon Rabi frequencies of stimulated Raman transitions vary with focusing angles for different combinations of OAM and SAM of optical states. We demonstrate the formation of vortex-antivortex structure and discuss interference of three vortex states in a BEC.