A current challenge in condensed matter physics is the search for novel quantum states of matter. In this paper, the authors provide a simple guiding principle for finding quantum spin liquids in real materials. Like in the case of unconventional superconductivity that involves pairing of two fermions into a bound state, it is shown here that chiral quantum liquids naturally emerge in the vicinity of a class of magnetic quantum critical points, due to pairing of two bosons into a bound state of zero total spin.
A peculiar manifestation of the Aharonov-Bohm effect in Mott insulators, presents as a versatile scheme to manipulate the intriguing ground-state spin chirality, such as, tune the magnitude continuously, switch an abrupt jump, or even reverse its sign from a para-chiral phase to a dia-chiral phase. Such an unusual mechanism is due to the coupling between multiple-spin ring exchanges and magnetic flux, and the competition between spin chirality and magnetism, and is demonstrated explicitly in both quasi-one-dimensional ladders and two-dimensional lattices with triangles as elementary plaquettes.
We study the ground-state phase diagram of the quantum
spin-1/2 Heisenberg model on the kagome lattice with first-
(J1<0), second-
(J2<0), and third-neighbor interactions
(Jd>0) by means of analytical low-energy field theory and numerical density-matrix renormalization group (DMRG) studies. The results offer a consistent picture of the
Jd-dominant regime in terms of three sets of spin chains weakly coupled by the ferromagnetic interchain interactions
J1,2. When either
J1 or
J2 is much stronger than the other one, the model is found to support one of two cuboctohedral phases, cuboc1, and cuboc2. These cuboc states host noncoplanar long-ranged magnetic order and possess finite scalar spin chirality. However, in the compensated regime ${J}_{1}\ensuremath{\simeq}{J}_{2}$, a valence bond crystal phase emerges between the two cuboc phases. We find excellent agreement between an analytical theory based on coupled spin chains and unbiased DMRG calculations, including at a very detailed level of comparison of the structure of the valence bond crystal state. To our knowledge, this is the first such comprehensive understanding of a highly frustrated two-dimensional quantum antiferromagnet. We find no evidence of either the one-dimensional gapless spin liquid or the chiral spin liquids, which were previously suggested by parton mean-field theories.