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Bulletin of the American Physical Society

Novel Phases and Chiral Interactions in Spin-1 Magnets

Ciarán Hickey

Published Mar 9, 2018• 0 citations
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The frustrated XY model on the honeycomb lattice has drawn lots of attention because of the potential emergence of chiral spin liquid (CSL) with the increasing of frustrations or competing interactions. In this paper, we study the extended spin-$\frac{1}{2}$ XY model with nearest-neighbor $({J}_{1})$, and next-nearest-neighbor $({J}_{2})$ interactions in the presence of a three-spins chiral $({J}_{\ensuremath{\chi}})$ term using density matrix renormalization group methods. We obtain a quantum phase diagram with both conventionally ordered and topologically ordered phases. In particular, the long-sought Kalmeyer-Laughlin CSL is shown to emerge under a small ${J}_{\ensuremath{\chi}}$ perturbation due to the interplay of the magnetic frustration and chiral interactions. The CSL, which is a nonmagnetic phase, is identified by the scalar chiral order, the finite spin gap on a torus, and the chiral entanglement spectrum described by chiral $SU{(2)}_{1}$ conformal field theory.

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We obtain the ground-state phase diagram of two spin chains consisting in a set of two-level systems asymmetrically coupled to an XX chain through a chiral interaction. The interaction is parametrized by its magnitude and an angle defined by the relative orientation of the spins in different chains. From the entanglement spectrum, we identify the critical lines separating distinct magnetically ordered phases, with the interaction angle able to shift or fully suppress the transition. By increasing the coupling strength, the system is driven through a quantum phase transition, leading to the formation of two types of in-plane antiferromagnetic stripes. The interaction strength sets stripe formation, while the angle controls the spins' orientations. The chiral interaction also induces a nontrivial finite vector spin chirality with opposite orientation on the chains. We show that the vector spin chirality emerges smoothly from the decoupled limit and occurs for angles different from zero and π / 2 , where collinear order is favored instead.
We study the spin-1/21/21/2 Heisenberg model on the triangular lattice with the nearest-neighbor J1>0{J}_{1}>0J1​>0, the next-nearest-neighobr J2>0{J}_{2}>0J2​>0 Heisenberg interactions, and the additional scalar chiral interaction ${J}_{\ensuremath{\chi}}({\stackrel{P\vec}{S}}_{i}\ifmmode\times\else\texttimes\fi{}{\stackrel{P\vec}{S}}_{j})\ifmmode\cdot\else\textperiodcentered\fi{}{\stackrel{P\vec}{S}}_{k}$ for the three spins in all the triangles using large-scale density matrix renormalization group calculation on cylinder geometry. With increasing J2{J}_{2}J2​ (${J}_{2}/{J}_{1}\ensuremath{\le}0.3$) and ${J}_{\ensuremath{\chi}}$ (${J}_{\ensuremath{\chi}}/{J}_{1}\ensuremath{\le}1.0$) interactions, we establish a quantum phase diagram with the magnetically ordered ${120}^{\ensuremath{\circ}}$, stripe, and noncoplanar tetrahedral phase. In between these magnetic order phases, we find a chiral spin liquid (CSL) phase, which is identified as a $\ensuremath{\nu}=1/2$ bosonic fractional quantum Hall state with possible spontaneous rotational symmetry breaking. By switching on the chiral interaction, we find that the previously identified spin liquid in the ${J}_{1}\ensuremath{-}{J}_{2}$ triangular model ($0.08\ensuremath{\lesssim}{J}_{2}/{J}_{1}\ensuremath{\lesssim}0.15$) shows a phase transition to the CSL phase at very small ${J}_{\ensuremath{\chi}}$. We also compute the spin triplet gap in both spin liquid phases, and our finite-size results suggest a large gap in the odd topological sector but a small or vanishing gap in the even sector. We discuss the implications of our results on the nature of the spin liquid phases.
The frustrated XY model on the honeycomb lattice has drawn lots of attention because of the potential emergence of chiral spin liquid (CSL) with the increasing of frustrations or competing interactions. In this paper, we study the extended spin-12\frac{1}{2}21​ XY model with nearest-neighbor (J1)({J}_{1})(J1​), and next-nearest-neighbor (J2)({J}_{2})(J2​) interactions in the presence of a three-spins chiral $({J}_{\ensuremath{\chi}})$ term using density matrix renormalization group methods. We obtain a quantum phase diagram with both conventionally ordered and topologically ordered phases. In particular, the long-sought Kalmeyer-Laughlin CSL is shown to emerge under a small ${J}_{\ensuremath{\chi}}$ perturbation due to the interplay of the magnetic frustration and chiral interactions. The CSL, which is a nonmagnetic phase, is identified by the scalar chiral order, the finite spin gap on a torus, and the chiral entanglement spectrum described by chiral SU(2)1SU{(2)}_{1}SU(2)1​ conformal field theory.