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Bulletin of the American Physical Society

Chiral phase of a simple two-dimensional spin-1 quantum magnet

Oleg A. Starykh, Zhentao Wang, Cristian D. Batista

Published Mar 15, 2016• 0 citations
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Emergent quasi-one-dimensionality in a kagome magnet: A simple route to complexity

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We study the ground-state phase diagram of the quantum $\text{spin-}1/2$ Heisenberg model on the kagome lattice with first- $({J}_{1}<0)$, second- $({J}_{2}<0)$, and third-neighbor interactions $({J}_{d}>0)$ by means of analytical low-energy field theory and numerical density-matrix renormalization group (DMRG) studies. The results offer a consistent picture of the ${J}_{d}\text{-dominant}$ regime in terms of three sets of spin chains weakly coupled by the ferromagnetic interchain interactions ${J}_{1,2}$. When either ${J}_{1}$ or ${J}_{2}$ is much stronger than the other one, the model is found to support one of two cuboctohedral phases, cuboc1, and cuboc2. These cuboc states host noncoplanar long-ranged magnetic order and possess finite scalar spin chirality. However, in the compensated regime ${J}_{1}\ensuremath{\simeq}{J}_{2}$, a valence bond crystal phase emerges between the two cuboc phases. We find excellent agreement between an analytical theory based on coupled spin chains and unbiased DMRG calculations, including at a very detailed level of comparison of the structure of the valence bond crystal state. To our knowledge, this is the first such comprehensive understanding of a highly frustrated two-dimensional quantum antiferromagnet. We find no evidence of either the one-dimensional gapless spin liquid or the chiral spin liquids, which were previously suggested by parton mean-field theories.

arXiv:1604.01459•Physical review. B./Physical review. B•Jul 27, 2016•27 citations
A current challenge in condensed matter physics is the search for novel quantum states of matter. In this paper, the authors provide a simple guiding principle for finding quantum spin liquids in real materials. Like in the case of unconventional superconductivity that involves pairing of two fermions into a bound state, it is shown here that chiral quantum liquids naturally emerge in the vicinity of a class of magnetic quantum critical points, due to pairing of two bosons into a bound state of zero total spin.
A peculiar manifestation of the Aharonov-Bohm effect in Mott insulators, presents as a versatile scheme to manipulate the intriguing ground-state spin chirality, such as, tune the magnitude continuously, switch an abrupt jump, or even reverse its sign from a para-chiral phase to a dia-chiral phase. Such an unusual mechanism is due to the coupling between multiple-spin ring exchanges and magnetic flux, and the competition between spin chirality and magnetism, and is demonstrated explicitly in both quasi-one-dimensional ladders and two-dimensional lattices with triangles as elementary plaquettes.
We study the ground-state phase diagram of the quantum spin-1/2\text{spin-}1/2spin-1/2 Heisenberg model on the kagome lattice with first- (J1<0)({J}_{1}<0)(J1​<0), second- (J2<0)({J}_{2}<0)(J2​<0), and third-neighbor interactions (Jd>0)({J}_{d}>0)(Jd​>0) by means of analytical low-energy field theory and numerical density-matrix renormalization group (DMRG) studies. The results offer a consistent picture of the Jd-dominant{J}_{d}\text{-dominant}Jd​-dominant regime in terms of three sets of spin chains weakly coupled by the ferromagnetic interchain interactions J1,2{J}_{1,2}J1,2​. When either J1{J}_{1}J1​ or J2{J}_{2}J2​ is much stronger than the other one, the model is found to support one of two cuboctohedral phases, cuboc1, and cuboc2. These cuboc states host noncoplanar long-ranged magnetic order and possess finite scalar spin chirality. However, in the compensated regime ${J}_{1}\ensuremath{\simeq}{J}_{2}$, a valence bond crystal phase emerges between the two cuboc phases. We find excellent agreement between an analytical theory based on coupled spin chains and unbiased DMRG calculations, including at a very detailed level of comparison of the structure of the valence bond crystal state. To our knowledge, this is the first such comprehensive understanding of a highly frustrated two-dimensional quantum antiferromagnet. We find no evidence of either the one-dimensional gapless spin liquid or the chiral spin liquids, which were previously suggested by parton mean-field theories.