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Bulletin of the American Physical Society

Counterpropagating light as a means for all-optical phase matching

Amy L. Lytle, Eric Dyke, Etienne Gagnon

Published Mar 6, 2019• 0 citations
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Entangled photons, which may be generated through the process of spontaneous parametric down-conversion (SPDC) in a crystal with /spl chi//sup (2)/ nonlinearity, have long been in the spotlight for quantum-optics experiments. The generation of entangled photons by quasi-phase matching (QPM) in lithium niobate offers the promise of increased photon-pair production and, with the integration of a waveguide structure, control of the spatial characteristics of the down-converted photons. It turns out that the use of a waveguide structure, in conjunction with periodic poling to achieve quasi-phase matching, offers another critically important feature: the possibility of generating counterpropagating signal and idler photons. We consider the conditions required for generating counterpropagating photon beams and explore some of the unique properties of this source of light using a periodically poled LiNbO/sub 3/ waveguide.
The stationary light pulse (SLP) refers to a zero-group-velocity optical pulse in an atomic ensemble prepared by two counterpropagating driving fields. Despite the uniqueness of an optical pulse trapped within an atomic medium without a cavity, observations of SLP so far have been limited to trapping a single optical pulse due to the stringent SLP phase-matching condition, and this has severely hindered the development of SLP-based applications. In this Letter, we first show theoretically that the SLP process in fact supports two phase-matching conditions and we then utilize the result to experimentally demonstrate simultaneous SLP trapping of two optical pulses for the duration from 0.8 to 2.0 μs. The characteristic dissipation time, obtained by the release efficiency measurement from the SLP trapping state, is 1.22 μs, which corresponds to an effective Q factor of 2.9×10^{9}. Our Letter is expected to bring forth interesting SLP-based applications, such as, efficient photon-photon interaction, spatially multimode coherent quantum memory, creation of exotic photonic gas states, etc.
Nonlinear metasurfaces have recently been established as a new platform for generating photon pairs via spontaneous parametric down-conversion. While for classical harmonic generation in metasurfaces a high level of control over all degrees of freedom of light has been reached, this capability is yet to be developed for photon-pair generation. In this work, we theoretically and experimentally demonstrate for the first time precise control of the emission angle of photon pairs generated from a nonlinear metasurface. Our measurements show angularly tunable pair generation with high coincidence-to-accidental ratio for both co- and counterpropagating emission. The underlying principle is the transverse phase matching of guided-mode resonances with strong angular dispersion in a nonlinear metasurface consisting of a silicon dioxide grating on a nonlinear lithium niobate guiding layer. We provide a straightforward design strategy for photon-pair generation in such a device and find very good agreement between the calculations and experimental results. Here, we use all-optical emission angle tuning by means of the pump wavelength; however, the principle could be extended to modulation via the electro-optic effect in lithium niobate. In sum, this work provides an important addition to the toolset of subwavelength thickness photon-pair sources.